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nitrogenous and carbonaceous aerosols in PM_(2.5) and TSP during pre-monsoon:Characteristics and sources in the highly polluted mountain valley

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Journal of Environmental Sciences 2022年第5期34卷 10-24页

作者： Hemraj Bhattarai Lekhendra Tripathee Shichang Kang Pengfei Chen Chhatra Mani Sharma Kirpa Ram Junming Guo Maheswar Rupakheti Earth System Science Programme and Graduate Division of Earth and Atmospheric Sciences The Chinese University of Hong KongHong KongChina State Key Laboratory of Cryospheric Science Northwest Institute of Eco-environment and ResourcesChinese Academy of Sciences(CAS)Lanzhou 730000China Key Laboratory of Tibetan Environment Changes and Land Surface Processes Institute of Tibetan Plateau ResearchCASBeijing 100101China CAS Center for Excellence in Tibetan Plateau Earth Sciences Beijing 100085China Himalayan Environment Research Institute(HERI) Kathmandu 44602Nepal Central Department of Environmental Sciences Tribhuvan UniversityKathmandu 44613Nepal Institute of Environment and Sustainable Development Banaras Hindu UniversityVaranasi 221005India Institute for Advanced Sustainability Studies Potsdam 14467Germany

This study reports for the first time a comprehensive analysis of nitrogenous and carbona-ceous aerosols in simultaneously collected PM_(2.5) and TSP during pre-monsoon(March-May 2018)from a highly polluted urban Kathmandu Valley(KV)of the Himalayan *** mean mass concentration of PM_(2.5)(129.8 μg/m^(3))was only-25%of TSP mass(558.7 μg/m^(3))indicating the dominance of coarser mode ***,the mean concentration as well as fractional contributions of water-soluble total nitrogen(WSTN)and carbonaceous species reveal their predominance in find-mode *** mean mass concentration of WSTN was 17.43±4.70 μg/m^(3)(14%)in PM_(2.5) and 24.64±8.07 μg/m^(3)(5%)in ***,the fractional contribution of total carbonaceous aerosols(TCA)is much higher in PM_(2.5)(~34%)than that in TSP(~20%).The relatively low OC/EC ratio in PM_(2.5)(3.03±1.47)and TSP(4.64±1.73)suggests fossil fuel combustion as the major sources of carbonaceous aerosols with contributions from secondary organic ***-day air mass back trajectories sim-ulated with the HYSPLIT model,together with MODIS fire counts indicate the influence of local emissions as well as transported pollutants from the Indo-Gangetic Plain region to the south of the Himalayan *** component analysis(PCA)also suggests a mixed contribution from other local anthropogenic,biomass burning,and crustal *** re-sults highlight that it is necessary to control local emissions as well as regional transport while designing mitigation measures to reduce the KV's air pollution.

关键词： nitrogenous aerosol Carbonaceous aerosols Major ions Particulate pollution Kathmandu Valley(KV)

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