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How can technology and efficiency alleviate the dilemma of economic growth and carbon emissions in china's industrial economy? A metafrontier decoupling decomposition analysis

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Petroleum science 2024年第2期21卷 1415-1428页

作者： Miao Wang Chao Feng School of Business Zhengzhou UniversityZhengzhou450001HenanChina School of Economics and Business Administration Chongqing UniversityChongqing400030China

This paper attempts to explore the decoupling relationship and its drivers between industrial economic increase and energy-related CO_(2) emissions(ICE). Firstly, the decoupling relationship was evaluated by Tapio index. Then, based on the DEA meta-frontier theory framework which taking into account the regional and industrial heterogeneity and index decomposition method, the driving factors of decoupling process were explored mainly from the view of technology and efficiency. The results show that during2000-2019, weak decoupling was the primary state. Investment scale expansion was the largest reason hindering decoupling process of industrial increase from ICE. Both energy saving and production technology achieved significant progress, which facilitated the decoupling process. Simultaneously, the energy technology gap and production technology gap among regions have been narrowed, and played a role in promoting decoupling process. On the contrary, both scale economy efficiency and pure technical efficiency have inhibiting effects on decoupling process. The former indicates that the scale economy of china's industry was not conducive to improve energy efficiency and production efficiency, while the latter indicates that resource misallocation problem may exist in both energy market and product market.

关键词： china's industrial sector Decoupling process Meta-frontier DEA Index decomposition method Driving factors

Impact of well placement and flow rate on production efficiency and stress field in the fractured geothermal reservoirs

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Deep Underground science and Engineering 2024年第3期3卷 358-368页

作者： Xinghui Wu Meifeng Cai Xu Wu Ketong Zhang Ziqing Yin Yu Zhu School of City and Architecture Engineering Zaozhuang UniversityZaozhuangChina School of Civil and Resource Engineering University of Science and Technology BeijingBeijingChina Beijing Municipal Engineering Research Institute BeijingChina Department of Civil and Environmental Engineering University of StrathclydeGlasgowUK

Geothermal energy has gained wide attention as a renewable alternative for mitigating greenhouse gas *** advancements in enhanced geothermal system technology have enabled the exploitation of previously inaccessible geothermal ***,the extraction of geothermal energy from deep reservoirs poses many challenges due to high‐temperature and high‐geostress *** factors can significantly impact the surrounding rock and its fracture formation.A comprehensive understanding of the thermal–hydraulic–mechanical(THM)coupling effect is crucial to the safe and efficient exploitation of geothermal *** study presented a THM coupling numerical model for the geothermal reservoir of the Yangbajing geothermal *** proposed model investigated the geothermal exploitation performance and the stress distribution within the reservoir under various combinations of geothermal wells and mass flow *** geothermal system performance was evaluated by the criteria of outlet temperature and geothermal *** results indicate that the longer distance between wells can increase the outlet temperature of production wells and improve extraction efficiency in the short *** contrast,the shorter distance between wells can reduce the heat exchange area and thus mitigate the impact on the reservoir stress.A larger mass flow rate is conducive to the production capacity enhancement of the geothermal system and,in turn causes a wider range of stress *** findings provide valuable insights into the optimization of geothermal energy extraction while considering reservoir safety and long‐term *** study deepens the understanding of the THM coupling effects in geothermal systems and provides an efficient and environmentally friendly strategy for a geothermal energy system.

关键词： geothermal exploitation performance geothermal reservoir mass flow rate stress field well placementa

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A multifunctional electrolyte additive for zinc-ion capacitors with low temperature resistant and long lifespan

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Journal of Energy Chemistry 2024年第7期94卷 477-485页

作者： Ming Sun Zekai Zhang Shuqing Fu Yifan Zhang Ruoyu Wang Hongchun Mu Cheng Lian Wenqiang Wang Gengchao Wang Shanghai Engineering Research Center of Hierarchical Nanomaterials Shanghai Key Laboratory of Advanced Polymeric MaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Chemical Engineering Shanghai Engineering Research Center of Hierarchical NanomaterialsFrontiers Science Center for Materiobiology and Dynamic Chemistryand School of Chemistry and Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular ScienceFudan UniversityShanghai 200438China

Aqueous zinc-ion capacitors (ZICs) are considered as potential candidates for next generation electrochemical energy storage devices due to their high safety and low ***,the existing aqueous ZICs usually have the problems of zinc dendrite growth and unsatisfactory performance at low ***,an erythritol (Eryt) additive with inhibition of zinc dendrites and anti-freezing capability was introduced into the *** experimental characterization and theoretical calculation confirm that the Eryt adsorbed on the surface of zinc anodes regulates the deposition orientation of Zn^(2+) and inhibits the formation of *** also reconstructs the solvation structure in the electrolyte to reduce water activity,enabling the electrolyte to have a lower freezing point for operation at low *** the assistance of Eryt,the Zn||Zn symmetric cell exhibits a long cycle life of 2000 h,while the ZIC assembled with activated carbon (AC) cathode and zinc anode (Zn||AC) maintains a capacity retention of 98.2% after 30,000 cycles at a current density of 10 A g^(-1)(even after 10,000 cycles at-20°C,the capacity retention rate reached 94.8%.).This work provides a highly scalable,low-cost and effective strategy for the protection of the anodes of low-temperature aqueous ZICs.

关键词： Zinc-ioncapacitors Electrolyte additive Dendrite-free Freeze-resistant electrolyte

Boundary slip and lubrication mechanisms of organic friction modifiers with effect of surface moisture

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Friction 2024年第7期12卷 1483-1498页

作者： Xiaobin YI Haiyu XU Ge JIN Yang LU Biqiang CHEN Shaofeng XU Junqin SHI Xiaoli FAN State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsNorthwestern Polytechnical UniversityXi’an 710072China Xi’an Thermal Power Research Institute Co. Ltd.Xi’an 710054China NingboTech University Ningbo 315000China

Surface moisture or humidity impacting the lubrication property is a ubiquitous phenomenon in tribological systems,which is demonstrated by a combination of molecular dynamics(MD)simulation and experiment for the organic friction modifier(OFM)-containing *** stearic acid and poly-α-olefin 4cSt(PAO4)were chosen as the OFM and base oil molecules,*** physical adsorption indicates that on the moist surface water molecules are preferentially adsorbed on friction surface,and even make OFM adsorption film thoroughly leave surface and mix with base *** shear process,the adsorption of water film and desorption OFM film are further enhanced,particularly under higher shear *** simulated friction coefficient(that is proportional to shear rate)increases firstly and then decreases with thickening water film,in good agreement with experiments,while the slip length shows a contrary *** wear increases with humidity due to tribochemistry revealing the continuous formation and removal of Si–O–Si *** tribological discrepancy of OFM-containing lubricant in dry and humid conditions is attributed to the slip plane’s transformation from the interface between OFM adsorption film and lubricant bulk to the interface between adsorbed water *** work provides a new thought to understand the boundary lubrication and failure of lubricant in humid environments,likely water is not always harmful in oil lubrication systems.

关键词： organic friction modifier(OFM) boundary lubrication boundary slip surface moisture

Co-electrolysis of ethylene glycol and carbon dioxide for formate synthesis

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science china Chemistry 2024年第5期67卷 1539-1544页

作者： Dongfeng Du Fusong Kang Shiru Yang Bin Shao Jingshan Luo Institute of Photoelectronic Thin Film Devices and Technology State Key Laboratory of Photovoltaic Materials and CellsKey Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinMinistry of Education Engineering Research Center of Thin Film Photoelectronic TechnologyNankai UniversityTianjin 300350China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China Frontiers science Center for New Organic Matter Nankai UniversityTianjin 300071China College of Electronic Information and Optical Engineering Tianjin Key Laboratory of Optoelectronic Sensor and Sensing Network TechnologyNankai UniversityTianjin 300350China

Co-electrolysis of waste plastics and carbon dioxide(CO_(2)) into value-added chemicals or fuels is a promising pathway for a sustainable society, but efficient and selective conversion remains a challenge. Herein, a gold-mediated nickel hydroxide(Au/Ni(OH)_(2)) is developed to oxidize waste plastic-derived ethylene glycol(EG) into formate. In-situ electrochemical experiments and theoretical results reveal that the introduction of Au favors the redox properties and EG adsorption behavior of Ni(OH)_(2). The Au/Ni(OH)_(2) catalyst shows an excellent formate selectivity of >90% at high current densities of above 100 m A cm^(-2). When coupled with sputtered bismuth(Bi) cathode for CO_(2) reduction, a high formate Faradic efficiency(FE) of 188.2% at 200 m A cm^(-2)and a good formate productivity of 7.33 mmol m^(-2)s^(-1)at 10 A are obtained in a flow cell and a zero-gap membrane electrode assembly(MEA) cell, respectively. This work demonstrates a promising strategy to convert waste plastics and CO_(2) into valuable products.

关键词： waste plastic upcycling ethylene glycol oxidation carbon dioxide reduction electrocatalysis formate synthesis

Microlensing bias on the detection of strong lensing gravitational wave

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science china(Physics,Mechanics & Astronomy) 2024年第6期67卷 156-165页

作者： Xikai Shan Xuechun Chen Bin Hu Guoliang Li Institute for Frontier in Astronomy and Astrophysics Beijing Normal UniversityBeijing 102206China Department of Astronomy Beijing Normal UniversityBeijing 100875China Purple Mountain Observatory Chinese Academy of SciencesNanjing 210023China

Identifying strong lensing gravitational wave(SLGW)events is of utmost importance in astrophysics as we approach the historic first detection of SLGW amidst the growing number of gravitational wave(GW)***,one crucial method for identifying SLGW signals involves assessing the overlap of parameters between two ***,the distribution of discrete matter,such as stars and sub-halos,within the strong lensing galaxy can imprint a wave optical(WO)effect on the SLGW *** frequency dependent imprints introduce biases in parameter estimation and impact SLGW *** this study,we assess the influence of the stellar microlensing field embedded in a strong lensing *** findings demonstrate that the WO effect reduces the detection efficiency of SLGW by 5%-50%for various false alarm probabilities per pair(FAPper pair).Specifically,at an FAPper pairof 10^(-5),the detection efficiency decreases from~10%to~5%.Consequently,the presence of the microlensing field can result in missing half of the strong lensing ***,the microlensing WO effect introduces a noticeable bias in intrinsic parameters,particularly for chirp mass and mass ***,it has tiny influence on extrinsic *** all parameters,~30%of events exhibit a 1σparameter bias,~12%exhibit a 2σparameter bias,and~5%exhibit a 3σparameter bias.

关键词： gravitational wave gravitational strong lensing gravitational micro lensing wave optical effect

Electrostatic Interaction-directed Construction of Hierarchical Nanostructured Carbon Composite with Dual Electrical Conductive Networks for Zinc-ion Hybrid Capacitors with Ultrastability

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Energy & Environmental Materials 2024年第1期7卷 188-196页

作者： Changyu Leng Zongbin Zhao Xuzhen Wang Yuliya V.Fedoseeva Lyubov G.Bulusheva Alexander V.Okotrub Jian Xiao Jieshan Qiu State Key Lab of Fine Chemicals School of Chemical Engineering Liaoning Key Lab for Energy Materials and Chemical Engineering Dalian University of Technology Nikolaev Institute of Inorganic Chemistry Siberian Branch of the Russian Academy of Sciences College of Chemical Engineering Beijing University of Chemical Technology

Metal-organic framework(MOF)-derived carbon composites have been considered as the promising materials for energy ***,the construction of MOF-based composites with highly controllable mode via the liquid-liquid synthesis method has a great challenge because of the simultaneous heterogeneous nucleation on substrates and the self-nucleation of individual MOF nanocrystals in the liquid phase.

关键词： carbon composite electrostatic interaction metal–organic framework coating self-assembly zinc-ion hybrid capacitor

Fracture sealing performance of granular lost circulation materials at elevated temperature:A theoretical and coupled CFD-DEM simulation study

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Petroleum science 2024年第1期21卷 567-581页

作者： Chong Lin Qi-Cong Xu Lie-Xiang Han Gao Li Hai He Hong-Ling Zhou Ji-Ping She CCDC Drilling&Production Technology Research Institute Guanghan618300SichuanChina State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500SichuanChina College of Materials science and Engineering Chongqing UniversityChongqing400044China State Key Lab of Oil and Gas Reservoir Geology and Exploitation(Chengdu University of Technology) Chengdu610059SichuanChina College of Energy Chengdu University of TechnologyChengdu610059SichuanChina

Lost circulation is a common downhole problem of drilling in geothermal and high-temperature,high-pressure(HTHP)*** circulation material(LCM)is a regular preventive and remedial measure for lost ***,conventional LCMs seem ineffective in high-temperature *** may be due to the changes in the mechanical properties of LCMs and their sealing performance under high-temperature *** understand how high temperature affects the fracture sealing performance of LCMs,we developed a coupled computational fluid dynamics-discrete element method(CFD-DEM)model to simulate the behavior of granular LCMs in *** summarized the literature on the effects of high temperature on the mechanical properties of LCMs and the rheological properties of drilling *** conducted sensitivity analyses to investigate how changing LCM slurry properties affected the fracture sealing efficiency at increasing *** results show that high temperature reduces the size,strength,and friction coefficient of LCMs as well as the drilling fluid ***,softer,and less frictional LCM particles have lower bridging probability and slower bridging *** particles tend to form dual-particle bridges rather than single-particle *** result in a deeper,tighter,but unstable sealing *** drilling fluid viscosity leads to faster and shallower sealing zones.

关键词： Geothermal well drilling HTHP formationLost circulation material CFD-DEM Fracture sealing

Lamellar quasi-solid electrolyte with nanoconfined deep eutectic solvent for high-performance lithium battery

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Nano Research 2024年第7期17卷 6176-6183页

作者： Shiwei Liu Jing Wang Keqi Wu Zhirong Yang Yan Dai Junmei Zhang Wenjia Wu Jingtao Wang School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China

Electrolytes with high-efficiency lithium-ion transfer and reliable safety are of great importance for lithium *** having superior ionic conductivity(10^(−3)–10^(−2) S·cm^(−1)),traditional liquid-state electrolytes always suffer from low lithium-ion transference number(tLi+<0.4)and thus undesirable battery ***,the deep eutectic solvent(DES)is vacuum-filtered into the~1 nm interlayer channel of vermiculite(Vr)lamellar framework to fabricate a quasi-solid electrolyte(Vr-DES QSE).We demonstrate that the nanoconfinement effect of interlayer channel could facilitate the opening of solvation shell around ***,the interaction from channel wall could inhibit the movement of *** enable high-efficiency lithium-ion transfer:2.61×10^(−4)S·cm^(−1)at 25℃.Importantly,the tLi+value reaches 0.63,which is 4.5 times of that of bulk DES,and much higher than most present liquid/quasi-solid *** addition,Vr-DES QSE shows significantly improved interfacial stability with Li anode as compared with *** assembled Li symmetric cell can operate stably for 1000 h at 0.1 mA·cm^(−2).The lithium iron phosphate(LFP)|Vr-DES QSE|Li cell exhibits high capacity of 142.1 mAh·g^(−1)after 200 cycles at 25℃ and 0.5 C,with a capacity retention of 94.5%.The strategy of open solvation shell through nanoconfinement effect of lamellar framework may shed light on the development of advanced electrolytes.

关键词： quasi-solid electrolyte deep eutectic solvent lamellar structure lithium-ion transference number solvation shell