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Polar organic tracers in PM_(2.5) aerosols from an inland background area in Southwest China: Correlations between secondary organic aerosol tracers and source apportionment

引用

Journal of Environmental Sciences 2018年第7期30卷 281-293页

作者： Li Li Wei Lai Jinguo Pu Hengqin Mo Dongjue Dai Guilin Wu Shihuai Deng Rural Environment Protection Engineering & Technology Center of Sichuan Province College of Environment Sichuan Agricultural University School of Environment Tsinghua University

PM2.5 aerosol samples were collected over 12 hr and 24 hr intervals in an inland background area, Gongga Mountain National Nature Reserve（hereafter shortened to Gongga）, during the summer of 2011. Polar organic tracers, inorganic ions and meteorological data were measured. The purpose of this work was to investigate the variation patterns, formation and sources of the secondary organic aerosol tracers in the studied atmosphere. The average concentrations of isoprene oxidation products, α-pinene oxidation products, β-caryophyllinic acid, sugars, sugar alcohols and anhydrosugars were 88.6 ± 106.1, 3.6 ± 5.7,0.13 ± 0.30, 13.6 ± 13.1, 31.9 ± 31.4 and 14.8 ± 10.7 ng/m^3 respectively in all aerosol *** aged α-pinene second organic aerosol（SOA） tracers（i.e., 3-hydroxyglutraric acid（3 HGA）, 3-hydroxy-2,2-dimethylglutaric acid（HDMGA）, 3-acetylpentandioic acid（APDA） and 3-methyl-1,2,3-butanetricarboxylic acid（MBTCA）） correlated significantly with each other in the 24 hr PM2.5 aerosol samples, indicating that OH· is the major factor controlling the formation of these α-pinene SOA tracers. Using the positive matrix factorization（PMF） model and the tracer-based source apportionment method, we calculated that isoprene oxidation products, α-pinene oxidation products, sesquiterpene oxidation products, biomass burning, fungi spores and anthropogenic SOA accounted for 21.9% ± 5.5%, 8.4% ± 2.1%, 3.0% ± 0.7%, 5.2% ± 5.3%, 5.0% ± 6.2% and 31.4% ± 7.8% of organic carbon respectively during the sampling period.

关键词： isoprene oxidation products α-Pinene oxidation products β-Caryophyllinic acid Positive matrix factorization(PMF) Gongga Mountain National Nature Reserve

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