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Interfacial parasitic reactions of zinc anodes in zinc ion batteries:Underestimated corrosion and hydrogen evolution reactions and their suppression strategies

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Journal of Energy Chemistry 2022年第1期31卷 246-262,I0007页

作者： Aruuhan Bayaguud Yanpeng Fu Changbao Zhu State Key Laboratory of Optoelectronic Materials and Technologies Department of Materials Science and EngineeringKey Laboratory for Polymeric Composite and Functional Materials of Ministry of EducationSun-Yat Sen UniversityGuangzhou 510275GuangdongChina School of Materials and Energy Guangdong University of TechnologyGuangzhou 510006GuangdongChina

Featured with high power density,improved safety and low-cost,rechargeable aqueous zinc-ion batteries(ZIBs) have been revived as possible candidates for sustainable energy storage systems in recent ***,the challenges inherent in zinc(Zn) anode,namely dendrite formation and interfacial parasitic reactions,have greatly impeded their practical *** the critical issue of dendrite formation has attracted widespread concern,the parasitic reactions of Zn anodes with mildly acidic electrolytes have received very little *** that the low Zn reversibility that stems from interfacial parasitic reactions is the major obstacle to the commercialization of ZIBs,thorough understanding of these side reactions and the development of correlative inhibition strategies are ***,in this review,the brief fundamentals of corrosion and hydrogen evolution reactions at Zn surface is *** addition,recent advances and research efforts addressing detrimental side reactions are reviewed from the perspective of electrode design,electrode-electrolyte interfacial engineering and electrolyte *** facilitate the future researches on this aspect,perspectives and suggestions for relevant investigations are provided lastly.

关键词： Zinc anodes mildly acidic electrolytes Side reactions Coulombic efficiency Corrosions HER

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