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A review on 2D MoS_(2) cocatalysts in photocatalytic H_(2) production

Journal of Materials Science & Technology 2020年第21期56卷 89-121页

作者： Zizhan Liang Rongchen Shen Yun Hau Ng Peng Zhang Quanjun Xiang Xin Li Key Laboratory of Energy Plants Resource and Utilization Ministry of Agriculture and Rural AffairsCollege of Forestry and Landscape ArchitectureSouth China Agricultural UniversityGuangzhou510642China School of Energy and Environment City University of Hong KongHong KongChina State Center for International Cooperation on Designer Low-Carbon&Environmental Materials(CDLCEM) School of Materials Science and EngineeringZhengzhou UniversityZhengzhou450001China State Key Laboratory of Electronic Thin Film and Integrated Devices University of Electronic Science and Technology of ChinaChengdu610054China

Owing to their unique physicochemical,optical and electrical properties,two-dimensional(2D)MoS_(2) cocatalysts have been widely applied in designing and developing highly efficient composite photocatalysts for hydrogen generation under suitable light *** this review,we first elaborated on the fundamental aspects of 2D MoS_(2) cocatalysts to include the structural design principles,synthesis strategies,strengths and ***,we thoroughly highlighted and discussed the modification strategies of 2D MoS_(2) H2-evolution cocatalysts,including doping heteroatoms(***,non-metals,and co-doping),designing interfacial coupling morphologies,controlling the physical properties(***,size,structural defects or pores),exposing the reactive facets or edge sites,constructing cocatalyst heterojunctions,engineering the interfacial bonds and confinement *** the future,the forefront challenges in understanding and in precise controlling of the active sites at molecular level or atomic level should be carefully studied,while various potential mechanisms of photogenerated-electrons interactions should be *** applications of MoS_(2) cocatalyst in the overall water splitting are also *** review may offer new inspiration for designing and constructing novel and efficient MoS_(2)-based composite photocatalysts for highly efficient photocatalytic hydrogen evolution.

关键词： 2D MoS2 cocatalysts Photocatalytic H2 production Heteroatom doping cocatalyst heterojunctions Charge dynamics

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