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Multi-Pollutant Formation and Control in Pressurized Oxy-Combustion:SO_(x),NO_(x),Particulate Matter,and Mercury

Engineering 2024年第8期39卷 127-153页

作者： Gaofeng Dai Jiaye Zhang Zia ur Rahman Yufeng Zhang Yili Zhang Milan Vujanović Hrvoje Mikulčić Nebojsa Manic Aneta Magdziarz Houzhang Tan Richard L.Axelbaum Xuebin Wang MOE Key Laboratory of Thermo-Fluid Science and Engineering Xi’an Jiaotong UniversityXi’an 710049China School of Ecology and Environment Hainan UniversityHaikou 570228China Faculty of Mechanical Engineering&Naval Architecture University of ZagrebZagreb 10000Croatia Faculty of Mechanical Engineering University of MariborMaribor 2000Slovenia Faculty of Mechanical Engineering University of BelgradeBelgrade 11120Serbia AGH University of Krakow Krakow 30059Poland Consortium for Clean Coal Utilization Department of EnergyEnvironmental&Chemical EngineeringWashington University in St.LouisSt.LouisMO 63130USA

Oxy-combustion is a promising carbon-capture technology,but atmospheric-pressure oxy-combustion has a relatively low net efficiency,limiting its application in power *** pressurized oxycombustion(POC),the boiler,air separation unit,flue gas recirculation unit,and CO_(2)purification and compression unit are all operated at elevated pressure;this makes the process more efficient,with many advantages over atmospheric pressure,such as low NO_(x)emissions,a smaller boiler size,and *** is also more promising for industrial application and has attracted widespread research interest in recent *** can produce high-pressure CO_(2)with a purity of approximately 95%,which can be used directly for enhanced oil recovery or ***,the pollutant emissions must meet the standards for carbon capture,storage,and *** of the high oxygen and moisture concentrations in POC,the formation of acids via the oxidation and solution of SO_(x)and NO_(x)can be increased,causing the corrosion of pipelines and ***,particulate matter(PM)and mercury emissions can harm the environment and human *** main distinction between pressurized and atmospheric-pressure oxy-combustion is the former’s elevated pressure;thus,the effect of this pressure on the pollutants emitted from POC—including SO_(x),NO_(x),PM,and mercury—must be understood,and effective control methodologies must be incorporated to control the formation of these *** paper reviews recent advances in research on SO_(x),NO_(x),PM,and mercury formation and control in POC systems that can aid in pollutant control in such systems.

关键词： Pressurized oxy-combustion Sulfur oxides Nitrogen oxides Particulate matter Mercury direct contact cooler Carbon capture and sequestration

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