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One-pot hydrothermal preparation of hierarchical manganese oxide nanorods for high-performance symmetric supercapacitors

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Journal of Energy Chemistry 2022年第2期31卷 116-126页

作者： Bidhan Pandit Emad S.Goda Mahmoud H.Abu Elella Aafaq ur Rehman Sang Eun Hong Sachin R.Rondiya Pranay Barkataki Shoyebmohamad F.Shaikh Abdullah M.Al-Enizi Salah MEl-Bahy Kuk Ro Yoon Department of Materials Science and Engineering and Chemical Engineering Universidad Carlos III de MadridAvenida de la Universidad 3028911 LeganésMadridSpain Organic Nanomaterials Lab Department of ChemistryHannam UniversityDaejeon 34054Republic of Korea Fire Protection Laboratory National Institute of Standards136Giza 12211Egypt Chemistry Department Faculty of ScienceCairo UniversityGiza 12613Egypt Graduate School of Energy Science and Technology Chungnam National University99 Daehak-roYuseong-guDaejeon 34134Republic of Korea School of Chemistry Cardiff UniversityMain BuildingPark PlaceCardiffCF103AT WalesUnited Kingdom Department of Physics Visvesvaraya National Institute of TechnologySouth Ambazari RoadNagpur-440010MaharashtraIndia Department of Chemistry College of ScienceKing Saud UniversityP.O.Box 2455Riyadh 11451Saudi Arabia Department of Chemistry Turabah University CollegeTaif UniversityP.O.Box 11099Taif 21944Saudi Arabia

An eco-friendly,new,and controllable approach for the preparation of manganese oxide(a-MnO_(2))nanorods has been introduced using hydrothermal reaction for supercapacitor *** in-depth crystal structure analysis ofα-MnO_(2) is analyzed by X-ray Rietveld refinement by using Full Prof program with the help of pseudo-Voigt profile *** developed a-MnO_(2) electrode attains a remarkable capacitance of 577.7 F/g recorded at a current density value of 1 A/g with an excellent cycle life when is used for 10,000 repeated cycles due to the porous nanorod-morphology assisting the ease penetration of electrolyte ions into the electroactive *** diffusive and capacitive contributions of the electrode have been estimated by considering standard numerical packages in *** successfully assembling the aqueous symmetric supercapacitor(SSC)cell by utilizing the as-preparedα-MnO_(2),an excellent capacitance of 163.5 F/g and energy density of 58.1 Wh/kg at the constant current density of 0.5 A/g are obtained with an expanded potential frame of 1.6 ***,the cell has exceptionally withstood up to 10,000 cycles with an ultimate capacitance retention of 94.1%including the ability to light an LED for 18 *** findings recommend the developed a-MnO_(2) electrode to be a highly felicitous electrode for the field of energy storage.

关键词： α-MnO_(2)nanorods Rietveld refinement Symmetrical supercapacitors High energy density

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The 4f-Hybridization Strength in Ce_(m)M_(n)In_(3m+2n) Heavy-Fermion Compounds Studied by Angle-Resolved Photoemission Spectroscopy

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Chinese Physics Letters 2021年第10期38卷 37-42页

作者： Jiao-Jiao Song Yang Luo Chen Zhang Qi-Yi Wu Tomasz Durakiewicz Yasmine Sassa Oscar Tjernberg Martin Mansson Magnus HBerntsen Yin-Zou Zhao Hao Liu Shuang-Xing Zhu Zi-Teng Liu Fan-Ying Wu Shu-Yu Liu Eric DBauer Ján Rusz Peter MOppeneer Ya-Hua Yuan Yu-Xia Duan Jian-Qiao Meng School of Physics and Electronics Central South UniversityChangsha 410083China Institute of Physics Maria Curie Sklodowska University20-031 LublinPoland Department of Physics and Astronomy Uppsala UniversityBox 516S-75120 UppsalaSweden Department of Physics Chalmers University of Technology41296 GoteborgSweden Department of Applied Physics KTH Royal Institute of TechnologyAlba Nova10691 StockholmSweden Condensed Matter and Magnet Science Group Los Alamos National LaboratoryLos AlamosNew Mexico 87545USA

We systemically investigate the nature of Ce 4f electrons in structurally layered heavy-fermion compounds Ce_(m)M_(n)In_(3m+2n)(with M=Co,Rh,Ir,and Pt,m=1,2,n=0–2),at low temperature using on-resonance angle-resolved photoemission *** heavy quasiparticle bands f^(0),f^(1/7/2)and f^(1/5/2),are observed in all compounds,whereas their intensities and energy locations vary greatly with *** strong f0 states imply that the localized electron behavior dominates the Ce 4f *** Ce 4f electrons are partially hybridized with the conduction electrons,making them have the dual nature of localization and *** quantitative comparison reveals that the f^(1/5/2)–f^(0)intensity ratio is more suitable to reflect the 4f-state hybridization strength.

关键词： spectroscopy materials strength

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