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Ultra‑Stable Sodium‑Ion Battery Enabled by All‑Solid‑State Ferroelectric‑Engineered Composite Electrolytes

Nano-Micro Letters 2024年第11期16卷 704-717页

作者： Yumei Wang Zhongting Wang Xiaoyu Xu Sam Jin An Oh Jianguo Sun Feng Zheng Xiao Lu Chaohe Xu Binggong Yan Guangsheng Huang Li Lu College of Aerospace Engineering Chongqing UniversityChongqing 400044People’s Republic of China National University of Singapore(chongqing)research Institute Chongqing 401123People’s Republic of China College of Materials Science and Engineering Chongqing UniversityChongqing 400044People’s Republic of China Department of Mechanical Engineering National University of Singapore9 Engineering Drive 1Singapore 117575Singapore Fujian Key Laboratory of special Energy Manufacturing Xiamen Key Laboratory of Digital Vision MeasurementHuaqiao UniversityXiamen 361021People’s Republic of China

Symmetric Na-ion cells using the NASICON-structured electrodes could simplify the manufacturing process,reduce the cost,facilitate the recycling post-process,and thus attractive in the field of large-scale stationary energy ***,the long-term cycling performance of such batteries is usually *** investigation reveals the unavoidable side reactions between the NASICON-type Na_(3)V_(2)(PO_(4))_(3)(NVP)anode and the commercial liquid electrolyte,leading to serious capacity fading in the symmetric NVP//NVP *** resolve this issue,an all-solid-state composite electrolyte is used to replace the liquid electrolyte so that to overcome the side reaction and achieve high anode/electrolyte interfacial *** ferroelectric engineering could further improve the interfacial ion conduction,effectively reducing the electrode/electrolyte interfacial *** NVP//NVP cell using the ferroelectric-engineered composite electrolyte can achieve a capacity retention of 86.4%after 650 ***,the electrolyte can also be used to match the Prussianblue cathode NaxFeyFe(CN)_(6−z)·nH_(2)O(NFFCN).Outstanding long-term cycling stability has been obtained in the all-solid-state NVP//NFFCN cell over 9000 cycles at a current density of 500 mA g^(-1),with a fading rate as low as 0.005%per cycle.

关键词： Sodium-ion battery NVP anode All-solid-state Cyclic stability Ferroelectric

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Characterization of Domeless receptors and the role of Bd Domeless3 in anti-symbiont-like virus defense in Bactrocera dorsalis

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Journal of Integrative Agriculture 2024年第4期23卷 1274-1284页

作者： Wei Zhang Shaoyang Li Rong Li Jinzhi Niu Jinjun Wang Key Laboratory of Entomology and Pest Control Engineering College of Plant ProtectionSouthwest UniversityChongqing 400715China Key Laboratory of Agricultural Biosafety and Green Production of Upper Yangtze River Ministry of Education/International Joint Laboratory of China-Belgium on Sustainable Crop Pest ControlAcademy of Agricultural SciencesSouthwest UniversityChongqing 400715China

The Janus kinase/signal transducers and activators of transcription(JAK/STAT)signaling pathway play a pivotal role in innate *** invertebrates,Domeless receptors serve as the key upstream regulators of this *** our study on Bactrocera dorsalis,we identified three cytokine receptors:BdDomeless1,BdDomeless2,and *** receptor encompasses five fibronectin-type-III-like(FN III)extracellular domains and a transmembrane ***,these receptors exhibit the increased responsiveness to diverse pathogenic ***,only BdDomeless3 is upregulated during symbiont-like viral ***,silencing BdDomeless3 enhanced the infectivity of Bactrocera dorsalis cripavirus(BdCV)and *** picorna-like virus(BdPLV),underscoring BdDomeless3’s crucial role in antiviral defense of *** the suppression of Domeless3 expression,six antimicrobial peptide genes displayed decreased expression,potentially correlating with the rise in viral *** our knowledge,this is the first study identifying cytokine receptors associated with the JAK/STAT pathway in tephritid flies,shedding light on the immune mechanisms of ***.

关键词： Bactrocera dorsalis JAK/STAT pathway Domeless receptors antiviral immunity symbiont-like virus

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Stability of bedded rock slopes subjected to hydro-fluctuation and associated strength deterioration

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第8期16卷 3233-3257页

作者： Bin Xu Xinrong Liu Yue Liang Xiaohan Zhou Zuliang Zhong School of River and Ocean Engineering Chongqing Jiaotong UniversityChongqing400074China School of Civil Engineering Chongqing UniversityChongqing400045China

Reservoir-induced earthquakes(RIEs)occur frequently in the Three Gorges Reservoir Area(TGRA)and the rock mass strength of the hydro-fluctuation belt(HFB)deteriorates severely due to the reservoirinduced seismic *** models of typical bedded rock slopes(BRSs),***(GIS),moderately(MIS),and steeply(SIS)inclined slopes,were proposed according to field *** dynamic response mechanism and stability of the BRSs,affected by the rock mass deterioration of the HFB,were investigated by the shaking table test and the universal distinct element code(UDEC)***,the amplification coefficient of the peak ground acceleration(PGA)of the slope was gradually attenuated under multiple seismic loads,and the acceleration response showed obvious“surface effect”and“elevation effect”in the horizontal and vertical directions,***“S-type”cubic function and“steep-rise type”exponential function were used to characterize the cumulative damage evolution of the slope caused by microseismic waves(low seismic waves)and high seismic waves,*** to the dynamic responses of the acceleration,cumulative displacement,rock pressure,pore water pressure,damping ratio,natural frequency,stability coefficient,and sliding velocity of the slope,the typical evolution processes of the dynamic cumulative damage and instability failure of the slope were generalized,and the numerical and experimental results were *** the dynamic effects of the slope height(SH),slope angle(SA),bedding plane thickness(BPT),dip angle of the bedding plane(DABP),dynamic load amplitude(DLA),dynamic load frequency(DLF),height of water level of the hydro-fluctuation belt(HWLHFB),degradation range of the hydro-fluctuation belt(DRHFB),and degradation shape of the hydro-fluctuation belt(DSHFB),the sensitivity of factors influencing the slope dynamic stability using the orthogonal analysis method(OAM)was DLA>DRHFB>SA>SH>DLF>HWLHFB>DSHFB>DABP>BPT.

关键词： Bedded rock slopes Hydro-fluctuation belt Shaking table test UDEC simulation Dynamic response mechanism

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Precise construction of RuPt dual single-atomic sites to optimize oxygen electrocatalytic behaviors for high-performance Zn-air batteries

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Journal of Energy Chemistry 2024年第10期97卷 520-528页

作者： Xiaolin Hu Zhenkun Wu Chaohe Xu School of Science Chongqing Key Laboratory of New Energy Storage Materials and Devices Chongqing University of Technology School of Chemistry and Engineering Chongqing University College of Materials Science and Engineering Chongqing University

The development of redox bifunctional electrocatalysts with high performance,low cost,and long lifetimes is essential for achieving clean energy *** study proposed an atom capture strategy for anchoring dual single atoms（DSAs） in a zinc-zeolitic imidazolate framework（Zn-ZIF）,followed by calcination under an N2atmosphere to synthesize ruthenium-platinum DSAs supported on a nitrogendoped carbon substrate（RuPt DSAs-NC）.Theoretical calculations showed that the degree of Ru 5dxz-*O 2pxorbital hybridization was high when*O was adsorbed at the Ru site,indicating enhanced covalent hybridization of metal sites and oxygen ligands,which benefited the adsorption of intermediate *** presence of the RuPtN6active center optimized the absorption-desorption behavior of intermediates,improving the electrocatalytic performance of the oxygen reduction reaction（ORR） and the oxygen evolution reaction（DER）,RuPt DSAs-NC exhibited a 0.87 V high half-wave potential and a 268 mV low overpotential at 10 mA cm-2in an alkaline ***,rechargeable zinc-air batteries（ZABs）achieved a peak power density of 171 MW *** RuPt DSAs-NC demonstrated long-term cycling for up to 500 h with superior round-trip *** study provided an effective structural design strategy to construct DSAs active sites for enhanced electrocata lytic performance.

关键词： Atom capture Dual single atoms catalysts Oxygen evolution reaction Oxygen reduction reaction Rechargeable Zn-air batteries

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Comprehensive analysis of the gut microbiome and posttranslational modifications elucidates the route involved in microbiota-host interactions

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Zoological research 2024年第1期45卷 95-107页

作者： Hai-Yang Wang Lan-Xiang Liu Xue-Yi Chen Yang-Dong Zhang Wen-Xia Li Wen-Wen Li Lian Wang Xiao-Long Mo Hong Wei Ping Ji Peng Xie NHC Key Laboratory of Diagnosis and Treatment on Brain Functional Diseases First Affiliated Hospital of Chongqing Medical UniversityChongqing 400016China College of Stomatology and Affiliated Stomatological Hospital of chongqing Medical University Chongqing 401147China chongqing Key Laboratory for Oral Diseases and Biomedical Sciences Chongqing 401147China Department of Neurology Yongchuan Hospital of Chongqing Medical UniversityChongqing 402160China Department of Pathology Faculty of Basic MedicineChongqing Medical UniversityChongqing 400016China Department of Neurology First Affiliated Hospital of Chongqing Medical UniversityChongqing 400016China Yu-Yue Pathology Scientific research Center Chongqing 401329China

The gut microbiome interacts with the host to maintain body homeostasis,with gut microbial dysbiosis implicated in many ***,the underlying mechanisms of gut microbe regulation of host behavior and brain functions remain *** study aimed to elucidate the influence of gut microbiota on brain functions via post-translational modification mechanisms in the presence or absence of bacteria without any *** conducted succinylome analysis of hippocampal proteins in germ-free(GF)and specific pathogen-free(SPF)mice and metagenomic analysis of feces from SPF *** results were integrated with previously reported hippocampal acetylome and phosphorylome data from the same batch of *** bioinformatics analyses revealed 584 succinylation sites on 455 proteins,including 54 up-regulated succinylation sites on 91 proteins and 99 down-regulated sites on 51 proteins in the GF mice compared to the SPF *** constructed a panoramic map of gut microbiota-regulated succinylation,acetylation,and phosphorylation,and identified cross-talk and relative independence between the different types of post-translational modifications in modulating complicated intracellular *** correlation analysis indicated that 13 taxa,predominantly belonging to the Bacteroidetes phylum,were correlated with the biological functions of post-translational *** correlations between these taxa and succinylation and negative correlations between these taxa and acetylation were identified in the modulation of intracellular *** study highlights the hippocampal physiological changes induced by the absence of gut microbiota,and proteomic quantification of succinylation,phosphorylation,and acetylation,contributing to our understanding of the role of the gut microbiome in brain function and behavioral phenotypes.

关键词： Gut microbiota Hippocampal protein Post-translational modifications Succinylation Acetylation Phosphorylation

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Retrieval-and-alignment based large-scale indoor point cloud semantic segmentation

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Science China(Information Sciences) 2024年第4期67卷 164-180页

作者： Zongyi XU Xiaoshui HUANG Bo YUAN Yangfu WANG Qianni ZHANG Weisheng LI Xinbo GAO School of Computer Science and Technology Chongqing University of Posts and Telecommunications Shanghai Artificial Intelligence Laboratory School of Electronic Engineering and Computer Science Queen Mary University of London

Current methods for point cloud semantic segmentation depend on the extraction of descriptive features. However, unlike images, point clouds are irregular and often lack texture information, making it demanding to extract discriminative features. In addition, noise, outliers, and uneven point distribution are commonly present in point clouds, which further complicates the segmentation task. To address these problems, a novel architecture is proposed for direct and accurate large-scale point cloud segmentation based on point cloud retrieval and alignment. The proposed approach involves using a feature-based point cloud retrieval method for searching for reference point clouds with annotations from a dataset. In the following segmentation stage, an overlap-based point cloud registration method has been developed to align the target and reference point clouds. For accurate and robust alignment, an overlap region estimation module is trained to locate the optimal overlap region between two pieces of point clouds in a coarse-to-fine manner. In the detected overlap region, the global and local features of the points are extracted and combined for featuremetric registration to obtain accurate transformation parameters between the target and reference point clouds. After alignment, the annotated segmentation of the reference is transferred to the target point clouds to obtain accurate segmentation results. Extensive experiments are conducted to show that the developed method outperforms the state-of-the-art approaches in terms of both accuracy and robustness against noise and outliers.

关键词： point cloud semantic segmentation large-scale indoor point clouds point cloud alignment overlap estimation label transfer

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Microstructure Evolution and Mechanical Properties of Friction Stir Welded Al-Cu-Li Alloy

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Acta Metallurgica Sinica(English Letters) 2024年第5期37卷 855-871页

作者： Peng Chen Wenhao Chen Jiaxin Chen Zhiyu Chen Yang Tang Ge Liu Bensheng Huang Zhiqing Zhang School of New Energy and Materials Southwest Petroleum UniversityChengdu 610500China Sichuan Provincial Engineering research Center of Advanced Materials Manufacturing Technology for Shale Gas High-Efficient Exploitation Southwest Petroleum UniversityChengdu 610500China College of Materials Science and Engineering Chongqing UniversityChongqing 400045China School of Mechatronic Engineering Southwest Petroleum UniversityChengdu 610500China School of Robot Engineering Yangtze Normal UniversityChongqing 408100China

The investigation concentrates on friction stir welded(FSW)Al-Cu-Li alloy concerning its local microstructural evolution and mechanical *** grain features were characterized by electron back scattered diffraction(EBSD)technology,while precipitate characterization was conducted by using transmission electron microscopy(TEM)aligned along[011]Al and[001]Al zone *** mechanical properties are evaluated through micro-hardness and tensile *** can be found that nugget zones exhibit finely equiaxed grains evolved through complete dynamic recrystallization(DRX),primarily occurring in continuous dynamic recrystallization(CDRX)and discontinuous dynamic recrystallization(DDRX).In the thermal-mechanically affected zone(TMAZ),numerous sub-structured grains,exhibiting an elongated morphology,were created due to partial DRX,signifying the dominance of CDRX,DDRX,and geometric dynamic recrystallization(GDRX)in this region.T_(1)completely dissolves in the nugget zone(NZ)leading to the formation of Guinier-Preston zones and increase ofδ′,β′and S′.Conversely,T_(1)partially solubilizes in TMAZ,the lowest hardness zone(LHZ)and heat affected zone(HAZ),and the residual T_(1)undergoes marked coarsening,revealing various T_(1)*** solubilization and coarsening of T_(1)are primary contributors to the degradation of hardness and strength.θ′primarily dissolves and coarsens in NZ and TMAZ,whilst this precipitate largely coarsens in HAZ and LHZ.σ,TB,grain boundary phases(GBPs)and precipitate-free zone(PFZ)are newly generated during FSW.σexists in the TMAZ,LHZ and HAZ,whereas TB nucleates in *** and PFZ mostly develop in LHZ and HAZ,which can cause strain localization during tensile deformation,potentially leading to LHZ joint fracture.

关键词： Al-Cu-Li alloy Friction stir welding Microstructure evolution Mechanical properties

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Video caching and scheduling with edge cooperation

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Digital Communications and Networks 2024年第2期10卷 450-460页

作者： Zhidu Li Fuxiang Li Tong Tang Hong Zhang Jin Yang School of Communication and Information Engineering Chongqing University of Posts and TelecommunicationsChongqing400065China Advanced Network and Intelligent Connection Technology Key Laboratory of chongqing Education Commission of China Chongqing400065China Key Laboratory of Ubiquitous Sensing and Networking in chongqing Chongqing400065China

In this paper,we explore a distributed collaborative caching and computing model to support the distribution of adaptive bit rate video *** aim is to reduce the average initial buffer delay and improve the quality of user *** the difference between global and local video popularities and the time-varying characteristics of video popularity,a two-stage caching scheme is proposed to push popular videos closer to users and minimize the average initial buffer *** on both long-term content popularity and short-term content popularity,the proposed caching solution is decouple into the proactive cache stage and the cache update *** the proactive cache stage,we develop a proactive cache placement algorithm that can be executed in an off-peak *** the cache update stage,we propose a reactive cache update algorithm to update the existing cache policy to minimize the buffer *** results verify that the proposed caching algorithms can reduce the initial buffer delay efficiently.

关键词： Video service Distributed and collaborative caching Long-term popularity Short-term popularity

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Enhancing visible-light-driven NO oxidation through molecular‐level insights of dye-loaded sea sands

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Rare Metals 2024年第2期43卷 543-554页

作者： Yu-Han Li Bang-Fu Chen Sónia A.C.Carabineiro You-Yu Duan Ping Tan Wing-Kei Ho Fan Dong Engineering research Center for Waste Oil Recovery Technology and Equipment Ministry of EducationChongqing Key Laboratory of Catalysis and New Environmental MaterialsChongqing Technology and Business UniversityChongqing400067China Nanchang Institute of Technology Nanchang33044China LAQV-REQUIMTE Department of ChemistryNOVA School of Science and TechnologyUniversidade NOVA de Lisboa2829-516CaparicaPortugal College of Physics and Center of Quantum Materials and Devices Chongqing UniversityChongqing401331China Department of Science and Environmental Studies The Education University of Hong KongHong Kong999077China

Natural minerals,abundant and easily obtained through simple physical processing,offer a cost-effective and environmentally friendly solution for dyeing wastewater disposal and air pollution *** study investigates the photocatalytic removal of NO using natural different types of dyes,loaded on natural sand,under visible light *** examining various coating concentrations of dyes and sand weights,we discovered that sand loaded with Rhodamine B(RhB)exhibits high activity for the photo-oxidation of NO.A combination results of X-ray diffraction(XRD),X-ray photoelectron spectroscopy(XPS),Fourier transform infrared spectroscopy(FTIR)and thermogravimetric(TG)analyses confirm the presence of SiO_(2),CaCO_(3),Al_(2)O_(3)and iron oxides as the main components of the ***,studying RhB-loaded individual components reveals that CaCO_(3)plays a crucial role in enhancing the NO removal *** results and theoretical calculations demonstrate the establishment of a directional charge transfer channel from CaCO_(3)to RhB,facilitating the adsorption and activation of molecular NO and O_(2).This work not only promotes the utilization of natural mineral resources but also enriches the fields of environmental photochemistry and semiconductor photocatalysis.

关键词： Sand dyes Rhodamine B Photo-oxidation of NO Visible light illumination

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Analytical Expression for the Atomic Friction of a Single Asperity Based on the Prandtl-Tomlinson Model

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Acta Mechanica Solida Sinica 2024年第3期37卷 416-422页

作者： Weike Yuan Yue Ding Gangfeng Wang Xinrui Niu Department of Engineering Mechanics SVLMMLXi’an Jiaotong UniversityXi’an710049China Department of Mechanical Engineering City University of Hong KongHong Kong SAR999077China

The Prandtl-Tomlinson(PT)model has been widely applied to interpret the atomic friction mechanism of a single *** this study,we present an approximate explicit expression for the friction force in the one-dimensional PT model under quasi-static ***‘stick-slip’friction curves are first approximated properly by sawtooth-like lines,where the critical points before and after the‘slip’motion are described analytically in terms of a dimensionless parameterη.Following this,the average friction force is expressed in a closed form that remains continuous and valid forη>***,an analytical expression for the load dependence of atomic friction of a single asperity is derived by connecting the parameterηwith the normal *** the parameters reported in experiments,our prediction shows good agreement with relevant experimental results.

关键词： Atomic friction Stick-slip friction Prandtl-Tomlinson model Friction force microscope

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