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Observation of Mott instability at the valence transition of f-electron system

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National Science Review 2023年第6期10卷 183-190页

作者： Haifeng Yang Jingjing Gao Yingying Cao Yuanji Xu Aiji Liang Xiang Xu Yujie Chen Shuai Liu Kui Huang Lixuan Xu Chengwei Wang Shengtao Cui Meixiao Wang Lexian Yang Xuan Luo Yuping Sun Yi-feng Yang Zhongkai Liu Yulin Chen School of Physical Science and Technology Shanghai Tech University Key Laboratory of Materials Physics Institute of Solid State Physics Chinese Academy of Sciences Science Island Branch of Graduate School University of Science and Technology of China Beijing National Laboratory for Condensed Matter Physics and Institute of Physics Chinese Academy of Sciences University of Chinese Academy of Sciences Shanghai Tech Laboratory for Topological Physics State Key Laboratory of Low Dimensional Quantum Physics and Department of Physics Tsinghua University State Key Laboratory of Functional Materials for Informatics Shanghai Institute of Microsystem and Information Technology (SIMIT) Chinese Academy of Sciences High Magnetic Field Laboratory Chinese Academy of Sciences Collaborative Innovation Center of Microstructures Nanjing University Songshan Lake Materials Laboratory Department of Physics University of Oxford

Mott physics plays a critical role in materials with strong ele ctronic *** insulator-to-metal transition can be driven by chemical doping,external pressure,temperature and gate voltage,which is often seen in transition metal oxides with 3d electrons near the Fermi energy(*** superconductor).In4f-electron systems,however,the insulator-to-metal transition is mostly driven by Kondo hybridization and the Mott physics has rarely been explored in ***,by combining the angle-resolved photo emission spectroscopy and strongly correlated band structure calculations,we show that an unusual Mott instability exists in YbInCu4accompanying its mysterious first-order valence *** contrasts with the prevalent Kondo picture and demonstrates that YbInCu4is a unique platform to explore the Mott physics in Kondo lattice *** work provides important insight for the understanding and manipulation of correlated quantum phenomena in the f-electron system.

关键词： valence transition orbital-selectiveMott transition Kondo coupling heavy fermions strong correlations ARPES DMFT

Scaling behavior of the thermopower of the archetypal heavy-fermion metal YbRh2Si2

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Frontiers of physics 2016年第2期11卷 89-95页

作者： V. R. Shaginyan A. Z. Msezane G. S. Japaridze K. G. Popov J. W. Clark V. A. Khodel Petersburg Nuclear Physics Institute NRC Kurchatov Institute Gatchina 188300 Russia Clark Atlanta University Atlanta GA 30314 USA Komi Science Center Ural Division RAS Syktyvkar 167982 Russia Department of Physics St. Petersburg State University Russia McDonnell Center for the Space Sciences 8J Department of Physics Washington University St. Louis MO 63130 USA Centro de Ciencias Matemdticas Universidade de Madeira 9000-390 Funchal Madeira Portugal Russian Research Center Kurchatov Institute Moscow 123182 Russia

We reveal and explain the scaling behavior of the thermopower S/T exhibited by the archetypal heavy-fermion （HF） metal YbRh2Si2 under the application of magnetic field B at temperature T. We show that the same scaling is demonstrated by different HF compounds such as/3-YbA1B4 and the strongly correlated layered cobalt oxide [BiBa0.66K0.3602]CoO2. Using YbRh2Si2 as an example, we demonstrate that the scaling behavior of SIT is violated at the antiferromagnetic phase transition, while both the residual resistivity Po and the density of states, N, experience jumps at the phase transition, causing the thermopower to make two jumps and change its sign. Our elucidation is based on flattening of the single-particle spectrum that profoundly affects Po and N. To depict the main features of the SIT behavior, we construct a T-B schematic phase diagram of YbRh2Si2. Our calculated SIT for the HF compounds are in good agreement with experimental facts and support our observations.

关键词： thermoelectric and thermomagnetic effects quantum phase transition flat bands,non-Fermi-liquid states strongly correlated electron systems heavy fermions

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Frontiers of physics 2016年第5期11卷 57-78页

作者： V. R. Shaginyan A. Z. Msezane G. S. Japaridze K. G. Popov V. A. Khodel Petersburg Nuclear Physics Institute NRC Kurchatov Institute Gatchina 188300 Russia Clark Atlanta University Atlanta GA 30314 USA Komi Science Center Ural Division RAS Syktyvkar 167982 Russia Russian Research Centre Kurchatov Institute Moscow 123182 Russia McDonnell Center for the Space Sciences & Department of Physics Washington University St. Louisa MO 63130 USA

The aim of this review paper is to expose a new state of matter exhibited by strongly correlated Fermi systems represented by various heavy-fermion （HF） metals, two-dimensional liquids like 3He, compounds with quantum spin liquids, quasicrystals, and systems with one-dimensional quantum spin liquid. We name these various systems HF compounds, since they exhibit the behavior typical of HF metals. In HF compounds at zero temperature the unique phase transition, dubbed throughout as the fermion condensation quantum phase transition （FCQPT） can occur; this FCQPT creates flat bands which in turn lead to the specific state, known as the fermion condensate. Unlimited increase of the effective mass of quasiparticles signifies FCQPT; these quasiparticles determine the thermodynamic, transport and relaxation properties of HF compounds. Our discussion of numerous salient experimen- tal data within the framework of FCQPT resolves the mystery of the new state of matter. Thus, FCQPT and the fermion condensation can be considered as the universal reason for the non-Fermi liquid behavior observed in various HF compounds. We show analytically and using arguments based completely on the experimental grounds that these systems exhibit universal scaling behavior of their thermodynamic, transport and relaxation properties. Therefore, the quantum physics of different HF compounds is universal, and emerges regardless of the microscopic structure of the compounds. This uniform behavior allows us to view it as the main characteristic of a new state of matter exhibited by HF compounds.

关键词： quantum phase transition flat bands systems quantum spin liquids heavy fermions effects scaling behavior new state of matter non-Fermi-liquid states strongly correlated electron quasicrystals thermoelectric and thermomagnetic

Localized 4f-electrons in the quantum critical heavy fermion ferromagnet CeRh_(6)Ge_(4)

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Science Bulletin 2021年第14期66卷 1389-1394,M0003页

作者： An Wang Feng Du Yongjun Zhang David Graf Bin Shen Ye Chen Yang Liu Michael Smidman Chao Cao Frank Steglich Huiqiu Yuan Center for Correlated Matter and Department of Physics Zhejiang UniversityHangzhou 310058China Institute for Advanced Materials Hubei Normal UniversityHuangshi 435002China National High Magnetic Field Laboratory and Department of Physics Florida State UniversityTallahasseeFL 32306USA Zhejiang Province Key Laboratory of Quantum Technology and Device Department of PhysicsZhejiang UniversityHangzhou 310058China Department of Physics Hangzhou Normal UniversityHangzhou 310036China Max Planck Institute for Chemical Physics of Solids Dresden 01187Germany State Key Laboratory of Silicon Materials Zhejiang UniversityHangzhou 310058China

Ferromagnetic quantum critical points were predicted to be prohibited in clean itinerant ferromagnetic systems,yet such a phenomenon was recently revealed in CeRh_(6)Ge_(4),where the Curie temperature can be continuously suppressed to zero under a moderate hydrostatic *** we report the observation of quantum oscillations in CeRh_(6)Ge_(4)from measurements using the cantilever and tunnel-diode oscillator methods in fields up to 45 T,clearly demonstrating that the ferromagnetic quantum criticality occurs in a clean *** order to map the Fermi surface of CeRh_(6)Ge_(4),we performed angle-dependent measurements of quantum oscillations at ambient pressure,and compared the results to density functional theory *** results are consistent with the Ce 4f electrons remaining localized and not contributing to the Fermi surface,suggesting that localized ferromagnetism is a key factor for the occurrence of a ferromagnetic quantum critical point in CeRh_(6)Ge_(4).

关键词： heavy fermions Ferromagnetism Quantum phase transitions Electronic structure