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Ultrafast photoexcitation dynamics behavior of hydrogen-bonded polyfluorenol

Chinese Chemical Letters 2024年第1期35卷 486-491页

作者： Man Xu Chuanxin Wei Yunlong Zhang Hao Li Jingyao Ma Jinyi Lin Shengjie Wang Wei Xue Qi Wei Linghai Xie Wei Huang State Key Laboratory of Organic Electronics and Information Displays&School of Chemistry and Life Sciences&Institute of Advanced Materials(IAM) Nanjing University of Posts&TelecommunicationsNanjing 210023China Key Laboratory of Flexible Electronics(KLOFE)&Institute of Advanced Materials(IAM) Nanjing Tech University(NanjingTech)Nanjing 211816China Frontiers Science Center for Flexible Electronics(FSCFE) Shaanxi Institute of Flexible Electronics(SIFE)&Shaanxi Institute of Biomedical Materials and Engineering(SIBME)Northwestern Polytechnical UniversityXi’an 710072China

exciton behavior is crucial to the exploitation of light-emitting conjugated polymer(LCPs)for optoelectronic *** excitons are easily trapped by the intrinsically defect ***,we set a polyfluorenol(PPFOH)as an example to systematically investigate its photophysical behavior to check the role of defect structures in *** to time-resolved photoluminescence analysis,the feature emission peaks from individual chain of PPFOH in diluted DMF solution is effectively avoided the influence of fluorenone formation,but the residual green-band emission at 550nm is easily observed in the PL spectra of PPFOH dilute toluene solution obtained delay 1.5 ns,confirmed the formation of“guest”physical aggregation-induced defect ***,efficient and ultrafast energy transfer from individual chain to defect structure is observed in PPFOH ***,the efficient energy transfer happened for the film obtained from DMF solution(200 ps)than those of toluene ones(600 ps).Meanwhile,compared to relatively stable green-band emission in PPFOH film from toluene solution,red-shifted emission peak(11 nm)of PPFOH film from DMF solutions exposed to saturated DNT vapor also confirmed their different aggregation-induced green-band ***,this aggregation defect structures are influenced on the photophysical property of LCPs in solid states.

关键词： Photoexcitation dynamics Polyfluorenol Aggregation behavior Energy transfer exciton migration

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