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Tandem electrocatalysis for co_(2) reduction to multi-carbons

Science China Chemistry 2024年第11期67卷 3631-3651页

作者： Xindi Li Tianxiang Yan Yichen Meng Zhanpeng Liang Tianying Zhang Haoyuan Chi Ziting Fan Yifan Jin Haoran Zhang Sheng Zhang Key Laboratory for Green Chemical Technology of Ministry of Education Collaborative Innovation Centre of Chemical Science and EngineeringSchool of Chemical Engineering and TechnologyTianjin UniversityTianjin 300072China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China Joint School of National University of Singapore and Tianjin University International Campus of Tianjin UniversityFuzhou 350207China

The rising co_(2) concentration in the atmosphere due to extensive use of fossil fuels has led to serious climate and environmental issues. One efficient solution is that co_(2) capture from industrial emissions followed its conversion into value-added chemicals driven by renewable energies. co_(2) electroreduction(co_(2) RR) features a green and sustainable fashion towards effective co_(2) conversion, but still suffers from low multi-carbon selectivity and yield. considering the pivotal role of co intermediate in C–C coupling to multi-carbon formation, tandem co_(2) RR systems with separated co generation and consumption components could facilitate the coupling between *co-based intermediates to energy-intensive multi-carbons by manipulating co diffusion and surface coverage. In this aspect, we comprehensively reviewed the design principles of tandem systems for co_(2) electroreduction reaction. The chemistry behind the C–C coupling regarding to their distribution and diffusion was initially introduced, which was followed by achievements on tandem architectures, from catalysts, electrodes to systems. Future directions and perspectives on advanced tandem system designs for co_(2) RR were discussed at the end. This review contributes to the understanding of structureperformance correlations in tandem catalysis and helps guide the effective collection of multi-carbons of high-yield and highselectivity.

关键词： electrocatalytic co_(2)reduction tandem electrocatalysis design co mass transfer model

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