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Adverse effects of exposure to fine particles and ultrafine particles in the environment on different organs of organisms

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Journal of Environmental Sciences 2024年第1期135卷 449-473页

作者： Jianwei Zhang Zhao Chen Dan Shan Yang Wu Yue Zhao Chen Li Yue Shu Xiaoyu Linghu Baiqi Wang Department of Occupational and Environmental Health School of Public HealthTianjin Medical UniversityTianjin 300070China Department of Medical Tianjin Stomatological HospitalSchool of MedicineNankai UniversityTianjin 300041China Tianjin Key Laboratory of Environment Nutrition and Public HealthTianjin 300070China National Demonstration Center for Experimental Preventive Medicine Education(Tianjin Medical University) Tianjin 300070China

Particulate pollution is a global risk factor that seriously threatens human health.fine particles(FPs)and ultrafine particles(UFPs)have small particle diameters and large specific surface areas,which can easily adsorb metals,microorganisms and other pollutants.FPs and UFPs can enter the human body in multiple ways and can be easily and quickly absorbed by the cells,tissues and organs.In the body,the particles can induce oxidative stress,inflammatory response and apoptosis,furthermore causing great adverse effects.Epidemiological studies mainly take the population as the research object to study the distribution of diseases and health conditions in a specific population and to focus on the identification of influencing factors.However,the mechanism by which a substance harms the health of organisms is mainly demonstrated through toxicological studies.Combining epidemiological studies with toxicological studies will provide a more systematic and comprehensive understanding of the impact of PM on the health of organisms.In this review,the sources,compositions,and morphologies of FPs and UFPs are briefly introduced in the first part.The effects and action mechanisms of exposure to FPs and UFPs on the heart,lungs,brain,liver,spleen,kidneys,pancreas,gastrointestinal tract,joints and reproductive system are systematically summarized.In addition,challenges are further pointed out at the end of the paper.This work provides useful theoretical guidance and a strong experimental foundation for investigating and preventing the adverse effects of FPs and UFPs on human health.

关键词： fine particles Ultrafine particles Organs Adverse effect

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Comprehensive understanding on sources of high levels of fine particulate nitro-aromatic compounds at a coastal rural area in northern China

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Journal of Environmental Sciences 2024年第1期135卷 483-494页

作者： Yueru Jiang Xinfeng Wang Min Li Yiheng Liang Zhiyi Liu Jing Chen Tianyi Guan Jiangshan Mu Yujiao Zhu He Meng Yang Zhou Lan Yao Likun Xue Wenxing Wang Environment Research Institute Shandong UniversityQingdao 266237China Department of Environmental Systems Science Swiss Federal Institute of Technology ZurichZurich 8092Switzerland Department of Water Resources and Drinking Water Swiss Federal Institute of Aquatic Science and TechnologyDuebendorf 8600Switzerland Qingdao Eco-Environment Monitoring Center of Shandong Province Qingdao 266003China College of Oceanic and Atmospheric Sciences Ocean University of ChinaQingdao 266100China School of Environmental and Geographical Sciences Shanghai Normal UniversityShanghai 200234China

Nitro-aromatic compounds(NACs)are among the major components of brown carbon(BrC)in the atmosphere,causing negative impacts on regional climate,air quality,and ecological health.Due to the extensive origins,it is still a challenge to figure out the contributions and originating regions for different sources of atmospheric NACs.Here,field observations on fine particulate NACs were conducted at a coastal rural area in Qingdao,China in the winter of 2018 and 2019.The mean total concentrations of fine particulate nitro-aromatic compounds were 125.0±89.5 and 27.7±21.1 ng/m^(3)in the winter of 2018 and 2019,respectively.Among the measured eleven NACs,nitrophenols and nitrocatechols were the most abundant species.Variation characteristics and correlation analysis showed that humidity and anthropogenic primary emissions had significant influences on the NAC abundances.In this study,two tracing methods of the improved spatial concentration weighted trajectory(SCWT)model and the receptor model of positive matrix factorization(PMF)were combined to comprehensively understand the origins of NACs in fine particles at coastal Qingdao.Four major sources were identified,including coal combustion,biomass burning,vehicle exhaust,and secondary formation.Surprisingly,coal combustion was responsible for about half of the observed nitro-aromatic compounds,followed by biomass burning(~30%).The results by SCWT demonstrated that the coal combustion dominated NACs mainly originated from the Shandong peninsula and the areas to the north and southwest,while those dominated by biomass burning primarily came from local Qingdao and the areas to the west.

关键词： Nitro-aromatic compounds fine particles Source apportionment Originating region Combustion activities

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A preliminary study on pollution characteristics of surfactant substances in fine particles in the Beibu Gulf Region of China

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Journal of Environmental Sciences 2021年第4期33卷 363-372页

作者： Zhengzheng Zhang Hong Li Hongyan Liu Yingchen Bai Jinjuan Li Guorui Zhi Yanting Yu Wenjun Li Hao Zhang Fan Meng National Center for Quality Supervision and Test of Building Engineering China Academy of Building ResearchBeijing 100013China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100021China College of Resource and Environmental Engineering Guizhou UniversityGuiyang 550025China Puyang Institute of Environmental Protection Science Puyang 457000China College of Geoscience and Surveying Engineering Chinese University of Mining&TechnologyBeijing 100083China School of Science Chinese University of GeosciencesBeijing 100083China

The pollution characteristics of surfactant substances in fine particles(PM_(2.5))in spring were studied in the Beibu Gulf Region of China,68 samples of PM_(2.5)were collected at Weizhou Island in Beihai City from March 12 to April 17,2015.The Anionic Surfactant Substances(ASS)and Cationic Surfactant Substances(CSS)in the samples were analyzed using Byethyl Violet Spectrophotometry and Disulfide Blue Spectrophotometry,respectively.Combined with the data from backward trajectory simulation,the effects of air pollutants from remote transport on the pollution characteristics of surfactant substances in PM_(2.5)in the Beibu Gulf Region were analyzed and discussed.The results showed that the daily mean concentrations of ASS and CSS in spring in the Beibu Gulf Region were 165.20 pmol/m^(3)and 8.05 pmol/m^(3),and the variation ranges were 23.21–452.55 pmol/m^(3)and 0.65–31.31 pmol/m^(3),accounting for 1.82‰±1.65‰and 0.12‰±0.11‰of the mass concentration of PM_(2.5),respectively.These concentrations were lower than those in comparable regions around the world.There was no clear correlation between the concentrations of ASS and CSS in PM_(2.5)and the mass concentrations of PM_(2.5).Tourism and air transport had a positive contribution on the concentrations of ASS.The concentration of surfactant substances in PM_(2.5)was significantly impacted by wind speed and wind direction.Atmospheric temperature,air pressure and precipitation had little effect on the concentrations of surfactant substances.Surfactant substances in PM_(2.5)significantly impacted visibility.Results also showed that the main sources of surfactant substances were from the southern China and Southeast Asia.

关键词： fine particles Surfactant substances Pollution characteristics Impact factors Beibu gulf region of China

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Monitoring of Pollution of Air fine particles (PM2.5) and Study on Their Genetic Toxicity

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Biomedical and Environmental Sciences 2004年第4期17卷 452-458页

作者： DONG-QUNXU WEN-LIZHANG InstituteforEnvironmentalHealthandRelatedProductsSafety ChineseCenterforDiseaseControlandPreventionBeijing100021China

Objective To compare PM2.5 pollation level between the city of coal-fuel pollution (Taiyuan) and the city of pollution mixed with coal fuels and vehicle exhausts (Beijing), to analyze the concentration of B[a]p and Pb in the pollutants, and to study the DNA damage by PM2.5. Methods Air fine particles (PM2.5) were collected in Beijing and Taiyuan by means of the filter membrane method, the concentration of B[a]p and Pb were analyzed by high performance liquid chromatography and atomic absorption spectroscopy respectveily, and the damage of DNA by PM2.5 was detected by single cell gel-electrophoresis (SCGE) using the human lung epithelial cells (A549) as target cells. Results The concentration of PM2.5 in the winter of Beijing was 0.028-0.436 mg/m3, and that in Taiyuan was 0.132-0.681 mg/m3. The concentration of B[a]p was 0.104 and 0.156 礸/mg on PM2.5 of Beijing and Taiyuan, respectively, whereas the concentration of Pb was 1.094 and 1.137 礸/mg on PM2.5 of Beijing and Taiyuan, respectively. Exposure to PM2.5 at the concentrations of 5, 50, and 200 礸/mL for 12 h and 24 h caused DNA damage of the human alveolar epithelium, and the ratios of the tailing and length of the tail were all significantly different from those of the negative control group (P<0.05), and indicated a dose-response relationship. Conclusion PM2.5 has certain genetic toxicity.

关键词： Air pollution fine particles DNA damage

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Synthesis and Luminescence Properties of Pr^(3+) Doped Ca_xBa_(1-x)TiO_3 (0.3≤x<1) fine particles

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Journal of Wuhan University of Technology(Materials Science) 2009年第5期24卷 689-693页

作者：何声太 College of Materials Science and Engineering Tianjin Polytechnic University

CaxBa1-xTiO3 （CBT） fine particles doped with red luminescence center of Pr3＋ ions （Pr： CBT） were successfully synthesized by salt assisted spray pyrolysis （SASP） process. Scanning electronic microscope （SEM） and laser scattering analysis demonstrate that salt can be removed from the surface of particles by washing with Milli-Q water and the particles can be further separated by ball-milling to get well-dispersed Pr^3＋ ions doped CBT fine particles. The luminescence properties, such as photoluminescence （PL） and mechanoluminescence （ML）, of as-synthesized Pr： CBT particles were investigated. For Pr： CBT fine particles with different Ca molar ratios, all the samples show one emission at 612 nm, with increasing Ca molar ratio, PL intensity of Pr： CBT fine particles become stronger and stronger. When pressure was loaded on the Pr： CBT pellet, mechanoluminescence（ML） emission was measured. The results show that the ML intensity is proportional to the applied pressure.

关键词： synthesis luminescence mechanoluminescence photoluminescence Pr^3＋ doped CaxBa1-xTiO3 fine particles

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fine particulate matter(PM_(2.5)/PM_(1.0)) in Beijing,China: Variations and chemical compositions as well as sources

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Journal of Environmental Sciences 2022年第11期34卷 187-198页

作者： Lining Luo Xiaoxuan Bai Shuhan Liu Bobo Wu Wei Liu Yunqian Lv Zhihui Guo Shumin Lin Shuang Zhao Yan Hao Jiming Hao Kai Zhang Aihua Zheng Hezhong Tian State Key Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Center for Atmospheric Environmental Studies Beijing Normal UniversityBeijing 100875China School of Environment Tsinghua UniversityBeijing 100084China Department of Environmental Health Sciences School of Public Health University at Albany State University of New York One University Place RensselaerNY 12144USA Analysis and Testing Center Beijing Normal UniversityBeijing 100875China

Particulate matter(i.e.,PM_(1.0) and PM_(2.5)),considered as the key atmospheric pollutants,exerts negative effects on visibility,global climate,and human health by associated chemical compositions.However,our understanding of PM and its chemical compositions in Beijing under the current atmospheric environment is still not complete after witnessing marked alleviation during 2013–2017.Continuous measurements can be crucial for further air quality improvement by better characterizing PM pollution and chemical compositions in Beijing.Here,we conducted simultaneous measurements on PM in Beijing during 2018–2019.Results indicate that annualmean PM_(1.0) and PM_(2.5) concentrations were 35.49±18.61μg/m^(3) and 66.58±60.17μg/m^(3),showing a positive response to emission controls.The contribution of sulfate,nitrate,and ammonium(SNA)played an enhanced role with elevated PM loading and acted as the main contributors to pollution episodes.Discrepancies observed among chemical species between PM_(1.0) and PM_(2.5) in spring suggest that sand particles trend to accumulate in the range of 1–2.5μm.Pollution episodes occurred accompanied with southerly clusters and high formation of SNA by heterogeneous reactions in summer and winter,respectively.Results from positive matrix factorization(PMF)combined with potential source contribution function(PSCF)models showed that potential areas were seasonal dependent,secondary and vehicular sources became much more important compared with previous studies in Beijing.Our study presented a continuous investigation on PM and sources origins in Beijing,which provides a better understanding for further emission control as well as a reference for other cities in developing countries.

关键词： fine particles Haze Chemical species Seasonal variation Source apportionment

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Numerical simulation and experimental study of gas cyclone–liquid jet separator for fine particle separation

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Chinese Journal of Chemical Engineering 2022年第11期51卷 43-52页

作者： Liwang Wang Erwen Chen Liang Ma Zhanghuang Yang Zongzhe Li Weihui Yang Hualin Wang Yulong Chang School of Mechanical and Power Engineering East China University of Science and TechnologyShanghai 200237China College of Architecture and Environment Sichuan UniversityChengdu 610065China

To address the shortcomings of existing particulate matter trapping technology,especially the low separation efficiency of fine particles,herein,a novel gas cyclone-liquid jet separator was developed to research fine particle trapping.First,numerical simulation methods were used to investigate the flow field characteristics and dust removal efficiency of the separator under different working conditions,and to determined suitable experimental conditions for subsequent dust removal experiments.Afterward,the separation efficiency of the separator against five kinds of common particles,including g-C_(3)N_(4),TiO_(2),SiC,talc,and SiO_(2),was experimentally studied.A maximum separation efficiency of 99.48%was achieved for particles larger than 13.1μm,and 96.55%efficiency was achieved for particles larger than 2μm.The best crushing atomization effect was achieved for the separator when uGwas 10 m·s^(-1)and uLwas 3 m·s^(-1),while the best separation effect was achieved when uGwas 10 m·s^(-1)and uLwas 3.75 m·s^(-1).Studies have shown that the gas cyclone-liquid jet separator has excellent applicability in the separation of fine particles.

关键词： Gas cyclone-liquid jet Dust removal fine particles Numerical simulation

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Diurnal variation of number concentration and size distribution of ultrafine particles in the urban atmosphere of Beijing in winter

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Journal of Environmental Sciences 2007年第8期19卷 933-938页

作者： SHI Zong-bo HE Ke-bin YU Xue-chun YAO Zhi-liang YANG Fu-mo MA Yong-liang MA Rui JIA Ying-tao ZHANG Jie Department of Environmental Science and Engineering Tsinghua University Beijing 100084 China. TSI Asia Pacific Beijing Representative Beijing 100084 China College of Earth Sciences Graduate University-of Chinese Academy of Sciences Beijing 100049 China

Number concentration and distribution of airborne particles in the size range 5.6 to 560 nm diameter were measured in Beijing for a 15-d period in winter 2005. Dally average number concentrations of nucleation mode （5.6-20 um）, Aitken mode （20-100 um）, and accumulation mode （100-560 um） particles, and total particles were 17500, 32000, 4000, and 53500 cm^-3, respectively. Average particle size distribution was monomodal with a mode diameter of about 40 um at night and bimodal with mode diameters of about 10 and about 40 um during the daytime. New particle formation events, which were connected to diurnal variation of nucleation mode particles, were observed in more than half of the observation days. The events often started around 10：00-11：00 Chinese Standard Time （CST） and ended up after 3-4 h. Concentrations of Aitken and accumulation mode particles increased from midnight and reached their maxima at about 10：00 CST, and then decreased and became the lowest in the afternoon. Analysis of diurnal cycles in traffic volume and meteorological parameters revealed that the accumulation of the particles in Aitken and accumulation modes in the morning was influenced by formation of an inversion and increase in vehicle emission, and dispersion of such particles in the afternoon was associated with more effective vertical mixing and higher wind speed.

关键词： fine particles nucleation mode Aitken mode new particle formation

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Numerical prediction of particle slip velocity in turbulence by CFD-DEM simulation

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Particuology 2023年第9期80卷 170-179页

作者： Zhixin Sun Xiaokang Yan Lijun Wang Xiaoheng Li Ai Wang Haijun Zhang School of Chemical Engineering China University of Mining and TechnologyXuzhou221116China School of Low-Carbon Energy and Power Engineering China University of Mining and TechnologyXuzhou221116China National Engineering Research Center of Coal Preparation and Purification China University of Mining and TechnologyXuzhou221116China School of Engineering The University of NewcastleCallaghanNSW2308Australia

Turbulent environment improves the flotation recovery of fine particles by promoting the particle–bubble collision rate,which directly depends on the particle slip velocity.However,the existing slip velocity models are not applicable to fine particles in turbulence.The mechanism of turbulence characteristics and particle properties on the slip velocity of fine particles in turbulence was unclear.In this study,a coupled ANSYS FLUENT and EDEM based on computational fluid dynamics(CFD)and discrete element method(DEM)were used to simulate the slip velocity of fine particles in the approximately homogenous isotropic turbulence,which was excited by the grid.The reliability of the used CFD-DEM simulation method was validated against the slip velocity measured by the particle image velocimetry(PIV)experiments.In particular,the effects of the particle shapes,particle densities,and turbulence intensities on the slip velocity have been investigated with this numerical method.Numerical results show that particle shapes have no significant effect on fine particles between 37 and 225μm.The slip velocity of the spherical particles increases with the turbulence intensity and particle density.Based on the simulated data,a model which has a correlation coefficient of 0.95 is built by using nonlinear fitting.

关键词： Slip velocity fine particles Turbulence CFD-DEM

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Numerical study on the integrated effects of supplied air velocity and exhaust velocity on particles removal for industrial buildings

能源与人工环境(英文)

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能源与人工环境(英文) 2021年第4期2卷 380-391页

作者： Tingsen Chen Shi-Jie Cao School of Architecture Southeast University2 SipailouNanjing 210096China Guangdong Provincial Key Laboratory of Building Energy Efficiency and Application Technologies Guangzhou UniversityGuangzhou510006China Global Centre for Clean Air Research(GCARE) Department of Civil and Environmental EngineeringFaculty of Engineering and Physical SciencesUniversity of SurreyGuildfordSurreyUnited Kingdom

Due to production particularity in industrial buildings,high concentrations of particulate matter are always im-portant environmental issues.Long-term exposure to such hazardous environment may lead to respiratory and cardiovascular diseases.Mechanical ventilation plays a vital role in reducing indoor particulate matter concen-trations.However,the current industrial ventilation generally has the disadvantage of low ventilation efficiency and high energy consumption.In this study,we proposed a ventilation design by integrating supply and exhaust ventilation(i.e.,SEV),and further investigated the effects of combined velocities on both indoor particles re-moval and energy efficiency.Computational Fluid Dynamics(CFD)coupled with Discrete Phase Model(DPM)was employed.The RNG k-𝜀model was adopted to simulate airflow field.Lagrangian method was used to trace particles’dispersion processes.A series of cases were conducted under ventilated conditions with combinations of different supplied velocities of 0.75,1.12,1.50 and 1.87 m/s,and exhausted velocities of 0,0.28 and 0.56 m/s.Temperature effects were not considered in this work.The quantification of combined effects of supply velocity and exhaust velocity were investigated in terms of particle removal efficiency as well as energy saving.Results showed that combined effects of supply velocity and exhaust velocity can improve the ventilation efficiency by 20%-40%compared to the conventional supply ventilation without exhaust velocity.Moreover,the reasonable design of integrated velocities will save up to 70%energy while keeping the same ventilation efficiency of SEV.These findings will be of great importance for energy-efficient design for industrial ventilation systems.

关键词： Industrial ventilation fine particles Exhaust velocity Ventilation design Energy

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