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Doping effect of SrZrO_(3) on knln ceramics structure and their dielectric properties

Journal of Advanced Dielectrics 2018年第5期8卷 28-34页

作者： Emad Ewais Ragab Mahani Samy Mostafa Adel Ahmedx Refractory and Ceramic Materials Division(RCMD)Central Metallurgical R&D Institute P.O.87 Helwan 11421 CairoEgypt Microwave Physics and Dielectrics Department National Research Centre 33 EL Bohouth st.(former EL Tahrirst.)P.O.12622 GizaEgypt Tabbin Institute for Metallurgical Studies(TIMS)P.O.109 Helwan 11421 CairoEgypt Chemistry Department Helwan University HelwanCairoEgypt

In this work,lead-free systems;(1-x)(K_(0.465)Na_(0.465)Li_(0.07))NbO_(3)–xSrZrO_(3)(x=0,0.005,0.050,0.095 and 0.14)were synthesized by the conventional solid-state reaction ***,SEM,densification parameter as well as dielectric parameters of the obtained knln ceramics were *** analysis showed the formation of orthorhombic perovskite structure in all investigated ***_(3)(SZ)inhibited the grain growth and increased the distribution of grains uniformly in the micro*** addition,SZ changed the crystalline system of knln ceramics *** a consequence,the permittivity,dielectric loss as well as AC conductivity decreased *** ceramics of x=0.005 are characterized by low conductivity(10-10 S/cm),low dielectric loss(0.005)and relatively high permittivity(34).They can be useful for the electrical capacitors fabrication and filtering out noise from signals in resonant *** frequencies lower than 105 Hz,DC conductivity and separation of the charges at the interfaces were found to dominate the electrical behavior of ceramics,whereas at higher frequencies,a faster or dipole polarization may become more dominated.A broad peak has been observed in the imaginary part of electric modulus revealing to the non-Debye dielectric relaxation *** mechanical tunneling(QMT)was found to be the most suitable to characterize the electrical conduction mechanism in the ceramic compounds.

关键词： Lead-free ceramics knln dielectric properties.

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