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Frontiers of Chemical Science and Engineering 2024年第3期18卷 1-12页

作者： Li Zhao Xinru Liu Zihao Ye Bin Hu Haoyu Wang Ji Liu Bing Zhang Qiang Lu National Engineering Research Center of New Energy Power Generation North China Electric Power UniversityBeijing102206China

The composition of biomass pyrolysis gas is complex,and the selective separation of its components is crucial for its further ***-incorporated nitrogen-doped materials exhibit enormous potential,whereas the relevant adsorption mechanism is still ***,16 metal-incorporated nitrogen-doped carbon materials were designed based on the density functional theory calculation,and the adsorption mechanism of pyrolysis gas components H2,CO,CO_(2),CH_(4),and C2H6 was *** results indicate that metal-incorporated nitrogen-doped carbon materials generally have better adsorption effects on CO and CO_(2)than on H_(2),CH_(4),and C_(2)H_(6).Transition metal Mo-and alkaline earth metal Mg-and Ca-incorporated nitrogen-doped carbon materials show the potential to separate CO and CO_(2).The mixed adsorption results of CO_(2)and CO further indicate that when the CO_(2)ratio is significantly higher than that of CO,the saturated adsorption of CO_(2)will precede that of ***,the three metal-incorporated nitrogen-doped carbon materials can selectively separate CO_(2),and the alkaline earth metal Mg-incorporated nitrogen-doped carbon material has the best *** study provides theoretical guidance for the design of carbon capture materials and lays the foundation for the efficient utilization of biomass pyrolysis gas.

关键词： CO_(2)capture biomass pyrolysis gas selective adsorption carbon materials first-principles

Electrospinning-derived functional carbon-based materials for energy conversion and storage

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Chinese Chemical Letters 2024年第6期35卷 3-13页

作者： Xinyu Ren Hong Liu Jingang Wang Jiayuan Yu Institute for Advanced Interdisciplinary Research(iAIR) School of Chemistry and Chemical EngineeringUniversity of JinanJi’nan 250022China State Key Laboratory of Crystal materials Shandong UniversityJi’nan 250100China

The over-exploitation of fossil fuel energy has brought about serious environmental *** would be of great significance to construct efficient energy conversion and storage system to maximize utilize renewable energy,which contributes to reducing environmental *** the past few years,in terms of electrocatalysis and energy storage,carbon fiber materials show great advantages due to its outstanding electrical conductivity,good flexibility and mechanical *** a simple and low-cost technique,electrospinning can be employed to prepare various *** is noted that the functional fiber materials with different special structure and composition can be obtained for energy conversion and storage by combining electrospinning with other *** this paper,the structural design,controllable synthesis and multifunctional applications of electrospinning-derived functional carbon-based materials(EFCMs)is ***,we briefly introduce the history,basic principle and typical equipment of *** we discuss the strategies for preparing EFCMs with different structures and composition in *** addition,we show recently the application of advanced EFCMs in energy conversion and storage,such as nitrogen species reduction reaction,CO_(2) reduction reaction,oxygen reduction reaction,water-splitting,supercapacitors and ion *** the end,we propose some perspectives on the future development direction of EFCMs.

关键词： Electrospinning carbon materials Functional fiber Energy conversion Energy storage Electrocatalysis

carbon materials:The burgeoning promise in electronics

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International Journal of Minerals,Metallurgy and materials 2022年第3期29卷 404-423页

作者： Yuting Zheng Junjun Wei Jinlong Liu Liangxian Chen Kang An Xiaotong Zhang Haitao Ye Xiaoping Ouyang Chengming Li Institute for Advanced materials and Technology(IAMT State Key Laboratory for Advanced Metals and MaterialUniversity of Science and Technology BeijingBeijing 100083China Shunde Graduate School University of Science and Technology BeijingFoshan 528399China School of Computer and Communication Engineering University of Science and Technology BeijingBeijing 100083China School of Engineering University of LeicesterLeicester LE17RHUnited Kingdom School of materials Science and Engineering Xiangtan UniversityXiangtan 411105China

Current electronic technology based on silicon is approaching its physical and scientific limits. carbon-based devices have numer- ous advantages for next generation electronics (e.g., fast speed, low power consumption and simple process), that when combined with the unique nature of the versatile allotropes of carbon elements, are creating an electronics revolution. carbon electronics are greatly advancing with new preparations and sophisticated designs. In this perspective, representatives with various dimensions, e.g., carbon nanotubes, graphene, bulk diamond, and their extraordinary performance, are reviewed. The associated state-of-the-art devices and composite hybrid all-carbon structures are also emphasized to reveal their potential in the electronics field. Advances in commercial production have improved the cost effi-ciency, material quality, and device design, accelerating the promise of carbon materials.

关键词： carbon materials nanotube graphene diamond electronic devices

carbon materials Reinforced Aluminum Composites:A Review

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Acta Metallurgica Sinica(English Letters) 2014年第5期27卷 775-786页

作者： Yu Huang Qiubao Ouyang Di Zhang Jing Zhu Ruixiang Li Hong Yu State Key Laboratory of Metal Matrix Composites Shanghai Jiao Tong University Shanghai Composites Science and Technique Co. Ltd Shanghai Key Laboratory of Spacecraft Mechanism

carbon materials, including carbon fibers, graphite, diamond, carbon foams, carbon nanotubes, and graphene, are attractive reinforcements for aluminum matrix composites due to their excellent mechanical and/or physical properties as well as light weight. carbon materials reinforced aluminum （C/Al） composites are promising materials in many areas such as aerospace, thermal management, and automobile. However, there are still some challenging problems that need to be resolved, such as interfacial reactions, low wettability, and anisotropic properties. These problems have limited the use of these composites. This review mainly focuses on the categories, fabrication processes, existing problems and solutions, coatings and interfaces, challenges and opportunities of C/Al composites so as to provide a useful reference for future research.

关键词： carbon materials Aluminum composites Fabrication Interface Coatings

carbon materials in Perovskite Solar Cells: Prospects and Future Challenges

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能源与环境材料（英文） 2019年第2期2卷 107-118页

作者： Victoria Ferguson S.Ravi P.Silva Wei Zhang Advanced Technology Institute(ATI) University of SurreyGU27XHUK

Metal halide perovskite solar cells are emerging candidates for nextgeneration thin-film photovoltaic devices with the potential for extremely low fabrication cost and high power conversion *** solar cells have demonstrated a rapid development in device performance over the last decade,from an initial 3.81%to a most recently certified 24.2%,though the challenges of long-term stability and lead toxicity still *** materials,ranging from zero-dimensional carbon quantum dots to threedimensional carbon black materials,are promising candidates for the enhancement of both efficiency and stability of perovskite solar cells,offering unique advantages for incorporation into various device *** this review article,we present a concise overview of important and exciting advancements of perovskite solar cells that incorporate different dimensions of carbon material in their device architectures in an effort to simultaneously improve device performance and long-term *** also discuss the major advantages and potential challenges of each technique that has been developed in the most recent ***,we outline the future opportunities toward more efficient and stable perovskite solar cells utilizing carbon materials.

关键词： carbon materials long-term stability metal halide perovskite photovoltaics

carbon materials in electrocatalytic oxidation systems for the treatment of organic pollutants in wastewater:A review

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carbon Resources Conversion 2023年第4期6卷 262-273页

作者： Xintong Duan Dezhang Ren Shichun Wang Mengjie Zhang Yaguang Sun Shujing Sun Zhibao Huo Nahui Zhang College of Marine Ecology and Environment Shanghai Ocean University999 Huchenghuan RoadShanghai 201306China The Key Laboratory of Inorganic Molecule-Based Chemistry of Liaoning Province Shenyang University of Chemical TechnologyShenyang 110142China Liaoning Ecological Environmental Monitoring Center Shenyang 110165China

carbon materials are widely used as catalysts in electrocatalytic oxidative(EO)degradation of wastewater due to their large specific surface area and low *** materials can also be used as catalyst carriers for EO reactions due to their ease of functionalization with other heteroatoms and metals/metal *** improve the catalytic activity and current efficiency of carbon materials,modifying the structural and physicochemical properties of conventional carbon materials are common improvement *** review briefly outlines the recent research progress of carbon materials in EO for organic pollutants *** also discusses the modification strategies and corresponding electrocatalytic properties of various carbon materials(carbon nanomaterials and porous carbon materials),and explores the EO ***,some summaries of the remaining challenges and future developments of carbon materials in the field of electrocatalysis are given.

关键词： carbon materials Electrocatalytic oxidation Industrial wastewater Mechanism

carbon materials for stable Li metal anodes: Challenges, solutions, and outlook

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carbon Energy 2021年第6期3卷 957-975页

作者： Qiongqiong Lu Yulin Jie Xiangqi Meng Ahmad Omar Daria Mikhailova Ruiguo Cao Shuhong Jiao Yan Lu Yaolin Xu Leibniz Institute for Solid State and materials Research(IFW)Dresden e.V. DresdenGermany Hefei National Laboratory for Physical Sciences at the Microscale CAS Key Laboratory of Materials for Energy ConversionDepartment of Materials Science and EngineeringUniversity of Science and Technology of ChinaHefeiChina Department of Electrochemical Energy Storage Helmholtz-Zentrum Berlin für Materialien und Energie(HZB)BerlinGermany Institute of Chemistry University of PotsdamPotsdamGermany

Lithium(Li)metal is regarded as the ultimate anode for next-generation Li-ion batteries due to its highest specific capacity and lowest electrochemical ***,the Li metal anode has limitations,including virtually infinite volume change,nonuniform Li deposition,and an unstable electrode-electrolyte interface,which lead to rapid capacity degradation and poor cycling stability,significantly hindering its practical *** address these issues,intensive efforts have been devoted toward accommodating and guiding Li deposition as well as stabilizing the interface using various carbon materials,which have demonstrated excellent effectiveness,benefiting from their vast variety and excellent tunability of the structure-property *** review is intended as a guide through the fundamental challenges of Li metal anodes to the corresponding solutions utilizing carbon *** specific functionalities and mechanisms of carbon materials for stabilizing Li metal anodes in these solutions are discussed in *** from the stabilization of the Li metal anode in liquid electrolytes,attention has also been paid to the review of anode-free Li metal batteries and solid-state batteries enabled by strategies based on carbon ***,we have reviewed the unresolved challenges and presented our outlook on the implementation of carbon materials for stabilizing Li metal anodes in practical applications.

关键词： carbon materials interface engineering Li deposition regulation Li metal anode structure stabilization

carbon materials from melamine sponges for supercapacitors and lithium battery electrode materials: A review

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carbon Energy 2019年第2期1卷 253-275页

作者： Yanying Shi Guijing Liu Rencheng Jin Hui Xu Qingyao Wang Shanmin Gao School of Chemistry and materials Science Ludong UniversityYantaiChina

With the increasing energy demand together with the deteriorating environment and decreasing fossil fuel resources,the development of highly efficient energy conversion and storage devices is one of the key challenges of both fundamental and applied research in energy *** sponges(MS)with low density,high nitrogen content,and high porosity have been used to design and obtain three‐dimensional porous carbon electrode *** importantly,they are inexpensive,environment‐friendly,and easy to *** have been many reports on the modification of carbonized MS and MS‐based composites for supercapacitor and lithium battery electrode *** this paper,recent studies on the fabrication of electrode materials using MS as raw materials have been mainly reviewed,including carbonation,doping activation,and composite modification of MS,and expectations for the development of porous carbon materials for energy storage as a reference with excellent performance,environment‐friendliness,and long life.

关键词： activation carbon materials composites electrode materials melamine sponges

Catalytic wet air oxidation of phenol with functionalized carbon materials as catalysts:Reaction mechanism and pathway

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Journal of Environmental Sciences 2014年第8期26卷 1741-1749页

作者： Jianbing Wang Wantao Fu Xuwen He Shaoxia Yang Wanpeng Zhu School of Chemical and Environmental Engineering Beijing CampusChina University of Mining and Technology School of Environment Tsinghua University

The development of highly active carbon material catalysts in catalytic wet air oxidation（CWAO）has attracted a great deal of attention. In this study different carbon material catalysts（multi-walled carbon nanotubes,carbon fibers and graphite） were developed to enhance the CWAO of phenol in aqueous solution. The functionalized carbon materials exhibited excellent catalytic activity in the CWAO of phenol. After 60 min reaction,the removal of phenol was nearly100% over the functionalized multi-walled carbon,while it was only 14% over the purified multi-walled carbon under the same reaction conditions. Carboxylic acid groups introduced on the surface of the functionalized carbon materials play an important role in the catalytic activity in CWAO. They can promote the production of free radicals,which act as strong oxidants in CWAO. Based on the analysis of the intermediates produced in the CWAO reactions,a new reaction pathway for the CWAO of phenol was proposed in this study. There are some differences between the proposed reaction pathway and that reported in the literature. First,maleic acid is transformed directly into malonic acid. Second,acetic acid is oxidized into an unknown intermediate,which is then oxidized into CO2 and H2O. Finally,formic acid and oxalic acid can mutually interconvert when conditions are favorable.

关键词： Catalytic wet air oxidation Phenol carbon materials Radical Reaction pathway

Status and Opportunities of Zinc Ion Hybrid Capacitors: Focus on carbon materials, Current Collectors, and Separators

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纳微快报：英文版 2023年第6期15卷 73-111页

作者： Yanyan Wang Shirong Sun Xiaoliang Wu Hanfeng Liang Wenli Zhang College of Chemistry Chemical Engineering and Resource UtilizationNortheast Forestry University26 Hexing RoadHarbin 150040People’s Republic of China Guangdong Provincial Key Laboratory of Plant Resources Biorefinery School of Chemical Engineering and Light IndustryGuangdong University of Technology(GDUT)100 Waihuan Xi RoadPanyu DistrictGuangzhou 510006People’s Republic of China State Key Laboratory of Physical Chemistry of Solid Surfaces College of Chemistry and Chemical EngineeringXiamen UniversityXiamen 361005People’s Republic of China Jieyang Branch of Chemistry and Chemical Engineering Guangdong Laboratory(Rongjiang Laboratory) Jieyang 515200People’s Republic of China School of Advanced Manufacturing Guangdong University of Technology(GDUT)Jieyang 522000People’s Republic of China

Zinc ion hybrid capacitors(ZIHCs), which integrate the features of the high power of supercapacitors and the high energy of zinc ion batteries, are promising competitors in future electrochemical energy storage applications. carbon-based materials are deemed the competitive candidates for cathodes of ZIHC due to their cost-effectiveness, high electronic conductivity, chemical inertness, controllable surface states, and tunable pore architectures. In recent years, great research efforts have been devoted to further improving the energy density and cycling stability of ZIHCs. Reasonable modification and optimization of carbon-based materials offer a remedy for these challenges. In this review, the structural design, and electrochemical properties of carbon-based cathode materials with different dimensions, as well as the selection of compatible, robust current collectors and separators for ZIHCs are discussed. The challenges and prospects of ZIHCs are showcased to guide the innovative development of carbon-based cathode materials and the development of novel ZIHCs.

关键词： Zinc ion hybrid capacitors carbon materials carbon cathode Current collectors Separators