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Numerical Study and Optimization of CZTS-Based Thin-Film Solar Cell Structure with Different Novel buffer-layer Materials Using SCAPS-1D Software

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Energy and Power Engineering 2024年第4期16卷 179-195页

作者： Md. Zamil Sultan Arman Shahriar Rony Tota Md. Nuralam Howlader Hasibul Haque Rodro Mahfuja Jannat Akhy Md. Abir Al Rashik Department of Electrical and Electronic Engineering Hajee Mohammad Danesh Science and Technology University Dinajpur Bangladesh

This study explored the performances of CZTS-based thin-film solar cell with three novel buffer layer materials ZnS, CdS, and CdZnS, as well as with variation in thickness of buffer and absorber-layer, doping concentrations of absorber-layer material and operating temperature. Our aims focused to identify the most optimal thin-film solar cell structure that offers high efficiency and lower toxicity which are desirable for sustainable and eco-friendly energy sources globally. SCAPS-1D, widely used software for modeling and simulating solar cells, has been used and solar cell fundamental performance parameters such as open-circuited voltage (), short-circuited current density (), fill-factor() and efficiency() have been optimized in this study. Based on our simulation results, it was found that CZTS solar cell with Cd0.4Zn0.6S as buffer-layer offers the most optimal combination of high efficiency and lower toxicity in comparison to other structure investigated in our study. Although the efficiency of Cd0.4Zn0.6S, ZnS and CdS are comparable, Cd0.4Zn0.6S is preferable to use as buffer-layer for its non-toxic property. In addition, evaluation of performance as a function of buffer-layer thickness for Cd0.4Zn0.6S, ZnS and CdS showed that optimum buffer-layer thickness for Cd0.4Zn0.6S was in the range from 50 to 150nm while ZnS offered only 50 – 75 nm. Furthermore, the temperature dependence performance parameters evaluation revealed that it is better to operate solar cell at temperature 290K for stable operation with optimum performances. This study would provide valuable insights into design and optimization of nanotechnology-based solar energy technology for minimizing global energy crisis and developing eco-friendly energy sources sustainable and simultaneously.

关键词： Thin-Film Solar Cell CZTS buffer-layer Renewable Energy Green-House Gases Efficiency

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The Magnetoresistance of Nanostructured Co-ZnO Films with ZnO buffer-layers

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Materials Sciences and Applications 2014年第14期5卷 996-1003页

作者： Xiaoli Li Long Cheng Long Cheng Yalei Wang Yan Gao Zhiyong Quan Xiufang Qin Harry J. Blythe Gillian A. Gehring Xiaohong Xu Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education School of Chemistry and Materials Science Shanxi Normal University Linfen China Department of Physics and Astronomy University of Sheffield Sheffield UK

Co-ZnO films were prepared on oxidised silicon by magnetron sputtering at room temperature both with and without a ZnO buffer-layer. The Co-ZnO films consisted of Co particles dispersed in a semiconductor matrix. The combination of a Co-ZnO layer and a ZnO buffer-layer has a higher magnetoresistance than the Co-ZnO layer alone on an insulating Si substrate. The causes of this effect were investigated using X-ray photoelectron spectroscopy, depth profiling using Auger electron spectroscopy and electrical resistance as well as measurements of the change in the saturation magnetisation, the field cooled- and zero field cooled-magnetisation. This work has shown clearly what criteria are needed to optimise the magnetoresistance and how these conditions may be met by adding a buffer-layer thus making granular films based on ZnO more suitable for applications as field sensors.

关键词： Magnetron Sputtering Magnetoresistance ZnO buffer-layer

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Self-catalyst synthesis of aligned ZnO nanorods by pulsed laser deposition

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Science China(Physics,Mechanics & Astronomy) 2009年第2期52卷 207-211页

作者： LEN Song-En Andy University of Maryland at College Park College Park Maryland USA

High-density well-aligned ZnO nanorods were successfully synthesized on ZnO-buffer-layer coated indium phosphide (InP) (100) substrates by a pulsed laser deposition (PLD) method. Scanning electron microscopy images show that the ZnO buffer layer formed uniform drip-like structure and ZnO nano- rods were well-oriented perpendicular to the substrate surface. The sharp diffraction peak observed at 34.46° in X-ray diffraction scanning pattern suggests that the ZnO nanorods exhibit a (002)-preferred orientation. The PL spectra of ZnO samples shows a strong near band edge emission centered at about 380 nm and a weak deep level emission centered at around 495 nm, and it demonstrates that the ZnO nanorods produced in this work have high optical quality, which sheds light on further applications for nanodevices.

关键词： ZnO nanorods buffer-layer self-catalyst pulsed laser deposition

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