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defect promoted photothermoelectric effect in densely aligned zno nanorod arrays for self-powered position-sensitive photodetection

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Journal of Materiomics 2022年第3期8卷 693-701页

作者： Xinxin Du Weiliang Tian Ziqi Zhang Bin Hui Jiahui Pan Jianhua Sun Kewei Zhang State Key Laboratory of Bio-Fibers and Eco-Textiles Collaborative Innovation Center for Marine Biomass FibersMaterials and Textiles of Shandong ProvinceCollege of Materials Science and EngineeringInstitute of Marine Biobased MaterialsQingdao UniversityQingdao266071China Key Laboratory of Chemical Engineering in South Xinjiang College of Life ScienceTarim UniversityAlar843300China Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification Technology Guangxi UniversityNanning530004China

Sustainable light energy from ambient environment has attracted particular attention to meet the evergrowing need of small-scale *** modulation of intercorrelated thermal and electronic transport is one of the crucial aspects for reliable photothermoelectric ***,a defectpromoted photothermoelectric effect is demonstrated in densely aligned zno nanorod array with rich lattice *** defect-rich zno device delivers high electrical conductivity and large Seebeck coefficient to enable significant improvement of photothermoelectric energy conversion and self-powered *** position sensitivity reaches approximately 0.19 mV mm^(-1),and the temperature gradient induced electric field makes up for the suppression in the photothermoelectric *** synergism between intrinsic defects and extra temperature field plays an important role in promoting the photothermoelectric properties of dense zno nanorod *** study is interesting for interpreting the thermo-phototronic phenomena as well as demonstrating the possibility of defect engineering and phonon engineering to enable highly efficient light energy scavenging and self-powered photodetection.

关键词： defect-rich zno Photodetectors Light energy Photothermoelectric Self-powered

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