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Polyoxometalate-based electrolyte materials in redox flow batteries:Current trends and emerging opportunities

materials Reports(Energy) 2022年第2期2卷 39-57页

作者： Yiyang Liu Jialin Zhang Shanfu Lu Yan Xiang Beijing Key Laboratory of Bio-inspired Energy materials and Devices School of Space and EnvironmentBeihang UniversityBeijing100191PR China

Redox flow batteries have received wide attention for electrochemical energy conversion and storage devices due to their specific advantage of uncoupled power and energy devices,and therefore potentially to reduce the capital costs of energy *** structural features of polyoxometalates exhibit unique advantages in redox flow batteries,such as,stable chemical properties,multi-electron reaction,good redox reversibility,low permeability,etc,which furnishes a novel perspective for settling various problems of redox flow *** was a comprehensive and critical review of this type of batteries,focusing mainly on the chemistry of polyoxometalate electrolyte materials and introducing a systematic ***,challenges and perspectives of polyoxometalate electrolyte materials and polyoxometalate redox flow batteries are discussed.

关键词： Redox flow battery electrolyte materials Polyoxometalate electrolyte design

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Recent progress in the all-solid-state flexible supercapacitors

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SmartMat 2022年第3期3卷 349-383页

作者： Yongrui Yang Tao Zhu Lening Shen Yanghe Liu Dong Zhang Bowen Zheng Keven Gong Jie Zheng Xiong Gong School of Polymer Science and Polymer Engineering The University of AkronAkronOhioUSA Department of Chemical Biomolecular and Corrosion EngineeringThe University of AkronAkronOhioUSA Copley High School CopleyOhioUSA Western Reserve Academy HudsonOhioUSA

In the past few years,supercapacitors(SCs)have attracted great attention in both academic and industrial sectors due to their high energy storage efficiency,reliable stability,and eco-friendly *** solid-state SCs as one of the ongoing focuses for the development of wearable and portable electronics have become the most promising energy storage devices for the smart power system due to their high power density,fast electrochemical response,high efficiency on the charge-discharge process,and excellent electrochemical *** this study,the recent progress in the electrodes and electrolytes used for approaching high-performance of the all-solid-state flexible SCs is *** first introduce basic operational principles of various *** then we overview the electrode materials including carbon materials,conducting polymers,transition metal oxides/chalcogenides/nitrides,MXenes,metal-organic frameworks,covalent-organic frameworks,and the polymer-based solid-state electrolytes in different ***,we summarize recent progress in the development of the all-solid-state flexible SCs and outlook for future research directions.

关键词： electrode materials electrolyte materials flexible supercapacitors solid-state supercapacitors

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