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Advances in Noble Metal-Decorated Metal Oxide Nanomaterials for Chemiresistive Gas Sensors:Overview

纳微快报：英文版 2023年第6期15卷 353-427页

作者： Li‑Yuan Zhu Lang‑Xi Ou Li‑Wen Mao Xue‑Yan Wu Yi‑Ping Liu Hong‑Liang Lu State Key Laboratory of ASIC and System Shanghai Institute of Intelligent Electronics and SystemsSchool of MicroelectronicsFudan UniversityShanghai 200433People’s Republic of China School of Opto‑Electronic Information and Computer Engineering University of Shanghai for Science and TechnologyShanghai 200093People’s Republic of China State Key Laboratory of Metal Matrix Composites School of Material Science and EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Highly sensitive gas sensors with remarkably low detection limits are attractive for diverse practical application fields including real-time environmental monitoring,exhaled breath diagnosis,and food freshness analysis.Among various chemiresistive sensing materials,noble metal-decorated semiconducting metal oxides(SMOs)have currently aroused extensive attention by virtue of the unique electronic and catalytic properties of noble metals.This review highlights the research progress on the designs and applications of different noble metal-decorated SMOs with diverse nanostructures(e.g.,nanoparticles,nanowires,nanorods,nanosheets,nanoflowers,and microspheres)for high-performance gas sensors with higher response,faster response/recovery speed,lower operating temperature,and ultra-low detection limits.The key topics include Pt,Pd,Au,other noble metals(e.g.,Ag,Ru,and Rh.),and bimetals-decorated SMOs containing ZnO,SnO_(2),WO_(3),other SMOs(e.g.,In_(2)O_(3),Fe_(2)O_(3),and CuO),and heterostructured SMOs.In addition to conventional devices,the innovative applications like photo-assisted room temperature gas sensors and mechanically flexible smart wearable devices are also discussed.Moreover,the relevant mechanisms for the sensing performance improvement caused by noble metal decoration,including the electronic sensitization effect and the Chemical sensitization effect,have also been summarized in detail.Finally,major challenges and future perspectives towards noble metal-decorated SMOs-based chemiresistive gas sensors are proposed.

关键词： Noble metal Bimetal Semiconducting metal oxide Chemiresistive gas sensor Electronic sensitization Chemical sensitization

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chemical sensitization OF TABULAR－GRAIN EMUL－SIONS IN THE PRESENCE OF SENSITIZING DYE

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影像科学与光化学 1995年第3期 277-285页

作者： WEIDE VICTOR YANG(3M Printing & Publishing Systems Division,St.Paul,55144,USA)

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ＣＨＥＭＩＣＡＬＳＥＮＳＩＴＩＺＡＴＩＯＮＯＦＴＡＢＵＬＡＲ－ＧＲＡＩＮＥＭＵＬ－ＳＩＯＮＳＩＮＴＨＥＰＲＥＳＥＮＣＥＯＦＳＥＮＳＩＴＩＺＩＮＧＤＹＥ￥ＣＨＥＭＩＣＡＬＳＥＮＳＩＴＩＺＡＴＩＯＮＯＦＴＡＢＵＬＡＲ－ＧＲＡＩＮＥＭＵＬ－ＳＩＯＮＳＩＮＴ...

关键词： AgX silver halide T-grain emulsion Chemical sensitization

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Improved sensing performance of WO_(3) nanoparticles decorated with Ag and Pt nanoparticles

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Rare Metals 2021年第6期40卷 1642-1650页

作者： Dong-Liang Feng Zheng-You Zhu Ling-Ling Du Xia-Xia Xing Chen Wang Jian Chen Yong-Tao Tian Da-Chi Yang Tianjin Key Laboratory of Optoelectronic Sensor and Sensing Network Technology and Department of ElectronicsCollege of Electronic Information and Optical EngineeringNankai UniversityTianjin 300350China School of Physics and Engineering and Key Laboratory of Materials Physics Ministry of EducationZhengzhou UniversityZhengzhou 450001China

Gas sensors built with metal oxide semiconductors have attracted tremendous attention due to the growing demand for the detection of inflammable,explosive and toxic gases.Herein,to improve the sensing response,WO_(3) nanoparticles decorated with Ag and Pt bimetals(Ag and Pt/WO_(3) NPs)have been developed via combined hydrolysis and hydrothermal strategies.Such sensors prototypes show high response to acetone(Ra/Rg=250@100×10^(-6),140℃),which is 6.1 fold as high as that of the pristine WO_(3) NPs(Ra/Rg=41@100×10^(-6),140℃).Moreover,the recovery time of Ag and Pt/WO_(3) NPs was reduced from 138 to 13 s compared with that of the pristine WO_(3) NPs.The improved acetone sensing performance may be attributed to that the chemical and electronic sensitization of Ag and Pt to WO_(3) NPs increases adsorbed oxygen species,speeds up the reaction and thus boosts the sensing response.Our strategy that decoration of dual precious metals onto WO_(3) NPs improves the acetone sensing performance may be applied to the gas sensors of other sensing materials.

关键词： WO_(3)nanoparticles Ag and Pt bimetals Acetone sensing Chemical sensitization Recovery time

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