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A Novel artificial neuron-like gas sensor Constructed from CuS Quantum Dots/Bi2S3 Nanosheets

Nano-Micro Letters 2022年第1期14卷 167-181页

作者： Xinwei Chen Tao Wang Jia Shi Wen Lv Yutong Han Min Zeng Jianhua Yang Nantao Hu Yanjie Su Hao Wei Zhihua Zhou Zhi Yang Yafei Zhang Key Laboratory of Thin Film and Microfabrication(Ministry of Education) Department of Micro/Nano ElectronicsSchool of Electronic Information and Electrical EngineeringShanghai Jiao Tong UniversityShanghai 200240People’s Republic of China

Real-time rapid detection of toxic gases at room temperature is particularly important for public health and environmental *** sensors based on conventional bulk materials often suffer from their poor surface-sensitive sites,leading to a very low gas adsorption ***,the charge transportation efficiency is usually inhibited by the low defect density of surface-sensitive area than that in the *** this work,a gas sensing structure model based on CuS quantum dots/Bi_(2)S_(3) nanosheets(CuS QDs/Bi_(2)S_(3) NSs)inspired by artificial neuron network is *** analysis by density functional calculation revealed that CuS QDs and Bi_(2)S_(3) NSs can be used as the main adsorption sites and charge transport pathways,***,the high-sensitivity sensing of NO_(2) can be realized by designing the artificial neuron-like *** experimental results showed that the CuS QDs with a size of about 8 nm are highly adsorbable,which can enhance the NO_(2) sensitivity due to the rich sensitive sites and quantum size *** Bi_(2)S_(3) NSs can be used as a charge transfer network channel to achieve efficient charge collection and *** neuron-like sensor that simulates biological smell shows a significantly enhanced response value(3.4),excellent responsiveness(18 s)and recovery rate(338 s),low theoretical detection limit of 78 ppb,and excellent selectivity for NO_(2).Furthermore,the developed wearable device can also realize the visual detection of NO2 through real-time signal changes.

关键词： artificial neuron-like gas sensor Heterostructure design Nitrogen dioxide detection Wearable device

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