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Arsenic species in electronic cigarettes:Determination and potential health risk

Journal of environmental Sciences 2020年第5期32卷 168-176页

作者： Qingqing Liu Chengzhi Huang XChris Le Chongqing Key Laboratory of Biomedical Analysis(Southwest University) Chongqing Science&Technology CommissionCollege of Chemistry and Chemical EngineeringSouthwest UniversityChongqing 400715China College of Resources and environment Southwest UniversityChongqing400715China Key Laboratory of Luminescent and Real-Time Analytical System Chongqing Science and Technology BureauCollege of Pharmaceutical SciencesSouthwest UniversityChongqing 400715China Department of Laboratory Medicine and Pathology Faculty of Medicine and DentistryUniversity of Alberta10102 Clinical Sciences BuildingEdmontonAlberta T6G 2G3Canada

Human exposure to contaminants from electronic cigarettes(e-cigarettes)and the associated health effects are poorly *** has been no report on the speciation of arsenic in e-liquid(solution used for e-cigarettes)and *** report here determination of arsenic species in e-liquids and aerosols generated from vaping the *** e-liquid samples of major brands,purchased from local and online stores in Canada and China,were analyzed for arsenic species using high-performance liquid chromatography and inductively coupled plasma mass *** condensed from vaping the eliquids were also analyzed and compared for arsenic *** arsenic species were detected,including inorganic arsenate(iAsⅤ),arsenite(iAsⅢ),monomethylarsonic acid(MMA),and three new arsenic species not reported *** e-liquids,iAsⅢwas detected in 59%,iAsⅤin 94%,and MMA in 47%of the *** the condensate of aerosols from vaping the e-liquids,iAsⅢwas detected in 100%,iAsv in 88%,and MMA in 13%of the *** arsenic species were predominant in e-liquids and aerosols of *** concentration of iAsⅢin the condensate of aerosols(median 3.27μg/kg)was significantly higher than that in the e-liquid(median 1.08μg/kg)*** concentration of inorganic arsenic in the vaping air was approximately 3.4μg/m3,which approaches to the permissible exposure limit(10μg/m3)set by the United States Occupational Safety and Health Administration(OSHA).According to the environmental Protection Agency’s unit risk factor(4.3×10-3 perμg/m3)for inhalation exposure to inorganic arsenic in the air,the estimated excess lung cancer risk from lifetime exposure to inorganic arsenic in the ecigarette vaping air(3.4μg/m3),assuming e-cigarette vaping at 1%of the time,is as high as1.5×*** results raise health concerns over the exposure to arsenic from electronic cigarettes.

关键词： electronic cigarettes e-liquid e-cigarette aerosol Arsenic speciation Inhalation exposure Metals Lung cancer risk

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