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Effect of Y_(2)O_(3) on microstructure and properties of CoCrFeNiTiNb high entropy alloy coating on Ti-6Al-4V surface by laser cladding

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Journal of Rare Earths 2024年第3期42卷 586-599,I0006页

作者： Zhen Li Wei Zhao Kedong Yu Ning Guo Guangchun Xiao Zhiming Wang Hui Zhang College of Mechanical Engineering Qilu University of Technology(Shandong Academy of Sciences)Jinan250353China shandong Institute of Mechanical Design and research Jinan250031China

The effects of Y_(2)O_(3) on the microstructure, microhardness, wear resistance, high-temperature oxidation resistance, hot corrosion resistance, and electrochemical corrosion behaviour of CoCrFeNiTiNb high entropy alloy coatings formed on Ti-6Al-4V alloy surfaces were studied. The results show that the addition of Y_(2)O_(3) changes the proportion of the phase but does not change its type. The average grain size is only 1/4.7 of that of the high entropy alloy(HEA) coating, and the fine-grained strengthening leads to increases in the microhardness and wear resistance of 21.8% and 26.9%, respectively. The addition of Y_(2)O_(3) enhances the denseness and bonding properties of the oxide and corrosion product layers, reducing the oxidation and hot corrosion rates by 60.3% and 40.3%, respectively. The addition of Y_(2)O_(3) doubles the corrosion resistance which is attributed to the refinement of the grains, the increased proportion of HCP and TiN, and the weakening of galvanic coupling corrosion.

关键词： Laser cladding High entropy alloy coatings Rare earths Wear properties High temperature properties Electrochemical corrosion

Overview of enhancing biological treatment of coal chemical wastewater:New strategies and future directions

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Journal of Environmental Sciences 2024年第1期135卷 506-520页

作者： Weiwei Ma Xiaoqi Zhang Hongjun Han Xueqing Shi Qiaoping Kong Tong Yu Fei Zhao School of Environmental and Municipal Engineering Qingdao University of TechnologyQingdao 266520China State key Laboratory of Urban Water Resource and Environment Harbin Institute of TechnologyHarbin 150090China

Coal chemical wastewater(CCW)is a type of refractory industrial wastewater,and its treatment has become the main bottleneck restricting the sustainable development of novel coal chemical *** treatment is considered as an economical,effective and environmentally friendly technology for CCW ***,conventional biological process is difficult to achieve the efficient removal of refractory organics because of CCW with the characteristics of composition complexity and high ***,seeking the novel enhancement strategy appears to be a favorable solution for enhancing biological treatment efficiency of *** review focuses on presenting a comprehensive picture about the exogenous enhancement strategies for CCW biological *** performance and potential application of exogenous enhancement strategies,including co-metabolic substrate enhancement,biofilm filler enhancement,adsorption material enhancement and conductive mediator enhancement,were ***,the enhancing mechanisms of different strategies were comprehensively discussed from a biological ***,the prospects of enhancement strategies based on the engineering performance,economic cost and environmental impact(3E)evaluation were *** novel enhancement strategy based on“low carbon emissions”,“resource recycling”and“water environment security”in the context of carbon neutrality was *** together,this review provides technical reference and new direction to facilitate the regulation and optimization of typical industrial wastewater biological treatment.

关键词： Coal chemical wastewater Biological treatment Exogenous enhancement Refractory organics 3E evaluation

Molecular Mechanism of Polysaccharides Extracted from Chinese Medicine Targeting Gut Microbiota for Promoting Health

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Chinese Journal of Integrative Medicine 2024年第2期30卷 171-180页

作者： ZHAO Wen-xiao WANG Tong ZHANG Ya-nan CHEN Qian WANG Yuan XING Yan-qing ZHENG Jun DUAN Chen-chen CHEN Lijun ZHAO Hai-jun WANG Shijun School of Nursing Shandong University of Traditional Chinese MedicineShandong University of Traditional Chinese MedicineJi'nan(250355)China shandong Co-innovation Center of Classic Traditional Chinese Medicine Formula Shandong University of Traditional Chinese MedicineJi'nan(250355)China College of Traditional Chinese Medicine Shandong University of Traditional Chinese MedicineJinan(250355)China

The accumulating evidence revealed that gut microbiota plays an important role in pathological process of disease including obesity,type 2 diabetes mellitus,heart failure,and non-alcoholic fatty liver *** extracted from Chinese medicine(CM)can not only alleviate pathological status but also promote health by anti-inflammatory,regulating immunity,lowering blood glucose and lipids,anti-cancer,and *** alterations of gut microbiota composition and metabolism pathways are the potential mechanisms of CM polysaccharides *** addition,they exert functions through gut-organ axis or play an indirect role by synergistic actions with other drugs or components mediated by gut *** review summarizes the molecular mechanisms of CM polysaccharides interacted with intestinal microbial inhabitants as potential prebiotics forpromoting health.

关键词： Chinese medicine polysaccharides gut microbiota short-chain fatty acids lipopolysaccharides gut-organaxis synergistic actions

Extraction and evolution of grader’s bionic morphological feature line using shape structure behavior function model

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International Journal of Agricultural and Biological Engineering 2024年第2期17卷 74-84页

作者： Bin Qi Yubin Lan Xiaoming Sun He Zhu Yanhao Li Ke Lou College of Agricultural Engineering and Food Science Shandong University of TechnologyZibo 255049ShandongChina shandong Provincial Engineering Technology research Center for Agricultural Aviation Intelligent Equipment Zibo 255049China

To improve the innovation of agricultural machinery product styling,this paper proposes a shape structure behavior function(SSBF)model suitable for the industrial design *** feature line evolution method combining shape grammar and genetic algorithm was used for modelling the of the grader,which not only maintains the product style characteristics but also reflects the typical identification characteristics of the bionic prototype and produces a new product modelling *** conducting cognitive and recognition experiments on product styling features,the ranking of product styling features and the contribution of each component to product styling were *** method of combining shape grammar and quadratic Bézier curve was used to express and encode feature lines,and genetic algorithm was used to evolve biomimetic forms to form product feature lines with typical biological morphological features;The extracted form bionic elements were integrated into the grader modelling design,and the interaction evaluation was carried out through the genetic algorithm evolution *** basic form elements were extracted and analyzed,and the deduction rules were formulated and *** derived feature line geometric data considered the product’s image features and the bio-inspired prototype,which can be used for the follow-up guidance of industrial design schemes.

关键词： bionic design shape-structure-behavior-function SSBF biologically inspired design BID shape grammars Quadratic Bézier curves

MnO-pillared graphene blocks enabling the ultrastable and ultrafast aqueous zinc ion batteries

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Science China Chemistry 2024年第9期67卷 2930-2940页

作者： Zheng Liu Zhipeng Qiu Zhiyuan Li Tong Wei Zhuangjun Fan Huan Pang School of Chemistry and Chemical Engineering Yangzhou University School of Materials Science and Engineering China University of Petroleum

Due to the low cost, high theoretical capacity, and environmental friendliness, manganese-based cathodes are regarded as promising alternatives for aqueous zinc ion batteries（AZIBs）. However, the practicality of the zinc-manganese system is faced with great challenges, such as the inevitable structural collapse of the cathode and controversial energy storage ***, we propose a novel concept of spatial deposition mechanism through the addition of MnSO4additives in the Mn O-pillared graphene blocks（G-MnO）. The covalent interface between MnO nanoparticles and multilayered graphene nanosheets can construct an in-built micro-electric field, which is beneficial for consecutive electron transfer（in both horizontal and vertical directions）. On this basis, the surficial activity of MnO confined in the interlayered nano-space is greatly enhanced and provides enough spatial deposition and subsequent reaction site for MnSO4additives, thus firstly extending the surficial controlled process to stereoscopic space, effectively improving the electrochemical performance of AZIBs. Therefore, the assembled Zn//G-Mn O battery exhibits an excellent rate capability of 281.5 mAhg-1at 0.1 A g-1and 106 mAhg-1at 20 Ag-1, and impressive cycling stability(93 mAhg-1remaining after 5,000 cycles). This finding may provide a new opportunity for the rational design of surficial controlled energy storage and conversion devices.

关键词： zinc-ion battery manganese monoxide laminated constructure ultrahigh rate performance graphene

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MOF-templated tubular Ni_(1−x)Co_(x)S_(2)-CdS heterojunction with intensified direct Z-scheme charge transmission for highly promoted visible-light photocatalysis

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Nano research 2024年第7期17卷 6281-6293页

作者： Chuan Jiang Yuanxin Qiu Xinxin Xin Yanyan Li Huilin Li Hui Wang Jixiang Xu Haifeng Lin Lei Wang Volodymyr Turkevych key Laboratory of Eco-chemical Engineering International S&T Cooperation Foundation of Eco-chemical Engineering and Green ManufactureCollege of Chemistry and Molecular EngineeringQingdao University of Science and TechnologyQingdao 266042China shandong Provincial key Laboratory of Olefin Catalysis and Polymerization Key Laboratory of Rubber-Plastics of Ministry of EducationSchool of Polymer Science and EngineeringQingdao University of Science and TechnologyQingdao 266042China V.Bakul Institute for Superhard Materials National Academy of Sciences of UkraineKyiv 04074Ukraine

Hollow semiconductor nanostructures with direct Z-scheme heterojunction have significant advantages for photocatalytic reactions,and optimizing the interfacial charge transmission of Z-scheme heterojunction is the hinge to achieve excellent solar conversion *** this work,tubular Ni_(1−x)Co_(x)S_(2)-CdS heterostructures with reinforced Z-scheme charge transmission were constructed through an In-metal-organic framework(MOF)templated *** Z-scheme charge transfer mechanism was sufficiently confirmed by combining density functional theory(DFT)calculation,X-ray photoelectron spectroscopy(XPS),surface photovoltage spectroscopy(SPV),and radical testing ***,the use of sodium citrate complexant contributes to the formation of intimate heterointerface,and the Fermi level gap between CdS and NiS_(2)is enlarged through Co doping into NiS_(2),which enhances the built-in electric field and photo-carriers transmission driving force for Ni_(1−x)Co_(x)S_(2)-CdS heterojunction,resulting in an evidently promoted activity toward H2 evolution reaction(HER).Under visible-light(λ>400 nm)irradiation,the Ni_(1−x)Co_(x)S_(2)-CdS composite with 10 mol%Co doping and 80 wt.%CdS(NC_(0.10)S-80%CdS)achieved an outstanding HER rate up to 35.94 mmol·g^(−1)·h^(−1)(corresponding to the apparent quantum efficiency of 34.7%at 420 nm),approximately 76.4 times that of 3 wt.%Pt-loaded CdS and it is much superior to that of most CdS-based photocatalysts ever ***,the good photocatalytic durability of Ni_(1−x)Co_(x)S_(2)-CdS heterostructures was validated by cycling and long-term HER *** work could inspire the development of high-performance Z-scheme heterojunction via optimizing the morphology and interfacial charge transmission.

关键词： tubular heterostructure Z-scheme charge transmission interfacial coupling built-in electric field visible-light photocatalysis

Quantification of the concrete freeze–thaw environment across the Qinghai–Tibet Plateau based on machine learning algorithms

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Journal of Mountain Science 2024年第1期21卷 322-334页

作者： QIN Yanhui MA Haoyuan ZHANG Lele YIN Jinshuai ZHENG Xionghui LI Shuo Department of Civil Engineering Qingdao University of TechnologyQingdao 266520China Department of Geography Qinghai Normal UniversityXining 810008China

The reasonable quantification of the concrete freezing environment on the Qinghai–Tibet Plateau(QTP) is the primary issue in frost resistant concrete design, which is one of the challenges that the QTP engineering managers should take into account. In this paper, we propose a more realistic method to calculate the number of concrete freeze–thaw cycles(NFTCs) on the QTP. The calculated results show that the NFTCs increase as the altitude of the meteorological station increases with the average NFTCs being 208.7. Four machine learning methods, i.e., the random forest(RF) model, generalized boosting method(GBM), generalized linear model(GLM), and generalized additive model(GAM), are used to fit the NFTCs. The root mean square error(RMSE) values of the RF, GBM, GLM, and GAM are 32.3, 4.3, 247.9, and 161.3, respectively. The R^(2) values of the RF, GBM, GLM, and GAM are 0.93, 0.99, 0.48, and 0.66, respectively. The GBM method performs the best compared to the other three methods, which was shown by the results of RMSE and R^(2) values. The quantitative results from the GBM method indicate that the lowest, medium, and highest NFTC values are distributed in the northern, central, and southern parts of the QTP, respectively. The annual NFTCs in the QTP region are mainly concentrated at 160 and above, and the average NFTCs is 200 across the QTP. Our results can provide scientific guidance and a theoretical basis for the freezing resistance design of concrete in various projects on the QTP.

关键词： Freeze–thaw cycles Quantification Machine learning algorithms Qinghai–Tibet Plateau Concrete

Transcriptome analysis reveals immune-related genes in tissues of Vibrio anguillarum-infected turbot Scophthalmus maximus

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Journal of Oceanology and Limnology 2024年第1期42卷 332-344页

作者： Yuting SONG Maqsood Ahmed SOOMRO Xianzhi DONG Guobin HU College of Marine Life Sciences Ocean University of ChinaQingdao 266003China Institute of Evolution&Marine Biodiversity Ocean University of ChinaQingdao 266003China Institute of Biophysis Chinese Academy of SciencesBeijing 100101China

Turbot Scophthalmus maximus is an important mariculture fish species with high economic ***,the bacterial diseases caused by Vibrio anguillarum infection bring huge economic losses to the turbot aquaculture *** understand the immune response of the turbot against *** infection and to explore novel immune-related genes,the transcriptome analysis of turbot spleen and gills were conducted after *** *** expressed genes(DEGs)were identified in spleen and gill of the turbot amounted to 17261 and 16436,respectively.A large number of immunerelated DEGs were enriched in cytokine-cytokine receptor interaction signaling pathway,and the others by the kyoto encyclopedia of genes and genomes(KEGG)*** gene ontology(GO)classification analysis revealed that *** infection had the greatest effect on biological processes and cellular *** immune-related DEGs were identified in the spleen(cstl.1,egfl6,lamb21,v2rx4,calcr,and gpr78a)and gills(ghra,sh3gl2a,cst12,inhbaa,cxcl8,and il-1b)by heat *** proteinprotein interaction(PPI)networks were constructed to analyze the immune *** results demonstrate that the maturation and antigen processing of major histocompatibility complex(MHC)class II molecule,and calcitonin-or adrenomedullin-regulated physiological activity were important events in the immunity of turbot against *** *** the gills,the protein interactions in TGF-βsignaling pathway,production of inflammatory factors,and endocytosis regulation were most *** research laid a foundation for discovering novel immune-related genes and enriching the knowledge of immune mechanisms of turbot against *** infection.

关键词： Scophthalmus maximus Vibrio anguillarum transcriptome differentially expressed genes immune mechanism

Development of the electric automatic steering system for agricultural vehicles

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International Journal of Agricultural and Biological Engineering 2024年第1期17卷 209-214页

作者： Guangshun An Chong Yu Juan Du Xiang Yin Youliang Ni Chengqian Jin School of Agricultural Engineering and Food Science Shandong University of TechnologyZibo 255000ShandongChina Nanjing research Institute for Agricultural Mechanization of Ministry of Agriculture and Rural Affairs Nanjing 210014China

Automatic guidance of agricultural vehicles requires automatic execution of operation commands received from the navigation controller by using electronically controlled mechanisms for wheel steering,speed changing and work *** steering contributes as a prerequisite technique in automatic and semi-automatic agricultural *** research aimed to develop an electric automatic steering system that was compact in its structure and integrated into original steering mechanism in a simply and convenient way for aftermarket modification.A brushless motor and reducer assembly was utilized to provide an adequate steering torque instead of manual maneuver.A rapid assembling approach was proposed by passing the steering shaft through the hollow output shaft.A digital proportional-integral-differential(PID)algorithm was implemented to calculate the rotation speeds and directions by comparing the desired angle and the actual angle,which was implemented in a printed circuit board with a microcontroller unit(MCU)and interface *** unmanned wheeled tractor was applied as test platform to integrate the newly developed electric automatic steering *** were conducted to evaluate its performance in terms of stability and *** autonomous navigation system guided the tractor along target paths in the field by sending steering commands to the electric automatic steering *** results show that the steering angle error was less than 0.81°when desired steering angle was less than 10°.The lateral error difference was no more than 4.76 cm when repeating following the same target path,which indicated that the electric automatic steering system responded accurately and robustly to steering commands.

关键词： automatic steering automatic navigation agricultural vehicles