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Thickness evolution of commercial Li-ion pouch cells with siliconbased composite anodes and nca cathodes

Science China(Technological Sciences) 2021年第1期64卷 83-90页

作者： ZHANG XingYu HE Jie ZHOU Jiang CHEN HaoSen SONG WeiLi FANG DaiNing State Key Laboratory of Mechanics and Control of Mechanical Structures College of Aerospace EngineeringNanjing University of Aeronautics and AstronauticsNanjing 210016China State Key Laboratory of Explosion Science and Technology Institute of Advanced Structure TechnologyBeijing Institute of TechnologyBeijing 100081China Lishen Research Institute Tianjin Lishen Battery Joint-stock Co.Ltd.Tianjin 300384China State Key Laboratory for Turbulence and Complex Systems College of EngineeringPeking UniversityBeijing 100871China

It is significant to monitor the thickness change of commercial Li-ion pouch cells that are assembled from Si-based electrodes and layered cathodes since the volume variation is critically linked with kinetic reaction mechanism and chemomechanical degradation. In this work, the single-point and full-field measurements are conducted on the thickness evolution of Si Ox/Cgraphite/lithium nickel-cobalt-aluminum oxide(Si Ox-G/nca) batteries. It is found that an abnormal overshoot that has been rarely observed in the previous studies appears at the beginning of discharge, which is believed to be the combined results between the rapid expansion of nca and the contraction of graphite related to the state of charge(SOC). Compared with the results of single-point measurement, the spatial displacement distribution obtained from three-dimensional(3D) scanning suggests the full-field thickness evolution of the entire cell scale, which is more feasible and efficient to provide full-field information for supporting pouch cell design and pack integration.

关键词： thickness change 3D scanning silicon-based anode nca cathode lithium-ion battery

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