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Study of the growth mechanism of a self‑assembled and ordered multi‑dimensional heterojunction at atomic resolution

Frontiers of Optoelectronics 2023年第4期16卷 37-48页

作者： Zunyu Liu Chaoyu Zhao Shuangfeng Jia Weiwei Meng Pei Li Shuwen Yan Yongfa Cheng Jinshui Miao Lei Zhang Yihua Gao Jianbo Wang Luying Li Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074China Ministry-of-Education Key Laboratory for the Green Preparation and Application of Functional materials Hubei Collaborative Innovation Center for Advanced Organic Chemical MaterialsSchool of Materials Science and EngineeringHubei UniversityWuhan 430061China Center for Electron Microscopy MOE Key Laboratory of Artificial Micro-and Nano-Structures and the Institute for Advanced StudiesSchool of Physics and TechnologyWuhan UniversityWuhan 430072China State Key Laboratory of Infrared Physics Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China

multi-dimensional heterojunction materials have attracted much attention due to their intriguing properties,such as high efciency,wide band gap regulation,low dimensional limitation,versatility and *** further improve the performance of materials,researchers have combined materials with various dimensions using a wide variety of ***,research on growth mechanism of such composite materials is still *** this paper,the growth mechanism of multidimensional heterojunction composite material is studied using quasi-two-dimensional(quasi-2D)antimonene and quasione-dimensional(quasi-1D)antimony sulfde as *** are synthesized by a simple thermal injection *** is observed that the consequent nanorods are oriented along six-fold symmetric directions on the nanoplate,forming ordered quasi-1D/quasi-2D *** transmission electron microscopy(TEM)characterizations confrm the chemical information and reveal orientational relationship between Sb2S3 nanorods and the Sb nanoplate as *** density functional theory calculations indicate that interfacial binding energy is the primary deciding factor for the self-assembly of ordered *** details may fll the gaps in the research on multi-dimensional composite materials with ordered structures,and promote their future versatile applications.

关键词： multi-dimensional composite materials Ordered heterostructures-Self-assembly Growth mechanism

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