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Defence Technology（防务技术） 2023年第4期22卷 69-73页

作者： Bhargav Appasani Avireni Srinivasulu Cristian Ravariu Department of Electronics Engineering Kalinga Institute of Industrial TechnologyBhubaneswarIndia Department of Electronics Engineering K R Mangalam UniversityGurgaonIndia Department of Electronic Devices Circuits and ArchitecturesPolytechnic University of BucharestBucharestRomania

A nearly perfect metamaterial absorber is proposed that can find utility in terahertz sensing *** design consists of two concentric elliptical ring resonators(ERRs)whose parameters are appropriately set to achieve dual band absorption with near perfect *** first absorption band at 3.62 THz having a Q-factor of 51.7 was caused due to the currents in the outer and inner *** second absorption peak at 3.814 THz having a Q factor of 1411.11 was a consequence of currents flowing across the gap between the two concentric ***,it is observed that the absorption bands are sensitive to the variation in refractive index of the surrounding *** sensitivity's in the absorption bands are 3 THz/RIU and 3.59 THz/RIU respectively.A sensor is proposed based on this design to detect harmful gases,which is demonstrated for detection of Methane and *** Q-factor and high sensitivity of the narrow band makes the design an excellent sensor for detecting variations in the refractive index.

关键词： Refractive index Plasma frequency Metamaterials Terahertz absorption Q-factor gas sensing

Room temperature NO_2 gas sensing of Au-loaded tungsten oxide nanowires/porous silicon hybrid structure

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Chinese Physics B 2016年第2期25卷 504-509页

作者：王登峰梁继然李昌青闫文君胡明 School of Electronics and Information Engineering Tianjin University

In this work, we report an enhanced nitrogen dioxide（NO_2） gas sensor based on tungsten oxide（WO_3）nanowires/porous silicon（PS） decorated with gold（Au） nanoparticles. Au-loaded WO_3 nanowires with diameters of 10 nm–25 nm and lengths of 300 nm–500 nm are fabricated by the sputtering method on a porous silicon substrate. The high-resolution transmission electron microscopy（HRTEM） micrographs show that Au nanoparticles are uniformly distributed on the surfaces of WO_3 nanowires. The effect of the Au nanoparticles on the NO_2-sensing performance of WO_3 nanowires/porous silicon is investigated over a low concentration range of 0.2 ppm–5 ppm of NO_2 at room temperature（25℃）. It is found that the 10-？ Au-loaded WO_3 nanowires/porous silicon-based sensor possesses the highest gas response characteristic. The underlying mechanism of the enhanced sensing properties of the Au-loaded WO_3 nanowires/porous silicon is also discussed.

关键词： Au-loaded WO3 nanowires hybrid structure gas sensing

Unlocking Co3O4–ZnO p-n heterojunction for superior acetone gas sensing detection

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Progress in Natural Science:Materials International 2024年第5期34卷 990-999页

作者： Xingxing Liu Tingting Shao Juntang Dong Huirong Kou Fuchun Zhang Yuyang Cheng Jiaming Guo Shuwei Tian Kuldeep K.Saxena Xinghui Liu School of Physics and Electronic Information Yan'an University Division of Research and Development Lovely Professional University Science and Technology on Aerospace Chemical Power Laboratory Laboratory of Emergency Safety and Rescue Technology Hubei Institute of Aerospace Chemotechnology Department of Materials Physics Saveetha School of Engineering Saveetha Institute of Medical and Technical Sciences (SIMTS)

In this study, we synthesized pure ZnO and Co3O4–ZnO precursors with varied Co, Zn ratios via solvothermal method, and then the precursors were calcined at 400°C for 2 h in a muffle furnace under air to obtain composites for acetone detection. The structure, morphology, elemental composition, microstructure and chemical state of these materials were systematically studied by various characterization techniques. Additionally, we also evaluated the gas sensing performance of the composites-based sensors, focusing on optimal operating temperature,baseline resistance, repeatability, stability, selectivity, response/recovery time, and resistance under varying relative humidity. The findings reveal that 3 % Co3O4–ZnO-based sensor exhibit the highest response value to 100 ppm acetone（74）, showing an enhancement of approximately 9.3 times compared to the pure ZnO-based sensor（8）. Furthermore, the 3 % Co3O4–ZnO-based sensor demonstrate the advantages of rapid response/recovery times（15 s/2 s）, outstanding selectivity, and remarkable stability. The gas sensing mechanism of the composite material is also discussed in detail, which provides insights into the observed enhancement of gas sensing performance. It provides an idea for the follow-up study on gas sensing performance of acetone sensors.

关键词： Acetone Co3O4–ZnO gas sensing Heterojunction Solvothermal method

Preparation of single atom catalysts for high sensitive gas sensing

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International Journal of Extreme Manufacturing 2024年第3期6卷 216-248页

作者： Xinxin He Ping Guo Xuyang An Yuyang Li Jiatai Chen Xingyu Zhang Lifeng Wang Mingjin Dai Chaoliang Tan Jia Zhang Key Laboratory of Microsystems and Microstructure Manufacturing Ministry of EducationHarbin Institute of TechnologyHarbin 150080People’s Republic of China Institute for Frontier Materials Deakin UniversityWaurn Ponds CampusLocked Bag 20000Victoria 3220Australia School of Electrical and Electronic Engineering Nanyang Technological UniversitySingapore 639798Singapore Department of Electrical and Electronic Engineering The University of Hong KongPokfulam RoadHong Kong Special Administrative Region of China 999077People’s Republic of China Chongqing Research Institute Harbin Institute of TechnologyChongqing 401120People’s Republic of China

Single atom catalysts(SACs)have garnered significant attention in the field of catalysis over the past decade due to their exceptional atom utilization efficiency and distinct physical and chemical *** the semiconductor-based electrical gas sensor,the core is the catalysis process of target gas molecules on the sensitive *** this context,the SACs offer great potential for highly sensitive and selective gas sensing,however,only some of the bubbles come to the *** facilitate practical applications,we present a comprehensive review of the preparation strategies for SACs,with a focus on overcoming the challenges of aggregation and low *** research efforts have been devoted to investigating the gas sensing mechanism,exploring sensitive materials,optimizing device structures,and refining signal post-processing ***,the challenges and future perspectives on the SACs based gas sensing are presented.

关键词： single atom catalysts preparation sensing mechanism gas sensing

Synthesis and room-temperature NO_2 gas sensing properties of a WO_3 nanowires/porous silicon hybrid structure

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Chinese Physics B 2014年第5期23卷 600-606页

作者：曾鹏张平胡明马双云闫文君 School of Electronics and Information Engineering Tianjin University

We report on the fabrication and performance of a room-temperature NO2 gas sensor based on a WO3 nanowires/porous silicon hybrid structure. The W18O49 nanowires are synthesized directly from a sputtered tungsten film on a porous silicon （PS） layer under heating in an argon atmosphere. After a carefully controlled annealing treatment, WO3 nanowires are obtained on the PS layer without losing the morphology. The morphology, phase structure, and crystallinity of the nanowires are investigated by using field emission scanning electron microscopy （FESEM）, X-ray diffractometer （XRD）, and high-resolution transmission electron microscopy （HRTEM）. Comparative gas sensing results indicate that the sensor based on the WO3 nanowires exhibits a much higher sensitivity than that based on the PS and pure WO3 nanowires in detecting NO2 gas at room temperature. The mechanism of the WO3 nanowires/PS hybrid structure in the NO2 sensing is explained in detail.

关键词： gas sensing WO3 nanowires porous silicon hybrid structure

Orientation controlled preparation of nanoporous carbon nitride fibers and related composite for gas sensing under ambient conditions

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Nano Research 2017年第5期10卷 1710-1719页

作者： Suqin Li Zhiwei Wang Xiaoshan Wang Fangfang Sun Kai Gao Ningxian Hao Zhipeng Zhang Zhongyuan Ma Hai Li Xiao Huang Wei Huang Key Laboratory of Flexible Electronics (KLOFE) & Institute of Advanced Materials (IAM) Jiangsu National Synergistic Innovation Centerfor Advanced Materials (SICAM) Nanjing Tech University 30 South Puzhu Road Nanjing 211816 China

Creating pores in suprastructures of two-dimensional （2D） materials while controlling the orientation of the 2D building blocks is important in achieving large specific surface areas and tuning the anisotropic properties of the obtained functional hierarchical structures. In this contribution, we report that arranging graphitic carbon nitride （g-C3N4） nanosheets into one-dimensional （1D） architectures with controlled orientation has been achieved by using 1D oriented melem hydrate fibers as the synthetic precursor via a polycondensation process, during which the removal of water molecules and release of ammonia gas led to the creation of pores without destroying the 1D morphology of the oriented structures. The resulting porous g-C3N4 fibers with both meso- and micro-sized pores and largely exposed edges exhibited good sensing sensitivity and selectivity towards NO2. The sensing performance was further improved by hybridization of the porous fibers with Au nanoparticles （Au NPs）, leading to a detection limit of 60 ppb under ambient conditions. Our results suggest that the highly porous g-C3N4 fibers and the related hybrid structures with largely exposed graphitic layer edges are excellent sensing platforms and may also show promise in other electronic and electrochemical applications.

关键词： graphitic carbon nitride Au nanoparticle gas sensing porous fiber chemiresistive sensor

Asymmetric side-chain engineering of organic semiconductor for ultrasensitive gas sensing

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Chinese Chemical Letters 2024年第3期35卷 428-433页

作者： Xiaoying Ma Xiaojuan Dai Lanyi Xiang Jiajun Chang Danfeng Zhi Haozhen Zhao Zhenjie Ni Ye Zou Xike Gao Fengjiao Zhang School of Chemical Sciences University of Chinese Academy of SciencesBeijing 100049China Laboratory of Organic Solids Institute of ChemistryChinese Academy of SciencesBeijing 100190China Key Laboratory of Synthetic and Self-Assembly Chemistry for Organic Functional Molecules Shanghai Institute of Organic ChemistryChinese Academy of SciencesShanghai 200032China Binzhou Institute of Technology Binzhou 256606China

Molecular structure of organic semiconductor plays a critical role in determining the performance and functionality of organic electronic devices,by optimizing the electrical,optical and physicochemical *** alkyl chains are fundamental units in tailering the solubility and assemblability,among which the asymmetric properties have been reported as key element for controlling the packing motifs and intrinsic charge ***,we expanded the scope of molecular asymmetry dependent sensing features based on a new series of naphthalene diimides(NDI)-based derivatives substituted with a same branching alkyl chain but various linear-shaped alkyl chains(Cn-).A clear molecular stacking change,from head-to-head bilayer to head-to-tail monolayer packing model,is observed based on the features of anisotropic molecular interactions with the change in the chain *** importantly,a unique LUMO level shift of 0.17 eV is validated for NDI-PhC4,providing a record sensitivity up to 150%to 0.01 ppb ammonia,due to the desired molecular reactivity and device amplification *** results indicate that asymmetric side-chain engineering opens a route for breath healthcare.

关键词： Organic thin film transistor Asymmetric side chain gas sensing Molecular stacking Energy level manipulating

The preparation of grid-textured V2O5 films and their potential applications in gas sensing

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Science China(Technological Sciences) 2020年第3期63卷 467-471页

作者： CHENG Rong HUANG WeiYi LIU XiangBo LING Francis Chi Chung GAO Ju NI Hao Department of Mechanical Engineering Tsinghua UniversityBeijing 100084China Department of Physics The University of Hong KongHong KongChina College of Science China University of Petroleum(Huadong)Qingdao 266580China

Novel nano-structured films of V2O5 are prepared by pulsed laser deposition method. Nanoscaled V2O5 ridges lie on SrTiO3 substrate and construct into grid-textured structures. Structural properties of the films have been analyzed by scanning electron microscope, X-ray diffraction and transmission electron microscope. The films have enlarged surface-to-volume ratio due to the ridge-channel structure which makes them applicable to gas sensing. Therefore, gas sensors based on the V2O5 films have been assembled which present reliable sensing properties to gaseous acetone, and ethanol at room temperature. The physical-chemical reactions between adsorbed O2^– and testing gases are the possible reason for this property.

关键词： V2O5 thin film gas sensing

Nanogenerators for Self-Powered gas sensing

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Nano-Micro Letters 2017年第4期9卷 81-99页

作者： Zhen Wen Qingqing Shen Xuhui Sun Institute of Functional Nano and Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devicesand Collaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215123People’s Republic of China

Looking toward world technology trends over the next few decades, self-powered sensing networks are a key field of technological and economic driver for global industries. Since 2006, Zhong Lin Wang's group has proposed a novel concept of nanogenerators(NGs), including piezoelectric nanogenerator and triboelectric nanogenerator, which could convert a mechanical trigger into an electric output. Considering motion ubiquitously exists in the surrounding environment and for any most common materials used every day, NGs could be inherently served as an energy source for our daily increasing requirements or as one of self-powered environmental sensors. In this regard, by coupling the piezoelectric or triboelectric properties with semiconducting gas sensing characterization, a new research field of self-powered gas sensing has been proposed. Recent works have shown promising concept to realize NG-based self-powered gas sensors that are capable of detecting gas environment without the need of external power sources to activate the gas sensors or to actively generate a readout signal. Compared with conventional sensors, these self-powered gas sensors keep the approximate ***, these sensors drastically reduce power consumption and additionally reduce the required space for integration,which are significantly suitable for the wearable devices. This paper gives a brief summary about the establishment and latest progress in the fundamental principle, updated progress and potential applications of NG-based self-powered gas sensing system. The development trend in this field is envisaged, and the basic configurations are also introduced.

关键词： Nanogenerator Self-powered gas sensing Piezoelectric Triboelectric

The gas sensing properties of TiO_2 nanotubes synthesized by hydrothermal method

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Chinese Chemical Letters 2011年第5期22卷 603-606页

作者： Yan Li Wang Shun Tan Jia Wang Zhi Jin Tan Qiu Xia Wu Zheng Jiao Ming Hong Wu Institute of Nanochemistry and Nanobiology School of Environmental and Chemical Engineering Shanghai University Shanghai 200444 China

In this paper,the TiO_2 nanotubes were synthesized by hydrothermal method using a 10 mol/L NaOH aqueous solution at 150℃. The structure of prepared materials was characterized by X-ray diffraction（XRD）,transmission electron microscopy（TEM）. scanning electron microscope（SEM） and Brunauer-Emmett-Teller（BET）.The prepared TiO_2 nanotubes were used to prepare thick film gas sensors and the gas sensing properties to various gases were *** show the prepared TiO_2 nanotube gas sensors responses to ethanol under dry condition at 450℃.This could be attributed to the fact that it had high porous morphology and a higher pore volume,which can promote the diffusion of ethanol deep inside the films and improve the sensor response. Moreover,the gas sensor made with nanotubes exhibit high selective response towards ethanol gas compared with H_2,CO,acetone.

关键词： TiO_2 nanotubes Hydrothermal method gas sensing