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Trace metal leaching from Cookware Locally Fabricated from Scrap metal: A Case Study of Ntungamo District, Uganda

American Journal of Analytical Chemistry 2022年第9期13卷 314-330页

作者： Samuel Habimaana Hannington Gumisiriza Grace Birungi Department of Chemistry Faculty of Science Mbarara University of Science and Technology Mbarara Uganda

Heavy metal exposure remains a significant public health problem, particularly in sub-Saharan Africa where use of artisanal cookware made from recycled metallic materials is still common. In this study, the effect of cookware composition, cleaning material, heating duration and temperature on metal migration from different cookware, including artisanal pans was investigated. Trace element concentrations were determined with Inductively Coupled Plasma Optical Emission Spectrometry (ICP-OES). Locally fabricated cookware leached the highest levels of metals, where the levels of Pb (9.00 ± 0.80 × 10-2 mg/l), Al (11.40 ± 0.02 × 10-2 mg/l), Cd (5.80 ± 0.30 × 10-2 mg/l), Cr (6.60 ± 0.03 × 10-2 mg/l) and Ni (3.00 ± 0.01 × 10-2 mg/l) were above the WHO permissible limits of heavy metals for drinking water. Steel wire was the most aggressive cleaning material to the cookware surfaces, followed by sand and then ash. For cookware heated at 100°C and above, an exponential relationship between temperature and the migration of Al, Pb and Cd was observed. The findings revealed heavy metal exposure from cookware usage, which poses potential health risks to the population. There is need for policies and civic education to minimize this exposure.

关键词： Local Fabrication Cookware metal leaching Scrap metal Uganda

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A magnetic-void-porous MnFe_(2)O_(4)/carbon microspheres nano-catalyst for catalytic ozonation:Preparation,performance and mechanism

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Environmental Science and Ecotechnology 2021年第3期7卷 35-47页

作者： Xiaoguang Jin Changyong Wu Xiangmiao Tian Panxin Wang Yuexi Zhou Jiane Zuo State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing100012China Research Center of Environmental Pollution Control Engineering Technology Chinese Research Academy of Environment SciencesBeijing100012China

Wastewater treatment is essential to guarantee human health and ecological *** ozonation with nanocatalysts is a widely studied and efficient treatment ***,this method has always been limited by nanocatalysts disadvantages such as easily loss,difficult to separate and reuse,and catalytic ability decay caused by aggregation,which could cause severe resources waste and potential risk to human health and *** remedy these challenges,a magnetic-void-porous MnFe_(2)O_(4)/carbon microsphere shell nanocatalyst(CMS-MnFe_(2)O_(4))was successfully synthesized using renewable natural *** separation test showed CMS-MnFe_(2)O_(4) was rapidly separated within 2 min under an external magnetic *** catalytic ozonation of oxalic acid(OA),CMS-MnFe_(2)O_(4) showed efficient and stable catalytic efficiency,reaching a maximum total organic carbon removal efficiency of 96.59% and maintained a 93.88% efficiency after 4 *** stable catalytic efficiency was due to the supporting effects of the carbon microsphere shell,which significantly enhanced CMS-MnFe_(2)O_(4) chemical stability and reduced the metal ions leaching to 10-20% of MnFe_(2)O_(4) through electron *** explore the catalytic mechanism,radical experiments were conducted and a new degradation pathway of OA involving superoxide anions rather than hydroxyl radicals was ***,this study suggests that an efficient,recyclable,stable,and durable catalyst for catalytic ozonation could be prepared.

关键词： Catalytic ozonation Magnetic nanocatalyst Separation recycling Catalytic mechanism metal leaching

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