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Lithium Salt Combining Fluoroethylene Carbonate Initiates Methyl Methacrylate Polymerization Enabling Dendrite-Free Solid-State Lithium Metal Battery

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Energy & Environmental Materials 2024年第6期7卷 50-59页

作者： Xue Ye Jianneng Liang Baorong Du Yongliang Li Xiangzhong Ren Dazhuan Wu Xiaoping Ouyang Qianling Zhang Jianhong Liu Institute of Process Equipment College of Energy EngineeringZhejiang UniversityHangzhou310000 China Graphene Composite research Center College of Chemistry and Environmental EngineeringShenzhen UniversityShenzhen518061 China

This work demonstrates a novel polymerization-derived polymer electrolyte consisting of methyl methacrylate,lithium bis(trifluoromethanesulfonyl)imide and fluoroethylene *** polymerization of MMA was initiated by the amino compounds following an anionic catalytic *** plays both roles including the initiator and Li ion source in the polymer ***,lithium bis(trifluoromethanesulfonyl)imide has difficulty in initiating the polymerization reaction of methyl methacrylate monomer,a very high concentration of lithium bis(trifluoromethanesulfonyl)imide is needed for initiating the ***,the fluoroethylene carbonate additive can work as a supporter to facilitate the degree of dissociation of lithium bis(trifluoromethanesulfonyl)imide and increase its initiator capacity due to the high dielectric *** as-prepared poly-methyl methacrylate-based polymer electrolyte has a high ionic conductivity(1.19×10^(−3)S cm^(−1)),a wide electrochemical stability window(5 V vs Li^(+)/Li),and a high Li ion transference number(t_(Li^(+)))of 0.74 at room temperature(RT).Moreover,this polymerization-derived polymer electrolyte can effectively work as an artificial protective layer on Li metal anode,which enabled the Li symmetric cell to achieve a long-term cycling performance at 0.2 mAh cm^(−2)for 2800 *** LiFePO_(4)battery with polymerization-derived polymer electrolyte-modified Li metal anode shows a capacity retention of 91.17%after 800 cycles at 0.5 *** work provides a facile and accessible approach to manufacturing poly-methyl methacrylate-based polymerization-derived polymer electrolyte and shows great potential as an interphase in Li metal batteries.

关键词： in situ polymerization lithium anode polymer electrolyte solid-state lithium batteries

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Preparation and Photostriction Properties of BiFeO_(3)-BaTiO_(3)Ceramics

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Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1079-1086页

作者： ZHENG Zewei ZHANG Liqiang CHEN Chen CAO Minghe YI Zhiguo LIU Hanxing School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China State key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China School of Microelectronics Shanghai UniversityShanghai 200444China International School of Materials Science and Engineering Wuhan University of TechnologyWuhan 430070China

Under illumination by 405,520 and 655 nm monochromatic visible light(light intensity of 30 kW/m^(2)),large photostriction(ΔL/L)of 0.19%,0.13%and 0.26%for 67BiFeO_(3)-33BaTiO_(3)(67BF-33BT)lead-free ferroelectric ceramics are obtained,*** studying the ferroelectric and photoelectric properties in conjunction with in situ Raman spectroscopy,it is found that the photostrictive effect of 67BF-33BT is not caused by the electrical strain induced by abnormal photovoltaic voltage,but related to the optical induced oxygen octahedral *** 67BF-33BT lead-free ferroelectric material with excellent photostrictive response in the visible light region is expected to play an important role in the field of optical drive electromechanical devices.

关键词： ferroelectric ceramics photostrictive effect visible light response

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Interface failure of segmental tunnel lining strengthened with steel plates based on fracture mechanics

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Frontiers of Structural and Civil Engineering 2024年第1期18卷 137-149页

作者： Yazhen SUN Yang YU Jinchang WANG Longyan WANG School of Transportation and Geomatics Engineering Shenyang Jianzhu UniversityShenyang 110168China School of Civil Engineering Shenyang Jianzhu UniversityShenyang 110168China Institute of Transportation Engineering Zhejiang UniversityHangzhou 310058China Center for Balance Architecture Zhejiang UniversityHangzhou310058China

Segmental tunnel lining strengthened with steel plates is widely used worldwide to provide a permanent strengthening *** existing studies assume an ideal steel-concrete interface,ignoring discontinuous deformation characteristics,making it difficult to accurately analyze the strengthened structure’s failure *** this study,interfacial fracture mechanics of composite material was applied to the segmental tunnel lining strengthened with steel plates,and a numerical three-dimensional solid nonlinear model of the lining structure was established,combining the extended finite element method with a cohesive-zone model to account for the discontinuous deformation characteristics of the *** results accurately describe the crack propagation process,and are verified by full-scale ***,dynamic simulations based on the calibrated model were conducted to analyze the sliding failure and cracking of the steel-concrete ***,detailed location of the interface bonding failure are further verified by model *** results show that,the cracking failure and bond failure of the interface are the decisive factors determining the instability and failure of the strengthened *** proposed numerical analysis is a major step forward in revealing the interface failure mechanism of strengthened composite material structures.

关键词： segmental tunnel lining steel plate strengthening connecting interface cohesive-zone model extended finite element method

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Mechanical properties and interfacial characteristics of 6061 Al alloy plates fabricated by hot-roll bonding

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International Journal of Minerals,Metallurgy and Materials 2024年第8期31卷 1890-1899页

作者： Zongan Luo Xin Zhang Zhaosong Liu Hongyu Zhou Mingkun Wang Guangming Xie State key Laboratory of Rolling and Automation Northeastern UniversityShenyang 110819China

This work aims to investigate the mechanical properties and interfacial characteristics of 6061 Al alloy plates fabricated by hotroll bonding(HRB)based on friction stir *** results showed that ultimate tensile strength and total elongation of the hot-rolled and aged joints increased with the packaging vacuum,and the tensile specimens fractured at the matrix after exceeding 1 ***-equilibrium grain boundaries were formed at the hot-rolled interface,and a large amount of Mg_(2)Si particles were linearly precipitated along the interfacial grain boundaries(IGBs).During subsequent heat treatment,Mg_(2)Si particles dissolved back into the matrix,and Al_(2)O_(3) film remaining at the interface eventually evolved into *** addition,the local IGBs underwent staged elimination during HRB,which facilitated the interface healing due to the fusion of grains at the *** process was achieved by the dissociation,emission,and annihilation of dislocations on the IGBs.

关键词： 6061 Al alloy hot-roll bonding vacuum mechanical properties interfacial grain boundaries

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Strip flatness prediction of cold rolling based on ensemble methods

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Journal of Iron and Steel research International 2024年第1期31卷 237-251页

作者： Wu-quan Yang Zhi-ting Zhao Liang-yu Zhu Xun-yang Gao Li Wang School of Mechanical and Power Engineering Shenyang University of Chemical TechnologyShenyang110142LiaoningChina

Aiming at the problem of insufficient prediction accuracy of strip flatness at the outlet of cold tandem rolling,the prediction performance of strip flatness based on different ensemble methods was studied and a high-precision prediction ensemble model of strip flatness at the outlet was ***,based on linear regression(LR),K nearest neighbors(KNN),support vector regression,regression trees(RT),and backpropagation neural network(BPN),bagging,boosting,and stacking ensemble methods were used for ensemble ***,three existing ensemble models,i.e.,random forest,extreme random tree(ET)and extreme gradient boosting,were used to conduct experiments and compare the *** research shows that bagging,boosting,and stacking three ensemble methods have the most significant improvement in the prediction accuracy of the regression trees model,which is increased by 5.28%,6.51%,and 5.32%,*** the same time,the stacking ensemble method improves both the simple model and the complex model,and the improvement effect on the simple base model is the greatest,which is 4.69%higher than that of the base model *** all of the ensemble models,the stacking ensemble model of level-1(ET,AdaBoost-RT,LR,BPN)paired with level-2(LR)was discovered to be the best model(EALB-LR)and can be further studied for industrial applications.

关键词： Tandem cold rolling Flatness prediction Machine learning Ensemble method

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Effect of long reaction distance on gas composition from organic-rich shale pyrolysis under high-temperature steam environment

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International Journal of Coal Science & Technology 2024年第3期11卷 102-119页

作者： Lei Wang Rui Zhang Guoying Wang Jing Zhao Dong Yang Zhiqin Kang Yangsheng Zhao key Laboratory of In-Situ Property Improving Mining of Ministry of Education Taiyuan University of TechnologyTaiyuan030024China The In-Situ Steam Injection Branch of State Center for research and Development of Organic-Rich Shale Exploitation Taiyuan University of TechnologyTaiyuan030024China College of Mining Engineering Taiyuan University of TechnologyTaiyuan030024China School of Energy Science and Engineering Henan Polytechnic UniversityJiaozuo454002China

When high-temperature steam is used as a medium to pyrolyze organic-rich shale,water steam not only acts as heat transfer but also participates in the chemical reaction of organic matter pyrolysis,thus affecting the generation law and release characteristics of gas *** this study,based on a long-distance reaction system of organic-rich shale pyrolysis via steam injection,the effects of steam temperature and reaction distance on gas product composition are analyzed in depth and compared with other pyrolysis *** advantages of organic-rich shale pyrolysis via steam injection are then *** volume concentration of hydrogen in the gas product obtained via the steam injection pyrolysis of organic-rich shale is the highest,which is more than 60%.The hydrogen content increases as the reaction distance is extended;however,the rate of increase changes *** the reaction distance from 800 to 4000 mm increases the hydrogen content from 34.91%to 69.68%and from 63.13%to 78.61%when the steam temperature is 500℃ and 555℃,***,the higher the heat injection temperature,the smaller the reaction distance required to form a high concentration hydrogen pyrolysis environment(hydrogen concentration>60%).When the steam pyrolysis temperature is increased from 500℃ to 555℃,the reaction distance required to form a high concentration of hydrogen is reduced from 3800 to 800 *** with the direct retorting process,the volume concentration of hydrogen obtained from high-temperature steam pyrolysis of organic-rich shale is 8.82 and 10.72 times that of the commonly used Fushun and Kivite furnaces,*** pyrolysis of organic-rich shale via steam injection is a pyrolysis process in a hydrogen-rich environment.

关键词： Steam temperature Pyrolysis gas Hydrogen-rich Reaction distance Direct retorting

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Ionic liquid-assisted preparation of hydroxyapatite and its catalytic performance for decarboxylation of itaconic acid

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Chinese Journal of Chemical Engineering 2024年第3期67卷 9-15页

作者： Shutong Pang Hualiang An Xinqiang Zhao Yanji Wang Hebei Provincial key Laboratory of Green Chemical Technology and Efficient Energy Saving Tianjin Key Laboratory of Chemical Process SafetySchool of Chemical Engineering and TechnologyHebei University of TechnologyTianjin 300130China

The synthesis of methacrylic acid from biomass-derived itaconic acid is a green route,for it can get rid of the dependence on fossil *** order to solve the problems on this route such as use of a preciousmetal catalyst and a corrosive homogeneous alkali,we prepared a series of hydroxyapatite catalysts by an ionic liquid-assisted hydrothermal method and evaluated their catalytic *** results showed that the ionic liquid[Bmim]BF_(4) can affect the crystal growth of hydroxyapatite,provide fluoride ion for fluorination of hydroxyapatite,and adjust the surface acidity and basicity,morphology,textural properties,crystallinity,and composition of ***[Bmim]BF4 dosage and hydrothermal temperature can affect the fluoride ion concentration in the hydrothermal system,thus changing the degree of fluoridation of *** fluoride-ion concentration can lead to the formation of CaF_(2) and thus significantly decrease the catalytic performance of *** hydrothermal time mainly affects the growth of hydroxyapatite crystals on the c axis,leading to different catalytic *** suitable conditions for the preparation of this fluoridized hydroxyapatite are as follows:a mass ratio of[Bmim]BF4 to calcium salt=0.2:1,a hydrothermal time of 12 h,and a hydrothermal temperature of 130℃.A maximal methacrylic acid yield of 54.7%was obtained using the fluoridized hydroxyapatite under relatively mild reaction conditions(250℃ and 2 MPa of N_(2))in the absence of a precious-metal catalyst and a corrosive homogeneous alkali.

关键词： Ionic liquid Hydroxyapatite Itaconic acid Methacrylic Decarboxylation reaction

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The deteriorated degradation resistance of Mg alloy microtubes for vascular stent under the coupling effect of radial compressive stress and dynamic medium

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Journal of Magnesium and Alloys 2024年第2期12卷 573-585页

作者： Mengyao Liu Yabo Zhang Qingyuan Zhang Yan Wang Di Mei Yufeng Sun Liguo Wang Shijie Zhu Shaokang Guan School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001China Henan key Laboratory of Advanced Magnesium Alloys Zhengzhou 450002China key Laboratory of Advanced Materials Processing&Mold Ministry of Education Zhengzhou 450002China

The degradation of Mg alloys relates to the service performance of Mg alloy biodegradable *** order to investigate the degradation behavior of Mg alloys as vascular stent materials in the near service environment,the hot-extruded fine-grained Mg-Zn-Y-Nd alloy microtubes,which are employed to manufacture vascular stents,were tested under radial compressive stress in the dynamic Hanks'Balanced Salt Solution(HBSS).The results revealed that the high flow rate accelerates the degradation of Mg alloy microtubes and its degradation is sensitive to radial compressive *** results contribute to understanding the service performance of Mg alloys as vascular stent materials.

关键词： Mg alloy Microtubes Degradation behavior Radial compressive stress Dynamic conditions

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Ionization Potential Depression Model for Warm/Hot and Dense Plasmas

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Chinese Physics Letters 2024年第8期41卷 45-57页

作者： Chensheng Wu Fuyang Zhou Jun Yan Xiang Gao Yong Wu Chunhua Zeng Jianguo Wang Institute of Applied Physics and Computational Mathematics Beijing 100088China Faculty of Science Kunming University of Science and TechnologyKunming 650500China

For warm/hot and dense plasmas(WDPs),ionization potential depression(IPD)plays a crucial role in determining its ionization balance and understanding the resultant microscopic plasma properties.A sophisticated and unified IPD model is necessary to resolve those existing discrepancies between theoretical and experimental ***,the applicability of those widely used IPD models nowadays is limited,especially for the nonlocal thermodynamic equilibrium(non-LTE)dense plasma produced by short-pulse *** this work,we propose an IPD model that considers inelastic atomic processes,in which three-body recombination and collision ionization processes are found to play a crucial role in determining the electron distribution and IPD for a *** IPD model is validated by reproducing latest experimental results of Al plasmas with a wide-range condition of 70 eV–700 eV temperature and 0.2–3 times solid density,as well as a typical non-LTE system of hollow Al *** is demonstrated that the present IPD model has a significant temperature dependence due to the consideration of the inelastic collision *** a lower computational cost and wider application range of plasma conditions,the proposed model is expected to provide a promising tool to study the ionization balance and the atomic processes,as well as the related radiation and particle transports properties of the WDP.

关键词： properties. collision determining

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A study of U-isotope ground state properties with covariant energy density functional

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Chinese Physics C 2024年第6期48卷 130-135页

作者：王俊辰田源续瑞瑞崔莹陶曦孙小东张智张玥韩银录葛智刚舒能川 China Nuclear Data Center China Institute of Atomic EnergyBeijing 102413China China Institute of Atomic Energy Beijing 102413China

In this study,we systematically analyzed the ground state of uranium isotopes from 225 to *** our calculations,we used the covariant energy density functional of density-dependent meson exchange interaction(DDME2)with separable pairing interaction(TMR).Using the multiple deformation constraint,we calculated the potential energy surface(PES)of the uranium isotopes for both even-even and even-odd nuclei with quadrupole and octupole *** on our calculation and upon comparing the experimental data and Hartree-Fock-Bogoliubov calculations with Gogny D1S calculation data,the ground state of uranium isotopes with reflection-asymmetric deformation was found to be preferred.

关键词： relativistic mean field density functional theory octupole deformation

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