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Enhanced gas production and CO_(2) storage in hydrate-bearing sediments via pre-depressurization and rapid CO_(2) injection

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Chinese Journal of Chemical Engineering 2024年第3期67卷 126-134页

作者： Hongnan Chen Yifei Sun Bojian Cao Minglong Wang Ming Wang Jinrong Zhong Changyu Sun Guangjin Chen State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China School of Chemistry and Chemical Engineering Changsha University of Science&TechnologyChangsha 410114China

Carbon emission reduction and clean energy development are urgent demands for mankind in the coming decades.Exploring an efficient CO_(2) storage method can significantly reduce CO_(2) emissions in the short term.In this study,we attempted to construct sediment samples with different residual CH_(4) hydrate amounts and reservoir conditions,and then investigate the potentials of both CO_(2) storage and enhanced CH_(4) recovery in depleted gas hydrate deposits in the permafrost and ocean zones,respectively.The results demonstrate that CO_(2) hydrate formation rate can be significantly improved due to the presence of residual hydrate seeds;However,excessive residual hydrates in turn lead to the decrease in CO_(2) storage efficiency.Affected by the T-P conditions of the reservoir,the storage amount of liquid CO_(2) can reach 8 times that of gaseous CO_(2),and CO_(2) stored in hydrate form reaches 2-4 times.Additionally,we noticed two other advantages of this method.One is that CO_(2) injection can enhance CH_(4) recovery rate and increases CH_(4) recovery by 10%-20%.The second is that hydrate saturation in the reservoir can be restored to 20%-40%,which means that the solid volume of the reservoir avoids serious shrinkage.Obviously,this is crucial for protecting the goaf stability.In summary,this approach is greatly promising for high-efficient CO_(2) storage and safe exploitation of gas hydrate.

关键词： Hydrate depressurization CO_(2) storage CH_(4) production Reservoir remediation

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Rate-limiting factors in hydrate decomposition through depressurization across various scales:A mini-review

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Chinese Journal of Chemical Engineering 2024年第3期67卷 206-219页

作者： Xian Sun Peng Xiao Qinfeng Shi Lingban Wang Zhenbin Xu Yuhao Bu Xiaohui Wang Yifei Sun Changyu Sun Guangjin Chen State Key Laboratory of Heavy Oil Processing China University of Petroleum(Beijing)Beijing 102249China Jining University Jining 273115China

Natural gas hydrate is an energy resource for methane that has a carbon quantity twice more than all traditional fossil fuels combined.However,their practical application in the field has been limited due to the challenges of long-term preparation,high costs and associated risks.Experimental studies,on the other hand,offer a safe and cost-effective means of exploring the mechanisms of hydrate dissociation and optimizing exploitation conditions.Gas hydrate decomposition is a complicated process along with intrinsic kinetics,mass transfer and heat transfer,which are the influencing factors for hydrate decomposition rate.The identification of the rate-limiting factor for hydrate dissociation during depressurization varies with the scale of the reservoir,making it challenging to extrapolate findings from laboratory experiments to the actual exploitation.This review aims to summarize current knowledge of investigations on hydrate decomposition on the subject of the research scale(core scale,middle scale,large scale and field tests)and to analyze determining factors for decomposition rate,considering the various research scales and their associated influencing factors.

关键词： Gas hydrate Rate-limiting factors Research scale depressurization Decomposition

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Numerical Simulation on Production Trials by Using depressurization for Typical Marine Hydrate Reservoirs:Well Type and Formation Dip

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Journal of Ocean University of China 2024年第3期23卷 661-675页

作者： QIN Fanfan SUN Jiaxin GU Yuhang CAO Xinxin MAO Peixiao NING Fulong JIANG Guosheng National Center for International Research on Deep Earth Drilling and Resource Development Faculty of EngineeringChina University of GeosciencesWuhan 430074China Laboratory for Marine Mineral Resources Qingdao National Laboratory for Marine Science and TechnologyQingdao 266237China

Natural gas hydrate has huge reserves and is widely distributed in marine environment.Its commercial development is of great significance for alleviating the contradiction between energy supply and demand.As an efficient research method,numerical simulation can provide valuable insights for the design and optimization of hydrate development.However,most of the current production models simplify the reservoir as a two-dimensional(2D)horizontal layered model,often ignoring the impact of formation dip angle.To improve the accuracy of production prediction and provide theoretical support for the optimization of production well design,two three-dimensional(3D)geological models with different dip angles based on the geological data from two typical sites are constructed.The vertical well,horizontal well and multilateral wells are deployed in these reservoirs with different permeabilities to perform production trial,and the sensitivity analysis of dip angles is also carried out.The short-term production behaviors in high and low permeability reservoirs with different dip angles are exhibited.The simulation results show that 1)the gas and water production behaviors for different well types in the two typical reservoirs show obviously different variation laws when the short-term depressurization is conducted in the inclined formation;2)the inclined formation will reduce the gas production and increase the water extraction,and the phenomena becomes pronounced as the dip angle increases,particularly in the low-permeability reservoirs;3)and the impact of formation dip on hydrate recovery does not change significantly with the variation of well type.

关键词： natural gas hydrate inclined formation depressurization production well type

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Numerical Investigation of Combined Production of Natural Gas Hydrate and Conventional Gas

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Fluid Dynamics & Materials Processing 2024年第3期20卷 505-523页

作者： Hongzhi Xu Jian Wang Shuxia Li Fengrui Zhao Chengwen Wang Yang Guo School of Petroleum Engineering China University of Petroleum(East China)Qingdao266580China CPOE Research Institute of Engineering Technology Tianjin300451China CNPC Offshore Engineering Company Limited Beijing100028China

Natural gas hydrate(NGH)is generally produced and accumulated together with the underlying conventional gas.Therefore,optimizing the production technology of these two gases should be seen as a relevant way to effectively reduce the exploitation cost of the gas hydrate.In this study,three types of models accounting for the coexistence of these gases are considered.Type A considers the upper hydrate-bearing layer(HBL)adjacent to the lower conventional gas layer(CGL);with the Type B a permeable interlayer exists between the upper HBL and the lower CGL;with the type C there is an impermeable interlayer between the upper HBL and the lower CGL.The production performances associated with the above three models are calculated under different conditions,including only a depressurized HBL(only HBL DP);only a depressurized CGL(only CGL DP);and both the HBL and the CGL being depressurized(HBL+CGL DP).The results show that for Type A and Type B coexistence accumulation models,when only HBL or CGL is depressurized,the gas from the other layer will flow into the production layer due to the pressure difference between the two layers.In the coexistence accumulation model of type C,the cumulative gas production is much lower than that of Type A and Type B,regardless of whether only HBL DP,only CGL DP,or HBL+CGL DP are considered.This indicates that the impermeable interlayer restricts the cross-flow of gas between HBL and CGL.For three different coexistence accumulation models,CGL DP has the largest gas-to-water ratio.

关键词： Natural gas hydrate conventional gas coexistence accumulation depressurization combined production

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Experimental study on sand production and coupling response of silty hydrate reservoir with different contents of fine clay during depressurization

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Petroleum 2023年第1期9卷 72-82页

作者： Xiangyu Fang Dianheng Yang Fulong Ning Linjie Wang Zhichao Liu Yanjiang Yu Wenwei Xie Hongfeng Lu Yanlong Li Meng Xu Faculty of Engineering China University of GeosciencesWuhan430074China Anhui Nuclear Exploration Technology Central Institute Wuhu241000China National Center for International Research on Deep Earth Drilling and Resource Development China University of GeosciencesWuhan430074China MLR Key Laboratory of Marine Mineral Resources Guangzhou Marine Geological SurveyGuangzhou510075China Laboratory for Marine Mineral Resources Qingdao National Laboratory for Marine Science and TechnologyQingdao266071China

To further understand the characteristics of clay and sand production(hereafter collectively referred to as sand production)and to provide optimization designs of sand control schemes are critical for gas production from clayey silt natural gas hydrate reservoirs in the South China Sea.Thus,gas-water-sand production behavoirs and coupling reservoir subsidence characteristics before,during,and after hydrate dissociation of the clayey silt hydrate reservoirs with different clay contents(5%,10%,15%,20%,25%,and 30%)have been studied through a self-developed experimental system.The results show that with the increase of clay content,the total mass of sand production first increases and then decreases,and it reaches maximum when the clayey content is 20%.The sand production is the lowest before hydrate dissociation and increases significantly during hydrate dissociation,which mainly occurs in the high-speed gas and water production stage at the beginning of hydrate dissociation.After hydrate dissociation,the sand production decreases significantly.During the whole depressurization process,the clay and free sand particles generally move to the sand outlet due to the fluid driving force and overlying stress extrusion.However,for conditions of high clay contents,those particles fail to pass through the sand control screen and gradually accumulate and block the screen by forming a mud cake,which greatly reduce the permeability of the screen and limite sand production as well as gas and water production.Our research lays a foundation for sand production prediction and sand control scheme selection during gas recovery from clayey silty hydrate reservoirs that greatly need to consider a balance between sand control and gas productivity.

关键词： Natural gas hydrate Clayey silt reservoir Clay content depressurization Sand production Sand control

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Influences of pore fluid on gas production from hydrate-bearing reservoir by depressurization

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Petroleum Science 2023年第2期20卷 1238-1246页

作者： Yi-Fei Sun Bo-Jian Cao Hong-Nan Chen Yin-Long Liu Jin-Rong Zhong Liang-Liang Ren Guang-Jin Chen Chang-Yu Sun Dao-Yi Chen State Key Laboratory of Heavy Oil Processing China University of PetroleumBeijing 102249China Division of Ocean Science and Technology Tsinghua Shenzhen International Graduate SchoolTsinghua UniversityShenzhenGuangdong 518055China School of Chemistry and Food Engineering Changsha University of Science&TechnologyChangshaHunan 410114China Oilfield Chemicals R&D Institute COSLHebei 065201China

In addition to the temperature and pressure conditions,the pore fluid composition and migration behavior are also crucial to control hydrate decomposition in the exploitation process.In this work,to investigate the effects of these factors,a series of depressurization experiments were carried out in a visible one-dimensional reactor,using hydrate reservoir samples with water saturations ranging from 20%to 65%.The results showed a linear relationship between gas production rates and gas saturations of the reservoir,suggesting that a larger gas-phase space was conducive to hydrate decomposition and gas outflow.Therefore,the rapid water production in the early stage of hydrate exploitation could release more gas-phase space in the water-rich reservoir,which in turn improved the gas production efficiency.Meanwhile,the spatiotemporal evolution of pore fluids could lead to partial accelerated decomposition or secondary formation of hydrates.In the unsealed reservoir,the peripheral water infiltration kept reservoir at a high water saturation,which hindered the overall production process and caused higher water production.Importantly,depressurization assisted with the N2 sweep could displace the pore water rapidly.According to the results,it is recommended that using the short-term N2 sweep as an auxiliary means in the early stage of depressurization to expand the gas-phase space in order to achieve the highest production efficiency.

关键词： CH4 hydrate Water saturation depressurization Gas-phase space N2 sweep

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Dissociation characteristics of methane hydrate using depressurization combined with thermal stimulation

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Chinese Journal of Chemical Engineering 2019年第9期27卷 2089-2098页

作者： Mingjun Yang Zhanquan Ma Yi Gao Lanlan Jiang Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education Dalian University of Technology

Methane hydrate is considered as a potential energy source in the future due to its abundant reserves and high energy density.To investigate the influence of initial hydrate saturation,production pressure,and the temperature of thermal stimulation on gas production rate and cumulative gas production percentage,we conducted the methane hydrate dissociation experiments using depressurization,thermal stimulation and a combination of two methods in this study.It is found that when the gas production pressures are the same,the higher the hydrate initial saturation,the greater change in hydrate reservoir temperature.Therefore,it is easier to appear the phenomenon of icing and hydrate reformation when the hydrate saturation is higher.For example,the reservoir temperature dropped to below zero in depressurization process when the hydrate saturation was about 37%.However,the same phenomenon didn’t appear as the saturation was about 12%.This may be due to more free gas in the reservoir with hydrate saturated of 37%.We also find that the temperature variation of reservoir can be reduced effectively by combination of depressurization and thermal stimulation method.And the average gas production rate is highest with combined method in the experiments.When the pressure of gas production is 2 MPa,compared with depressurization,the average of gas production can increase 54%when the combined method is used.The efficiency of gas production is very low when thermal stimulation was used alone.When the temperature of thermal stimulation is 11℃,the average rate of gas production in the experiment of thermal stimulation is less than 1/3 of that in the experiment of the combined method.

关键词： Methane hydrate depressurization Thermal stimulation Dissociation characteristics

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Investigation of the methane hydrate surface area during depressurization-induced dissociation in hydrate-bearing porous media

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Chinese Journal of Chemical Engineering 2021年第4期34卷 324-334页

作者： Xuke Ruan Xiao-Sen Li Guangzhou Institute of Energy Conversion Chinese Academy of SciencesGuangzhou 510640China CAS Key Laboratory of Gas Hydrate Guangzhou 510640China

The surface area of hydrate during dissociation in porous media is essentially important for the kinetics of hydrate dissociation.In this study,the methane hydrate surface area was investigated by the comparison results of experiments and numerical simulations during hydrate decomposition in porous media.The experiments of methane hydrate depressurizationinduced dissociation were performed in a 1D high pressure cell filled with glass beads,an improved and valid 1D corescale numerical model was developed to simulate gas production.Two conceptual models for hydrate dissociation surface area were proposed based on the morphology of hydrate in porous media,which formed the functional form of the hydrate dissociation surface area with porosity,hydrate saturation and the average radius of sand sediment particles.With the establishment of numerical model for depressurizationinduced hydrate dissociation in porous media,the cumulative gas productions were modeling and compared with the experimental data at the different hydrate saturations.The results indicated that the proposed prediction equations are valid for the hydrate dissociation surface area,and the graincoating surface area model performs well at lower hydrate saturation for hydrate dissociation simulation,whereas at higher hydrate saturation,the hydrate dissociation simulation from the porefilling surface area model is more reasonable.Finally,the sensitivity analysis showed that the hydrate dissociation surface area has a significant impact on the cumulative gas production.

关键词： Surface area Methane hydrate Hydrate dissociation Hydrate morphology depressurization

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HYDRODYNAMIC CHARACTERISTICS OF THE PROCESS OF depressurization OF SATURATED WATER

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Chinese Journal of Chemical Engineering 1994年第4期2卷 28-35页

作者：王立新欧阳藩 State Key Lab of Biochemical Eng Inst of Chemical Metallurgy Academia Sinica Beijing 100080 China China

Experiments were carried out to find the effects of dissolved gas pressure,liquid flow rateand nozzle geometry on the bubble generation when saturated water was depressurized through anozzle.A new method,high speed camera system was developed to measure the generated microbubblesdynamically.On the basis of the laws of ideal gas and solution,theoretical generated gas flow ratewas deduced,while the Smoluchowski′s equation was applied to describe the kinetics of bubblenucleation.It was found that the size distribution of nucleated bubbles was of skewed distribution.An explanation to this phenomenon was made and the Gamma function distribution was employedfor mathematical simulation.The results show good agreement between the experimental data and thepredictions by proposed model.

关键词： bubble generation bubble size distribution depressurization of saturated water

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The simulation of gas production from oceanic gas hydrate reservoir by the combination of ocean surface warm water flooding with depressurization

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Acta Mechanica Sinica 2012年第5期28卷 1287-1295页

作者： Hao Yang Yu-Hu Bai Qing-Ping Li Xinxing Heavy Industries Corporation Limited China National Offshore Oil Corporation Research Institute

A new method is proposed to produce gas from oceanic gas hydrate reservoir by combining the ocean surface warm water flooding with depressurization which can efficiently utilize the synthetic effects of thermal, salt and depressurization on gas hydrate dissociation. The method has the advantage of high efficiency, low cost and enhanced safety. Based on the proposed conceptual method, the physical and mathematical models are established, in which the effects of the flow of multiphase fluid, the kinetic process of hydrate dissociation, the endothermic process of hydrate dissociation, ice-water phase equilibrium, salt inhibition, dispersion, convection and conduction on the hydrate disso- ciation and gas and water production are considered. The gas and water rates, formation pressure for the combination method are compared with that of the single depressurization, which is referred to the method in which only depres- surization is used. The results show that the combination method can remedy the deficiency of individual producing methods. It has the advantage of longer stable period of high gas rate than the single depressurization. It can also reduce the geologic hazard caused by the formation defor- mation due to the maintaining of the formation pressure by injected ocean warm water.

关键词： Gas hydrate reservoir Ocean surface warmwater flooding depressurization Numerical simulation Combination exploitation

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