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Progress on direct assembly approach for in situ fabrication of electrodes of reversible solid oxide cells

Materials Reports(Energy) 2021年第2期1卷 61-69页

作者： Na Ai Yuanfeng Zou Zhiyi Chen Kongfa Chen San Ping Jiang College of Materials Science and Engineering Fuzhou UniversityFuzhouFujian350108China Testing Center Fuzhou UniversityFuzhouFujian350108China WA School of Mines:Minerals Energy&Chemical EngineeringCurtin UniversityPerthWA6102Australia

Reversible solid oxide cells(SOCs)are very efficient and clean for storage and regeneration of renewable electrical energy by switching between electrolysis and fuel cell *** of the most critical factors governing the efficiency and durability of SOCs technology is the stability of the interface between oxygen electrode and electrolyte,which is conventionally formed by sintering at a high temperature of~1000–1250℃,and which suffers from delamination problem,particularly for reversibly operated *** the other hand,our recent studies have shown that the electrode/electrolyte interface can be in situ formed by a direct assembly approach under the electrochemical polarization conditions at 800℃and *** direct assembly approach provides opportunities for significantly simplifying the cell fabrication procedures without the doped ceria barrier layer,enabling the utilization of a variety of high-performance oxygen electrode materials on barrier layer–free yttria-stabilized zirconia(YSZ)*** importantly,the in situ polarization induced interface shows a promising potential as highly active and durable interface for reversible *** objective of this progress report is to take an overview of the origin and research progress of in situ fabrication of oxygen electrodes based on the direct assembly *** prospect of direct assembly approach in the development of effective SOCs and in the fundamental studies of electrode/electrolyte interface reactions is discussed.

关键词： Reversible solid oxide cell Direct assembly Oxygen electrode Hydrogen electrode Polarization induced interface electrode/electrolyte interface stability

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