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element migration and enrichment characteristics of bedrock–regolith–soil–plant continuum system in the chestnut planting area,Chengde,China

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Acta Geochimica 2022年第5期41卷 839-860页

作者： Xiaofeng Wei Houyun Sun Zirang Chen Xia Li Hao Wei Wenru Jia Wei Li Sino-Zijin Resources Co.Ltd Beijing 100081China 2 School of Water Resources and EnvironmentChina University of Geosciences(Beijing) Beijing 100083China Beijing Institute of Geology for Mineral Resources Beijing 100012China China Institute of Geo-Environment Monitoring Beijing 100081China Hebei Center for Ecological and Environmental Geology Research Hebei GEO UniversityShijiazhuang 050031China

In order to probe the geochemical relationship between the quality of economic crops and ecological geochemistry,this project studies the chestnut production area of Chengde City,Hebei Province,China.The chemical weathering index,chemical depletion fraction CDF,mass transfer coefficient,and bioconcentration coefficient were used to quantify the characteristics of element migration and accumulation in the BRSPC(Bedrock–Regolith–Soil–Plant Continuum system)system of gneiss formation area and dolomite formation area.The results show that the soil CaO,SiO_(2),Al_(2)O_(3),and Na_(2)O elements in the gneiss construction area are abundant,and the B,Ge,S,and Mo elements are relatively lacking;the soil B,Mo and Ge elements in the dolomite construction area are abundant,and the SiO_(2),Al_(2)O_(3),and Na_(2)O elements are slightly lower;The weathering intensity of gneiss is low-medium,with the relatively high mobility and apparent transformation of Se,B,V,S,Mn,and Mo.The weathering intensity of dolostone is low,with the relatively high mobility and apparent transformation of Na_(2)O,P,and Ni.Chestnut is rich in Cu,Ni,Se,and Ge,walnut has a high content of Mo,and hawthorn is rich in Se and B.The contents of Mn in chestnut are 1–2 times higher in walnut and hawthorn.It lays the theoretical foundation for the industry optimization of special industrial crop planting in Chengde according to our research.

关键词： Critical zone Eco-geochemistry element migration Chestnut Chengde

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element migration and phase distribution characteristics during crystallization of rare earth phase in rare earth slag

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Journal of Rare Earths 2023年第5期41卷 780-788,I0006页

作者： Wanli Yi Xuefeng She Huai Zhang Zhenlong An Jingsong Wang Qingguo Xue State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBejing 100083China Department of Energy and Resources Engineering College of EngineeringPeking UniversityBeijing 100871China

The crystallization experiment of molten rare earth(RE)slag under different cooling rates was carried out.The characteristics of element migration and phase distribution during RE phase crystallization were studied by using different equipment.The experimental results show that there are two RE phases in the RE slag,namely(Ca,Ce,La)_(5)(SiO_(4))6F and(Ca,Ce,La,Mg)_(3)(Ti,Al,Nb)_(2)O_(7).During the cooling crystallization process of molten RE slag,Ca and P elements in the RE phase of(Ca,Ce,La)_(5)(SiO_(4))_(6)F migrate from inside to outside,and finally gather at the outer edge of the phase to form phase Ca_(3)(PO4)2.The RE phase(Ca,Ce,La)_(5)(SiO_(4))_(6)F is distributed inside the furnace-cooled slag,and the RE phase(Ca,Ce,-La,Mg)_(3)(Ti,AI,Nb)_(2)O_(7)is distributed in the surface layer of the furnace-cooled slag.And based on the phase distribution characteristics,the central hollowing method is proposed to realize the preliminary enrichment of valuable elements Ti,Nb and RE in RE slag.

关键词： Rare earth slag element migration Phase distribution element enrichment

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Trace element Mobility in Subducted Marble and Associated Eclogite:Constraints from UHP Rocks in the Shuanghe Area,Central-East China

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Journal of Earth Science 2024年第1期35卷 1-15页

作者： Xingao Hou Zhiqiang Yu Shefa Chen Lei Liu Yilin Xiao Key Laboratory of Metallogenic Prediction of Nonferrous Metals and Geological Environment Monitoring Ministry of EducationSchool of Geosciences and Info-PhysicsCentral South UniversityChangsha 410083China Key Laboratory of Mineralogy and Metallogeny Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou 510640China CAS Key Laboratory of Crust-Mantle Materials and Environments School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

In order to decipher element mobility in UHP meta-sedimentary rocks in the continental subduction zone,major and trace element compositions are investigated for a continuous profile from a representative UHP region in the Dabie Mountains.Among the lithologic contact zone,contents of K,Ca,LREE,and LILE exhibit varying degrees of downward trends in both marble and eclogite toward the contact zone,indicating that marble and their associated eclogite can release a large amount of K,Ca,and a small number of LILEs and LREEs.Titanite is the main Ti phase in both marble and eclogite.Titanite rims around rutile can occasionally be seen in eclogite.Contents of Ti and HFSE exhibit a well-coupled relation among marble and eclogite,indicating that substantial Ti and HFSEs were migrated from eclogite to marble,in accord with the capacity of a melt medium.Rutiles and titanites in marble exhibit a relatively limited variation in Nb/Ta ratios(12.9-16.2),similar to those of titanites in eclogite(14.2-16.7),which demonstrates that rutiles and titanites in marble were sourced from eclogite because of short-distance migrations of Ti and HFSEs.According to the P-T path and the temperature and pressure conditions of the peak metamorphism reported by previous studies,the eclogite associated with marble may not form supercritical fluids in the subduction zone because of the addition of carbonate minerals.

关键词： UHP metamorphism eclogite marble element migration fluid actions geochemistry

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Oxidation Kinetics,Structural Changes and element migration during Oxidation Process of Vanadium-titanium Magnetite Ore

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Journal of Iron and Steel Research(International) 2016年第11期23卷 1160-1167页

作者： Feng PAN Qing-shan ZHU Zhan DU Hao-yan SUN State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of Sciences Beijing 100039China

The oxidation kinetics, structural changes, and elements migration during the oxidation process of the va- nadium-titanium magnetite （VTM） ore were analyzed. Kinetics analysis indicated that the oxidation process was con- trolled by diffusion control and could be divided into interface diffusion and lattice diffusion with apparent activation energy of 99.69 kJ/mol and 144.08 kJ/mol in the range of 800--1000℃, respectively. The surface structure changed with the oxidization temperature as follows： dense surface→nano sized sheets→submicron particles→molten particles. The compact structure changed into porous one because of the elements migration and enrichment. Both Fe and Ti elements migrated in the opposite direction during the oxidation process. The V etement in the raw ore stably existed in the form of V^5＋ state, some vanadium migrated and occupied the tetrahedral sites of the hematite during the oxidation process.

关键词： vanadium-titanium magnetite ore oxidation kinetics structural change element migration

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Chemical weathering intensity and element migration features of the Xiashu loess profile in Zhenjiang, Jiangsu Province

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Journal of Geographical Sciences 2008年第3期18卷 341-352页

作者： CHEN Yingyong LI Xusheng HAN Zhiyong YANG Shouye WANG Yongbo YANG Dayuan School of Geographic and Oceanographic Sciences Nanjing University Nanjing 210093 China State Key Laboratory of Loess and Quaternary Geology Institute of Earth Environment CAS Xi＇an 710075 China State Key Laboratory of Marine Geology Tongji University Shanghai 200092 China

The chemical weathering intensity and element migration features of the Xiashu loess profile in Zhenjiang are studied in this paper.（1）The Xiashu loess profile underwent moderate chemical weathering.It seems that the precipitation is a more important factor than the temperature in controlling the process of the chemical weathering.（2）The major elements such as Si,K,Na,Ca,Mg,Mn and P were migrated and leached,while the elements Fe and Ti were slightly enriched.The migration features of the major elements reveal that the Xiashu loess finished the primary process of chemical weathering characterized by leaching of Ca and Na,and almost reached the secondary process characterized by leaching of K.Except the elements Sr and Ga,other trace elements such as Th,Ba,Cu,Zn,Co,Ni,Cr and V were enriched.It might be caused by both the biogeochemical process and the adsorption of trace elements by clay mineral and organic materials.（3）The difference of element migration down the Xiashu loess profile reveals that the climate was warm and wet at the early-middle stage of the middle Pleistocene.At the end of the middle Pleistocene,it became dry and cool.At the early stage of the Late Pleistocene,the paleoclimate became warm and wet again.As a whole,the paleoclimate generally became drier and cooler in this region from the beginning of the middle Pleistocene.

关键词： Xiashu loess chemical weathering element migration Zhenjiang

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Characteristics of element migration in the Process of Wall-Rock Alteration in the Shibangou Gold Deposit,Western Henan

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Acta Geologica Sinica(English Edition) 1999年第2期73卷 201-207页

作者： WEI Junhao LI Jianwei YUAN Yanbin Faculty of Earth Resources China University of Geosciences Wuhan Hubei 430074

Abstract The Shibangou gold deposit in western Henan is associated with irregular quartz veinlets occurring in altered shear zones dissecting a dioritic intrusion. The altered shear zones are characterized by silicification, pyritization, sericilization, chloritization and K-feldspar alteration. Zoning of altered rocks adjacent to the Au-bearing quartz veins is obviously exhibited. Fine-grained sulphides and quartz veinlets of different ages and small-scale fissures are widely distributed in the central part of the altered zones. Major mineralization types in this gold deposit are Au-bearing quartz veinlets and altered rocks in the shear zones. Samples were collected from drilling cores according to the alteration zoning and mineralization type and all samples were analyzed for major and trace elements. Mass balance, volume change (fv=97.3–71.9%) and major element variation sequences are studied in terms of major elements. The changes of mobile components (SiO2, K2O, Fe2O3) and CaO) and immobile component (Al2O3) in the wall-rock alteration are discussed. The gold mineralization is associated with the enrichment of As, Ag, Hg and Pb and depletion of Cu and Zn. The study of compositional variation of altered rocks proves to be a very efficient method for defining the extent of wall-rock alteration, fluid activity and mineralization and enrichment.

关键词： wall-rock alteration element migration mass balance Shibangou gold deposit

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migration of harmful elements in municipal sludge under hightemperature oxidation conditions

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Journal of Iron and Steel Research(International) 2023年第9期30卷 1701-1713页

作者： Xiao-dong Ping Hai-feng Wang Feng Wang Xin-yu Wan Zhi-wei An Jian-lei Pan State Key Laboratory of Advanced Steel Processes and Products Central Iron and Steel Research Institute Co.Ltd.Beijing 100081China Department of Science and Technology Development China Iron and Steel Research Institute Group Co.Ltd.Beijing 100081China Production and Equipment Department Chengde Jianlong Special Steel Co.Ltd.Chengde 067200HebeiChina Technology Department Chengde Jianlong Special Steel Co.Ltd.Chengde 067200HebeiChina

Municipal sludge is produced in large amounts and is difficult to treat.Incineration is the most direct and thorough treatment method.In order to study the feasibility of sintering for municipal sludge treatment,the municipal sludge reforming process was studied under high-temperature oxidation conditions.The results showed that the sludge reforming process could be divided into four stages:the precipitation and evaporation of adsorbed water,the precipitation and combustion of the volatile,the combustion of the residual volatile and solid carbon,and the decomposition of salts and the melting of sludge.An increase in the heating rate resulted in more intense sludge combustion and improved the sludge reaction capacity and combustion performance.After burning at 1300℃,Si,Ca,Mg,Al,K,Na,and Cu formed new phases and entered the slag.75%of P remained in the slag.80%of the S formed SO_(2) and entered the flue gas.Cl formed gaseous chlorides like HCl upon combustion and entered the flue gas.As sintering is a feasible method for treating municipal sludge,care must be taken to limit the amount of P that ends up in the ore.

关键词： Municipal sludge Oxidizing atmosphere Mini-sintering Reforming process element migration

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Geochemical characteristics and growth suitability assessment of Scutellaria baicalensis Georgi in the Earth's critical zone of North China

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Journal of Mountain Science 2022年第5期19卷 1245-1262页

作者： LI Xia WEI Xiao-feng WU Jin YIN Zhi-qiang WAN Li-qin SUN Hou-yun AN Yong-long College of Water Sciences Beijing Normal UniversityBeijing 100875China China Institute of Geo-Environment Monitoring Beijing 100081China Beijing Institute of Geology for Mineral Resources Beijing 100012China Faculty of Architecture Civil and Transportation EngineeringBeijing University of TechnologyBeijing 100124China School of Water Resources&Environment China University of GeosciencesBeijing 100083China

Geochemical differentiation of soils has a series of consequences on plant and places pressure on the ecological environment.The quantitative evaluation of element migration in the Earth’s critical zone is a challenging task.In this study,two demonstration study areas of Scutellaria baicalensis Georgi were selected,and multiple chemical weathering indexes,chemical loss fraction,mass migration coefficients and biological enrichment coefficient method were used to assess the ecological and geochemical suitability.The results show that for the element of Fe,Zn,Se,Cu,Co,Ni,Mo and Ge,the degree of weathering and soil maturation,were greater in the rhyolitic tuff area than in the Plagioclase gneiss area.In both research sites,the heavy metal level of samples in Scutellaria baicalensis Georgi did not exceed the standard limits.The plagioclase gneiss region’s surface soil environment was more alkaline,and the content of soil organic matter was lower,resulting in a higher bioenrichment intensity of Ge,Co,Cu,and Se elements in Scutellaria baicalensis Georgi than in the rhyolite-tuff area.The elements of Cd,Nb,Mo,Pb and As are considerably enriched in the soil of the plagioclase gneiss area but lost by leaching in the soil of the rhyolite tuff area,which is connected to the interplay of elemental abundance and human impact in the parent materials.This study provides a good example of how to assess growth suitability of Chinese medicinal materials in the Earth’s critical zone.

关键词： Earth’s critical zone Biogeochemistry characteristics Weathering mechanism element migration Chinese medicinal materials Chengde

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Effect mechanism of aluminum occurrence and content on the induration characteristics of iron ore pellets

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International Journal of Minerals,Metallurgy and Materials 2023年第12期30卷 2334-2346页

作者： Hongyu Tian Deqing Zhu Jian Pan Congcong Yang Weiqun Huang Mansheng Chu School of Metallurgy Northeastern UniversityShenyang 110819China School of Minerals Processing and Bioengineering Central South UniversityChangsha 410083China Ecological Geology Brigade of Jiangxi Geological Bureau Nanchang 330030China Engineering Research Center of Frontier Technologies for Low-carbon Steelmaking(Ministry of Education) Shenyang 110819China

With the intensified depletion of high-grade iron ores,the increased aluminum content in iron ore concentrates has become unavoidable,which is detrimental to the pelletization process.Therefore,the effect mechanism of aluminum on pellet quality must be identified.In this study,the influence of aluminum occurrence and content on the induration of hematite(H)and magnetite(M)pellets was investigated through the addition of corresponding Al-containing additives,including alumina,alumogoethite,gibbsite,and kaolinite.Systematic mineralogical analysis,combined with the thermodynamic properties of different aluminum occurrences and the quantitative characterization of consolidation behaviors,were conducted to determine the related mechanism.The results showed that the alumina from various aluminum occurrences adversely affected the induration characteristics of pellets,especially at an aluminum content of more than 2.0wt%.The thermal decomposition of gibbsite and kaolinite tends to generate internal stress and fine cracks,which hinder the respective microcrystalline bonding and recrystallization between Fe2O3particles.The adverse effect on the induration characteristics of fired pellets with different aluminum occurrences can be relieved to varying degrees through the formation of liquid phase bonds between the hematite particles.Kaolinite is more beneficial to the induration process than the other three aluminum occurrences because of the formation of more liquid phase,which improves pellet consolidation.The research results can further provide insights into the effect of aluminum occurrence and content in iron ore concentrates on downstream processing and serve as a guide for the utilization of high-alumina iron ore concentrates in pelletization.

关键词： iron ore pellet aluminum occurrence consolidation behavior element migration

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Thermodynamic modeling and elemental migration for the early stage of rodingitization:An example from the Xialu massif of the Xigaze ophiolite,southern Tibet

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Geoscience Frontiers 2021年第3期12卷 557-576页

作者： Wen-Yong Duan Xu-Ping Li Ze-Li Wang Shuang Chen Guang-Ming Sun Ling-Quan Zhao Shandong Provincial Key Laboratory of Depositional Mineralization and Sedimentary Minerals Shandong University of Science and TechnologyQingdao 266590China Institute of Geology Mineralogy and GeophysicsFaculty of GeosciencesRuhr-University Bochum44780 BochumGermany

The analysis of early stage rodingite from the ultramafic rocks of the Xialu Massif in the Xigaze Ophiolite,Tibet,in China shows that the rodingitization involved continuous changes in fluid composition during different stages of subduction.The early stage prehnite-bearing rodingite was produced at low pressures and temperatures along extensional fractures.Samples of rodingite were collected along a profile from the center to the margin of a rodingitized intrusive igneous rock(^10 m×30 m),and they record wide variations in bulk composition,mineralogy,and texture.The mineral assemblages,from center to margin,vary from(1)relics of primary clinopyroxene(Cpx_(r))and primary amphibole(Amp_(r))+newly formed late amphibole(Act)+primary plagioclase(Pl_(r))+clinozoisite+prehnite+albite+chlorite+titanite+ilmenite(R1 rodingite),through(2)relics of primary clinopyroxene(Cpx_(r))+newly formed late clinopyroxene(Cpx_(n))+primary and late amphiboles(Amp_(r)+Act)+clinozoisite+prehnite+albite+chlorite+titanite(R2 rodingite),to(3)newly formed late clinopyroxene(Cpx_(n))and amphibole(Act)+clinozoisite+prehnite+albite+chlorite+titanite(R3 rodingite).As a result of the metasomatic process of rodingitization,the content of CaO in the whole rock chemical composition from R1 to R3 increases,SiO_(2) decreases,and Na_(2)O+K_(2)O is almost completely removed.Massbalance diagrams show enrichments in large ion lithophile elements such as Rb,Cs,Ba,and Pb as well as Ni during rodingitization.The central part of the rodingitized intrusion(R1 rodingite)was only slightly affected by metasomatism.On the other hand,the contents of the rare earth elements(REEs),high field strength elements(HFSEs;e.g.Zr,Nb,Ta,Hf,and Y),and some highly compatible elements such as Cr and Sc decreased slightly during rodingitization.Thermodynamic modeling based on equilibrium mineral assemblages indicates that the rodingite of the Xialu Massif formed in an H_(2)O-saturated,CO_(2)-rich environment.The estimated conditions of metamorphism were-281-323℃and 0.4-3.9 kbar,rep

关键词： Early stage rodingitization element migration Thermodynamic modeling Xialu Massif Xigaze Ophiolite Southern Tibet

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