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Recent advances in solid-state metal-air batteries

Carbon Energy 2023年第2期5卷 148-170页

作者： Qi Sun Lei Dai Tingting Luo Ling Wang Feng Liang Shan Liu School of Chemical Engineering North China University of Science and TechnologyTangshanChina The National Engineering Center for Vacuum Metallurgy&Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunmingChina

Solid-state metal-air batteries have emerged as a research hotspot due to their high energy density and high safety.Moreover,side reactions caused by infiltrated gases(O_(2),H_(2)O,or CO_(2))and safety issues caused by liquid electrolyte leakage will be eliminated radically.However,the solid-state metal–air battery is still in its infancy,and many thorny problems still need to be solved,such as the large resistance of the metal/electrolyte interface and catalyst design.This review will summarize some important progress and key issues for solid-state metal-air batteries,especially the lithium-,sodium-,and zinc-based metal-air batteries,clarify some core issues,and forecast the future direction of the solid-state metal-air batteries.

关键词： cathode structure interface stability metal anode metal-air batteries solid electrolyte

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Recent advances in cathodes for all-solid-state lithium-sulfur batteries

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Chinese Chemical Letters 2023年第7期34卷 58-69页

作者： Shengbo Yang Bo Wang Qiang Lv Nan Zhang Zekun Zhang Yutong Jing Jinbo Li Rui Chen Bochen Wu Pengfei Xu Dianlong Wang MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage State Key Laboratory of Urban Water Resource and EnvironmentSchool of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001China

Lithium-sulfur(Li-S)batteries have been regarded as the candidate for the next-generation energy storage system due to the high theoretical specific capacity(1675 m Ah/g), energy density(2600 Wh/kg)and the abundance of elemental sulfur, but the application of Li-S batteries is impeded by a series of problems. Recently, all-solid-state Li-S batteries(ASSLSBs) have drawn great attention because many drawbacks such as safety issues caused by metallic lithium anodes and organic liquid electrolytes can be overcome through the use of solid-state electrolytes(SEs). However, not only the problems brought by sulfur cathodes still exist, but more trouble arouses from the interfaces between SEs and cathodes, hampering the practical application of ASSLSBs. Therefore, in order to deal with the problems, enormous endeavors have been done on ASSLSB cathodes during the past few decades, including engineering of cathode active materials, cathode host materials, cathode binder materials and cathode structures. In this review, the electrochemical mechanism and existing problems of ASSLSBs are briefly introduced. Subsequently, the strategies for developing cathode materials and designing cathode structures are presented. Then there follows a brief discussion of SE problems and expectations, and finally, the challenges and perspectives of ASSLSBs are summarized.

关键词： All-solid-state Li-S battery cathode active material cathode host material cathode structure Solid-state electrolyte

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