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稀有金属材料与工程 2006年第A3期35卷 65-66页

作者： Jae-Hyun Cho Joon-Boo Yu Sung-Ok Sohn Duk-Dong Lee Jeung-Soo Huh Department of Material Science Metallurgy Kyungpook National UniversitySangyuk-Dong 1370DaeguKorea School of Electronic Engineering Kyungpook National UniversitySangyuk-Dong 1370DaeguKorea

Polypyrrole (PPy) powder was synthesized by chemical polymerization at 0℃under atmospheric condition and its layer was prepared by dip coating method on the alumina substrate with interdigitated *** influence of relative humidity (RH 0～70%) to PPy sensor was *** measuring temperature was fixed at 25℃.Methanol and benzene were used as target *** analytic techniques were examined to observe changes in the properties of PPy *** sensitivity of PPy sensor to water vapor was linearly increased with the increasing *** the relative humidity increase from 0% to 70%,the sensitivities to methanol and benzene vapor were reduced,and reduction ratio of sensitivity was 94%, 92.5% at RH 70%,respectively.

关键词： VOCs polypyrrole humidity effect gas sensor

A Composite of Electrospun Nylon-6 Nanofibers and in-situ Polymerized Polypyrrole as an NH3 gas sensor

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复旦学报（自然科学版） 2007年第5期46卷 797-页

作者： Ji Shanzuo, Li Yang, Yang Mujie(Department of Polymer Science and Engineering, Zhejiang University, Hangzhou 310027, China) Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027

1 Results Electrospinning provides a simple and versatile method for preparing nanofibers with different morphology, such as porous fibers and nanotubes. It has been widely used for preparing nanomaterials with unique properties and potential applications in medicine, catalyst, photonics and sensors[1, 2]. In this study, uniform Nylon-6 nanofibers with diameter of ≈300 nm by electrospun from formic acid solution containing 15%wt Nylon-6. Polypyrrole (PPy) was then deposited on the nanofibers by in-situ ...

关键词： electrospining polypyrrole nylon-6 nanofibers gas sensor composite

MXene Key Composites:A New Arena for gas sensors

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Nano-Micro Letters 2024年第10期16卷 350-391页

作者： Yitong Wang Yuhua Wang Min Jian Qinting Jiang Xifei Li Hubei Province Key Laboratory of Systems Science in Metallurgical Process Wuhan University of Science and TechnologyWuhan 430081People's Republic of China Key Materials and Components of Electrical Vehicles for Overseas Expertise Introduction Center for Discipline Innovation Institute of Advanced Electrochemical Energy and School of Materials Science and EngineeringXi'an University of TechnologyXi'an 710048People's Republic of China College of Materials Science and Engineering Fuzhou UniversityFuzhou 350108FujianPeople's Republic of China

With the development of science and technology,the scale of industrial production continues to grow,and the types and quantities of gas raw materials used in industrial production and produced during the production process are also constantly *** gases include flammable and explosive gases,and even contain toxic ***,it is very important and necessary for gas sensors to detect and monitor these gases quickly and *** recent years,a new two-dimensional material called MXene has attracted widespread attention in various *** abundant surface functional groups and sites,excellent current conductivity,tunable surface chemistry,and outstanding stability make them promising for gas sensor *** the birth of MXene materials,researchers have utilized the efficient and convenient solution etching preparation,high flexibility,and easily functionalize MXene with other materials to pre-pare composites for gas *** has opened a new chapter in high-performance gas sensing materials and provided a new approach for advanced sensor ***,previous reviews on MXene-based composite materials in gas sensing only focused on the performance of gas sensing,without systematically explaining the gas sensing mechanisms generated by different gases,as well as summarizing and predicting the advantages and disadvantages of MXene-based composite *** article reviews the latest progress in the application of MXene-based composite materials in gas ***,a brief summary was given of the commonly used methods for preparing gas sens-ing device structures,followed by an introduction to the key attributes of MXene related to gas sensing *** article focuses on the performance of MXene-based composite materials used for gas sensing,such as MXene/graphene,MXene/Metal oxide,MXene/Transition metal sulfides(TMDs),MXene/Metal-organic framework(MOF),MXene/*** summarizes the advantages and disad

关键词： MXene Compound material gas sensor gas sensitive preparation gas sensitivity performance

Highly Sensitive Ammonia gas sensors at Room Temperature Based on the Catalytic Mechanism of N,C Coordinated Ni Single-Atom Active Center

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Nano-Micro Letters 2024年第12期16卷 515-531页

作者： Wenjing Quan Jia Shi Min Zeng Wen Lv Xiyu Chen Chao Fan Yongwei Zhang Zhou Liu Xiaolu Huang Jianhua Yang Nantao Hu Tao Wang Zhi Yang National Key Laboratory of Advanced Micro and Nano Manufacture Technology Shanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Department of Micro/Nano Electronics School of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China Shanghai Key Laboratory of Intelligent Sensing and Detection Technology School of Mechanical and Power EngineeringEast China University of Science and TechnologyShanghai 200237People’s Republic of China

Significant challenges are posed by the limitations of gas sensing mechanisms for trace-level detection of ammonia(NH3).In this study,we propose to exploit single-atom catalytic activation and targeted adsorption properties to achieve highly sensitive and selective NH3 gas ***,Ni singleatom active sites based on N,C coordination(Ni-N-C)were interfacially confined on the surface of two-dimensional(2D)MXene nanosheets(Ni-N-C/Ti_(3)C_(2)Tx),and a fully flexible gas sensor(MNPE-Ni-N-C/Ti_(3)C_(2)Tx)was *** sensor demonstrates a remarkable response value to 5 ppm NH3(27.3%),excellent selectivity for NH3,and a low theoretical detection limit of 12.1 *** analysis by density functional calculation reveals that the Ni single-atom center with N,C coordination exhibits specific targeted adsorption properties for ***,its catalytic activation effect effectively reduces the Gibbs free energy of the sensing elemental reaction,while its electronic structure promotes the spill-over effect of reactive oxygen species at the gas-solid *** sensor has a dual-channel sensing mechanism of both chemical and electronic sensitization,which facilitates efficient electron transfer to the 2D MXene conductive network,resulting in the formation of the NH3 gas molecule sensing ***,the passivation of MXene edge defects by a conjugated hydrogen bond network enhances the long-term stability of MXene-based electrodes under high humidity *** work achieves highly sensitive room-temperature NH3 gas detection based on the catalytic mechanism of Ni single-atom active center with N,C coordination,which provides a novel gas sensing mechanism for room-temperature trace gas detection research.

关键词： gas sensor Single atom Catalytic activation Targeted adsorption End-sealing passivation

Sensing properties and mechanisms of LaF_(3)-Co_(3)O_(4) nanorods for low-concentration methanol detection

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Rare Metals 2024年第5期43卷 2193-2204页

作者： Xiao-Xi He Hong-Feng Chai Yi-Wen Zhou Ke-Wei Liu Ze-Xin Yu Chao Zhang College of Mechanical Engineering Yangzhou UniversityYangzhou225127China Institutefor Manufacturing Technologies of Ceramic Components and Composites(IMTCCC) University of Stuttgart70569 StuttgartGermany

Methanol is one of the characteristic gases that distinguish between healthy individuals and lung cancer(LC)lesions in exhaled human *** concentration in exhaled breath is generally below one part per million(1×10^(-6)).The second-phase composite is widely regarded as one of the methods to improve the gas-sensing perfor-mance of metal oxide semiconductor(MOS)*** this study,LaF_(3)-Co_(3)O_(4) was synthesized by a simple hydrothermal method to enhance its low-concentration methanol gas-sensing performance.5 at%LaF_(3)-Co_(3)O_(4) nanorods exhibited excellent methanol detection performance,including a wider linear detection concentration range(0.2×10^(-6)~5×10^(-6)),a response value exceeding 4.0 for 1×10^(-6)methanol at 275°C and 75%relative humidity(RH),long-term stability(maximum deviation within 15%over 2 weeks),and excellent *** mechanism of performance enhancement was studied using various techniques,and density functional *** special spinel structure of Co_(3)O_(4),the high ionic migration of F-in LaF_(3),the larger specific surface area of 5 at%LaF_(3)-Co_(3)O_(4) nanorods,and the generated crystal defects all explain the excellentmethanol gas-sensing *** work provides a novel route to prepare MOS composite materials for low-concentration methanol gas detection.

关键词： gas sensor LaF_(3) Co_(3)O_(4) Methanol Lung cancer

Laser‑Induced and MOF‑Derived Metal Oxide/Carbon Composite for Synergistically Improved Ethanol Sensing at Room temperature

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Nano-Micro Letters 2024年第6期16卷 210-220页

作者： Hyeongtae Lim Hyeokjin Kwon Hongki Kang Jae Eun Jang Hyuk‑Jun Kwon Department of Electrical Engineering and Computer Science DGISTDaegu 42988South Korea Convergence Research Advanced Centre for Olfaction DGISTDaegu 42988South Korea

Advancements in sensor technology have significantly enhanced atmospheric ***,metal oxide and carbon(MO_(x)/C)hybrids have gained attention for their exceptional sensitivity and room-temperature sensing ***,previous methods of synthesizing MO_(x)/C composites suffer from problems,including inhomogeneity,aggregation,and challenges in ***,we introduce a refined method that employs a metal–organic framework(MOF)as a precursor combined with direct laser *** inherent structure of MOFs ensures a uniform distribution of metal ions and organic linkers,yielding homogeneous MO_(x)/C *** laser processing facilitates precise micropatterning(sensor rapidly detected ethanol gas even at room temperature(105 and 18 s for response and recovery,respectively),with a broad range of sensing performance from 170 to 3,400 ppm and a high response value of up to 3,500%.Additionally,this sensor exhibited enhanced stability and thermal resilience compared to previous MOF-based *** research opens up promising avenues for practical applications in MOF-derived sensing devices.

关键词： Metal-organic frameworks Metal oxide Carbon composite Laser gas sensor

Well-designed g-C_(3)N_(4)nanosheet incorporated Ag loaded Er_(0.05)La_(0.95)FeO_(3)heterojunctions for isoamyl alcohol detection

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Journal of Advanced Ceramics 2024年第6期13卷 736-745页

作者： Kaichun Xu Mengjie Han Zichen Zheng Zexin Yu Hanlin Liao Hui Sun Chao Zhang College of Mechanical Engineering Yangzhou UniversityYangzhou 225127China Institute for Manufacturing Technologies of Ceramic Components and Composites(IMTCCC) University of StuttgartStuttgart 70569Germany ICB UMR 6303 CNRSUniv.Bourgogne Franche-ComtéUTBMBelfort 90010France School of Space Science and Physics Shandong UniversityWeihai 264209China

Because the volatile content of isoamyl alcohol increases sharply on the seventh day of wheat mildew infection,isoamyl alcohol can be used as an early biomarker of wheat mildew ***,only a few sensors for isoamyl alcohol detection have been reported,and these sensors still suffer from low sensitivity and poor moisture ***,the isoamyl alcohol sensitivity of 5 at%Er@LaFeO_(3)(ELFO)was enhanced by loading Ag nanoparticles on the surface of the ELFO microspheres,while the optimal operating temperature was *** moisture resistance of Ag/ELFO was improved by the incorporation of g-C_(3)N_(4)nanosheets(NSs)on the surface of Ag/ELFO through electrostatic *** the requirements for practical applications in grain granaries,the sensing behavior of a Ag/ELFO-based sensor incorporating g-C_(3)N_(4)NSs at 20%relative humidity(RH)was systematically studied,and the sensor demonstrated excellent repeatability,long-term stability,and superior selectivity(791 at 50 ppm)for isoamyl alcohol with a low limit of detection(LOD=75 ppb).Furthermore,the practical results obtained for wheat at different mildew stages further confirmed the potential of the g-C_(3)N_(4)/Ag/ELFO-based sensor for monitoring the early mildew stage of *** work may offer guidance for enhancing the moisture resistance of gas-sensitive materials through the strategy of employing composite nanomaterials.

关键词： Ag gas sensor moisture resistance isoamyl alcohol Er@LaFeO_(3)(ELFO) g-C_(3)N_(4)nanosheet(NS)

Urchin-like Na-doped zinc oxide nanoneedles for low-concentration and exclusive VOC detections

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Journal of Advanced Ceramics 2024年第4期13卷 507-517页

作者： Yiwen Zhou Yifan Luo Zichen Zheng Kewei Liu Xiaoxi He Kaidi Wu Marc Debliquy Chao Zhang College of Mechanical Engineering Yangzhou UniversityYangzhou 225127China Material Science Department University of MonsMons 7000Belgium

In the early-stage diagnosis of lung cancer,the low-concentration(<5 ppm)volatile organic compounds(VOCs)are extensively identified to be the biomarkers for breath ***,the urchin-like sodium(Na)-doped zinc oxide(ZnO)n... 详细信息

In the early-stage diagnosis of lung cancer,the low-concentration(gas sensor with a 3:1 molar ratio of Na^(+)and citric acid showed outstanding sensing properties with an optimal selectivity to various VOCs(formaldehyde(HCOH),isopropanol,acetone,and ammonia)based on working temperature ***,significantly enhanced sensitivity(21.3@5 ppm)compared with pristine ZnO(~7-fold),low limit of detection(LOD)(298 ppb),robust humidity resistance,and long-term stability of formaldehyde sensing performances were obtained,which can be attributed to the formation of a higher concentration of oxygen vacancies(20.98%)and the active electron ***,the improved sensing mechanism was demonstrated by the exquisite band structure and introduction of the additional acceptor level,which resulted in the narrowed bandgap of ZnO.

关键词： zinc oxide(ZnO) heterovalent ions doping citric acid gas sensor volatile organic compound(VOC)detection lungcancer

A gas sensing neural circuit for an olfactory neuron

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Communications in Theoretical Physics 2024年第10期76卷 26-40页

作者： Xi-Kui Hu Song Zhu Juan Yang Zhao Yao Ping Zhou Jun Ma School of Science Chongqing University of Posts and Telecommunications School of Physics and Electronics Central South University Department of Physics Lanzhou University of Technology

A gas sensor can convert external gas concentration or species into electric voltage or current signals by physical adsorption or chemical changes. As a result, a gas sensor in a nonlinear circuit can be used as a sensitive sensor for detecting external gas signals from the olfactory system. In this paper, a gas sensor and a field-effect transistor are incorporated into a simple FithzHugh–Nagumo neural circuit for capturing and encoding external gas signals. An improved functional neural circuit is obtained, and the effect of gas concentration, gas species and neuronal activity can be discerned as the gate voltage, threshold voltage and activation coefficient of the field-effect transistor, respectively. The gas concentration can affect the neural activities from quiescent to normal working and, finally, to saturation state in bursting, spiking, periodic and chaotic firings with different frequencies. The effects of gas species and neuronal activity on the firing state can also be achieved in this functional neural circuit. In addition, variations in the gate voltage, threshold voltage and activation coefficient can cause switching between different firing modes. These results can be helpful in designing artificial olfactory devices for bionic gas recognition and other coupled systems arising in applied sciences.

关键词： bifurcation field-effect transistor gas sensor olfactory neural circuit