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Modeling and simulation of solvent behavior and temperature distribution within long stick propellants with large web thickness undergoing drying

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Defence Technology（防务技术） 2023年第10期28卷 42-55页

作者： Enfa Fu Qianling Liu Yu Luan Yao Zhu Weidong He Zhenggang Xiao Key Laboratory of Special Energy Materials Ministry of EducationSchool of Chemistry and Chemical EngineeringNanjing University of Science and TechnologyNanjing210094People's Republic of China

Drying is a complicated physical process which involves simultaneous heat and mass transfer in the removal of solvents inside *** drying techniques may result in the formation of a hard skin layer near the surface to block the free access of most solvent through for long stick propellants with large web thickness,which lead to lower drying efficiency and worse drying *** study aims to gain a comprehensive understanding of drying process and clarify the mechanism of the blocked layer near the propellant surface.A new three-dimensional coupled heat and mass transfer(3D-CHMT)model was successfully developed under transient *** drying experiment results show that the 3DCHMT model could be applied to describe the drying process well since the relative error of the content of solvent between simulation and experiment values is only 5.5%.The solvent behavior simulation demonstrates that the mass transfer process can be divided into super-fast(SF)and subsequent minorfast(MF)stages,and the SF stage is vital to the prevention of the blocked layer against the free access for solvent molecules inside propellant *** effective solvent diffusion coefficient(Deff)of the propellant surface initially increases from 3.4×10^(-6)to 5.3×10^(-6)m^(2)/s as the temperature increases,and then decreases to 4.1×10^(-8)m^(2)/s at 60-100 *** value of Deffof surface between 0-1.4 mm has a unique trend of change compared with other regions,and it is much lower than that of the internal at100 min under simulation ***,the temperature of the propellant surface increases rapidly at the SF stage(0-100 min)and then very slowly *** the evolution of Deffand temperature distribution demonstrate that the blocked layer near the propellant surface has been formed in the time period of approximately 0-100 min and its thickness is about 1.4 *** mitigate the formation of blocked layer and improve its drying quality of finial prop

关键词： Stick propellants Drying large web thickness 3D numerical modeling Heat transfer Solvent behavior

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