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Rational design of carbon skeleton interfaces for highly reversible sodium metal battery anodes

Journal of Energy Chemistry 2024年第5期92卷 404-413页

作者： Fenqiang Luo Taiyu Lyu Jie Liu Peiwan Guo Junkai Chen Xiaoshan Feng Dechao Wang Zhifeng Zheng Key Laboratory of Advanced Energy Storage Technology Fujian Province UniversityFujian Provincial Industry Technologies Development Base for New EnergyCollaborative Innovation Platform for Advanced Electrochemical Energy Storage TechnologyNational User-Side Energy Storage Innovation Research and Development CenterTan Kah Kee Innovation Laboratory(IKKEM)College of EnergyXiamen UniversityXiamen 361102FujianChina College of Environmental Science and Engineering Fujian Normal UniversityFuzhou 350007FujianChina Department of Chemical Engineering Tsinghua UniversityBeijing 100084China

Sodium metal batteries(SMBs)have attracted increasing attention over time due to their abundance of sodium resources and low ***,the widespread application of SMBs as a viable technology remains a great challenge,such as uneven metallic deposition and dendrite formation during *** skeletons as sodiophilic hosts can alleviate the dendrite formation during the plating/*** the carbon skeleton,how to rationalize the design sodiophilic interfaces between the sodium metal and carbon species remains key to developing desirable Na ***,we fabricated four kinds of structural features for carbon skeletons using conventional calcination and flash Joule *** roles of conductivity,defects,oxygen content,and the distribution of graphite for the deposition of metallic sodium were discussed in *** on interface engineering,the J1600 electrode,which has abundant Na-C species on its surface,showed the highest *** are uniform and rich F-Na species distributed in the inner solid electrolyte interface *** study investigated the different Na-deposition behavior in carbon hosts with distinct graphitic arrangements to pave the way for designing and optimizing advanced electrode materials.

关键词： Carbon skeleton graphited structure Deposition mechanism Sodiummetal batteries

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