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Magnesium-based energy materials: Progress, challenges, and perspectives

Journal of Magnesium and Alloys 2023年第11期11卷 3896-3925页

作者： Guang Han Yangfan Lu Hongxing Jia Zhao Ding Liang Wu Yue Shi Guoyu Wang Qun Luo Yu'an Chen Jingfeng Wang Guangsheng Huang Xiaoyuan Zhou Qian Li Fusheng Pan National Engineering Research Center for Magnesium Alloys Chongqing UniversityChongqing 400044China College of materials Science and Engineering Chongqing UniversityChongqing 400044China National Key Laboratory of Advanced Casting Technologies Chongqing UniversityChongqing 400044China Chongqing Institute of New Energy Storage materials and Equipment Chongqing 401135China State Key Laboratory of Advanced Special Steels Shanghai Key Laboratory of Advanced FerrometallurgySchool of Materials Science and EngineeringShanghai UniversityShanghai 200444China College of Physics Chongqing UniversityChongqing 401331China

Magnesium-based energy materials, which combine promising energy-related functional properties with low cost, environmental compatibility and high availability, have been regarded as fascinating candidates for sustainable energy conversion and storage. In this review,we provide a timely summary on the recent progress in three types of important mg-based energy materials, based on the fundamental strategies of composition and structure engineering. With regard to mg-based materials for batteries, we systematically review and analyze different material systems, structure regulation strategies as well as the relevant performance in mg-ion batteries(MIBs) and mg-air batteries(MABs), covering cathodes, electrolytes, anodes for MIBs, and anodes for MABs;as to mg-based hydrogen storage materials, we discuss how catalyst adding, composite, alloying and nanostructuring improve the kinetic and thermodynamic properties of de/hydrogenation reactions, and in particular, the impacts of composition and structure modification on hydrogen absorption/dissociation processes and free energy modification mechanism are focused;regarding mg-based thermoelectric materials, the relations between composition/structure and electrical/thermal transport properties of mg_(3)X_(2)(X = Sb, Bi), mg_(2)X(X = Si, Ge, Sn) and mg Ag Sb-based materials, together with the representative research progress of each material system, are summarized and discussed. Finally, by pointing out remaining challenges and providing possible solutions, this review aims to shed light on the directions and perspectives for practical applications of magnesium-based energy materials in the future.

关键词： mg-based battery materials mg-based hydrogen storage materials mg-based thermoelectric materials Composition regulation Structure engineering

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