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Pollution of hazardous substances in industrial construction and demolition wastes and their multi-path risk within an abandoned pesticide manufacturing plant

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Frontiers of Environmental Science & Engineering 2017年第1期11卷 123-135页

作者： Sheng Huang Xin Zhao Yanqiu Sun Jianli Ma Xiaofeng Gao Tian Xie Dongsheng XU Yi Yu Youcai Zhao The State Key Laboratory of Pollution Control and Resource Reuse Tongji University Shanghai 200092 China Shanghai Chengpei Enterprise Management Consulting Co. Ltd. Shanghai 200232 China Tianjin Academy of Environmental Sciences Tianjin 300191 China Debin Environmental Protection and Technology Holding Co. Ltd. Shanghai 200092 China Shanghai Design Institute in Environmental Sanitary Engineering Shanghai 200092 China

Exploration of heavy metals and organic pollutants, their leaching capacity along with health and environmental risks in contaminated industrial construction and demolition waste （ICDW） within a pesticide manufacturing plant were investigated. A maximum content of 90.8 mg·kg-1 Cd was found present in the wastes, which might originate from phosphorus rocks and industrial sulfuric acid used in pesticide production processes. An average concentration of 979.8 mg·kg-1 dichlorovos and other 11 organophosphorus pesticide were also detected. Relatively high leaching rates of around 4.14‰ were obtained from laboratory simulated ICDW using both glacial acetic acidsodium hydroxide and deionized water. Pesticide pollutants had the strongest tendency to retaining on dry bricks （leaching rate 1.68 9‰） compared to mortar-coatings, etc. due to their different physical characteristics and octanol-water partioning coefficient. Mobility of pesticide from on-site ICDW by water was spatially correlated to waste types, process sections and human activities, with a flux of leaching rate between 5.9‰ to 27.4%. Risk-based corrective action （RBCA） model was used to simulate the risk of contaminated ICDW debris randomly scattered. Oral and demlal ingestion amount by local workers was 9.8 × 10-3 and 1.9 × 10-2 mg.（kg-d）-1, respectively. Potential leaching risk to aquatic systems exceeded the limit for nearly 75% waste. Environmental and health risk exceedance was found in most ICDW, while the risk value of the most severely contaminated brick waste was 660 times beyond critical level. Implications for waste management involving construction and deconstruction work, waste transferring and regulation supplying were also provided.

关键词： Industrial demolition wastes Heavy metals Pesticides leaching characteristics Risk assessment Waste management

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