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Metal–Organic Frameworks and Their derivatives as Cathodes for Lithium‑Ion Battery Applications:A Review

Electrochemical Energy Reviews 2022年第2期5卷 312-347页

作者： R.Chenna Krishna Reddy Xiaoming Lin Akif Zeb Cheng‑Yong Su Guangzhou Key Laboratory of Materials for Energy Conversion and Storage Key Laboratory of Theoretical Chemistry of EnvironmentMinistry of EducationSchool of ChemistrySouth China Normal UniversityGuangzhou 510006GuangdongChina China MOE Laboratory of Bioinorganic and Synthetic Chemistry Lehn Institute of Functional MaterialsSchool of ChemistrySun Yat-Sen UniversityGuangzhou 510275GuangdongChina

The development of energy storage technology is important for resolving the issues and challenges of utilizing sustainable green energy in modern-day *** an emerging technology,lithium-ion batteries(LIBs)are a common source of power for a wide variety of electronic devices,and major advances require the development and exploitation of new electrode materials;thus,fundamental knowledge of their atomic and nanoscale properties is *** moving beyond conven-tional cathode candidates,metal–organic frameworks(mofs)chemistry provides an excellent direction for designing and developing promising high-performance cathode materials for use in ***,we carry out an overarching discussion on the development and application of mofs and their derivatives as cathodes for lithium-ion battery applications.A timely overview of the exciting progress of mofs as well as MOF-derived metallic components is *** unique char-acteristics of mofs,such as their large surface area,high tunable porosity with uniform pore size,unique structural and morphological features,controllable framework composition and low densities,combine together to provide good interfacial charge transport properties and short diffusion lengths for electrons and/or ions that adequately support electrochemical redox *** progress of mofs and their derived composites as cathode candidates for LIBs is emphasized based on their electrochemical results,while also discussing the remaining issues and potential upcoming research directions.

关键词： mofs and their derived derivatives Li-ion batteries Cathodes Lithium storage

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