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Enhanced post-combustion CO2 capture and direct air capture by plasma surface functionalization of graphene adsorbent

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Journal of Energy Chemistry 2025年第1期100卷 653-664页

作者： Rahul Navik Eryu Wang Xiao Ding Huang Yunyi Yiyu Liu Jia Li Guangdong-Hong Kong Joint Laboratory for Carbon Neutrality Jiangmen Laboratory of Carbon and Science and Technology Guangzhou HKUST Fok Ying Tung Research Institute The Hong Kong University of science and Technology (Guangzhou) Carbon Neutrality and Climate Change Thrust Society Hub The Hong Kong University of Science and Technology (Guangzhou) Stoddart Institute of Molecular science Department of Chemistry Zhejiang University

Graphene has enormous potential to capture CO2due to its unique properties and ***,graphene-based adsorbents have drawbacks of lower CO2adsorption capacity and poor *** work demonstrates a one-step rapid and sustainable N2/H2plasma treatment process to prepare graphene-based sorbent material with enhanced CO2adsorption *** treatment directly enriches amine species,increases surface area,and improves textural *** CO2adsorption capacity increases from 1.6 to 3.3 mmol/g for capturing flue gas,and from 0.14 to 1.3 mmol/g for direct air capture （DAC）.Importantly,the electrothermal property of the plasma-modified aerogels has been significantly improved,resulting in faster heating rates and significantly reducing energy consumption compared to conventional external heating for regeneration of *** aerogels display improved selectivity of 42 and 87 after plasma modification for 5 and 10 min,*** plasma-treated aerogels display minimal loss between 17%and 19% in capacity after 40 adsorption/desorption cycles,rendering excellent *** N2/H2plasma treatment of adsorbent materials would lower energy expenses and prevent negative effects on the global economy caused by climate change.

关键词： Carbon neutrality CO 2 capture Climate change Plasma treatment Graphene aerogel

Dynamically self-adjustable liquid-liquid and self-adaptive softcontact solid-solid triboelectric nanogenerator for wave energy harvesting

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Nano Research 2025年第1期18卷 404-414页

作者： Yong Long Bingqi Zhao Jianan Niu Yuxiu Liu Wei Sha Jiangwen Wang Zhong Lin Wang Weiguo Hu Guangzhou Institute of Blue Energy Knowledge CityHuangpu DistrictGuangzhou 510555China beijing Institute of Nanoenergy and Nanosystems Chinese Academy of SciencesBeijing 101400China School of Nanoscience and Technology University of Chinese Academy of SciencesBeijing 100049China

Water wave energy exhibits great potential toalleviate the global energy crisis. However, harvesting andutilizing wave energy are challenging due to its irregularity,randomness, and low frequency. Triboelectric nanogenerators(TENGs) have gained significant attention for harvesting waveenergy with high efficiency. This study presents a novelellipsoidal, pendulum-like TENG integrating both liquid-liquid(L-L) and solid-solid (S-S) triboelectricity (LS-TENG). Thisinnovative design enables continuous wave energy harvestingand self-powered marine environment monitoring under variousconditions, including temperature, humidity, and light intensity. The binary immiscible liquids within the LS-TENG’s innersoft balloon create dynamic, and self-adjustable L-L contact interfaces, significantly increasing the L-L contact area andenhancing L-L contact electrification (CE). The unique self-adaptive, soft S-S contact increases the S-S contact areacompared to traditional hard point contact, better adapting to the irregular movements of waves and promoting efficient S-SCE. The LS-TENG achieves highly efficient wave energy harvesting by coupling L-L and S-S CE. Furthermore, the uniquesoft contact design protects the S-S interfaces from mechanical wear and damage during long-term work. The LS-TENG’snovel structure provides an innovative and effective way for water wave energy harvesting.

关键词： self-adaptive soft-contact solid-solid liquid-liquid self-adjustable triboelectric nanogenerator

Enhanced electrochemical CO_(2)reduction coupled with urea oxidation using bifunctional atomically dispersed CuNi catalysts

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Nano Research 2025年第1期18卷 208-216页

作者： Wenjie Wu Haoyang Zhou Ying Liu Yifei Pan Qingqing Chen Yu Zhang Junjie Mao Wenjie Ma Ping Yu beijing National Laboratory for Molecular sciences Key Laboratory of Analytical Chemistry for Living BiosystemsInstitute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China College of Chemistry and Materials science Anhui Normal UniversityWuhu 241002China University of Chinese Academy of sciences Beijing 100049China

The electrochemical conversion of carbon dioxide(CO_(2))into chemical fuels represents a promising approach for addressing global carbon balance ***,this process is hindered by the kinetic limitations of anodic reactions,usually the oxygen evolution reaction,resulting in less efficient production of high value-added ***,we report an integrated electrocatalytic system that couples CO_(2)reduction reaction(CO_(2)RR)with urea oxidation reaction(UOR)using a bifunctional electrocatalyst with atomically dispersed dual-metal CuNi sites anchored on bamboo-like nitrogen-doped carbon nanotubes(CuNi-CNT),which were synthesized through a one-step pyrolysis *** bifunctional CuNi-CNT catalyst exhibits a near 100%CO Faraday efficiency for CO_(2)RR over a wide potential range and outstanding UOR performance with a negatively shifted potential of 210 mV at 10 mA·cm^(-2).In addition,we assemble a two-electrode electrolyzer using bifunctional CuNi-CNT-modified carbon fiber paper electrodes as both cathode and anode,capable of operating at a remarkably low cell voltage of 1.81 V at 10 mA·cm-2,significantly lower than conventional *** study provides a novel avenue to achieving an efficient carbon cycle with reduced electric power consumption.

关键词： electrochemical conversion bimetallic site catalyst bifunctional electrocatalyst carbon dioxide reduction urea oxidation

Catalyst–support Interaction in Polyaniline‑supported Ni_(3)Fe Oxide to Boost Oxygen Evolution Activities for Rechargeable Zn‑Air Batteries

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Nano-Micro Letters 2025年第1期17卷 176-190页

作者： Xiaohong Zou Qian Lu Mingcong Tang Jie Wu Kouer Zhang Wenzhi Li Yunxia Hu Xiaomin Xu Xiao Zhang Zongping Shao Liang An Department of Mechanical Engineering The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control Jiangsu Collaborative Innovation Center of Atmospheric Environment and Equipment TechnologySchool of Environmental Science and TechnologyNanjing University of Information Science and TechnologyNanjing 210044People’s Republic of China Department of Chemistry The Chinese University of Hong KongMa Lin BuildingShatinHong Kong SAR 999077People’s Republic of China WA School of Mines:Minerals Energy and Chemical Engineering(WASM‑MECE)Curtin UniversityPerthWA 6102Australia Research Institute for Advanced Manufacturing The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloonHong Kong SARPeople’s Republic of China

Catalyst–support interaction plays a crucial role in improving the catalytic activity of oxygen evolution reaction(OER).Here we modulate the catalyst–support interaction in polyaniline-supported Ni_(3)Fe oxide(Ni_(3)Fe oxide/PANI)with a robust hetero-interface,which significantly improves oxygen evolution activities with an overpotential of 270 mV at 10 mA cm^(-2)and specific activity of 2.08 mA cm_(ECSA)^(-2)at overpotential of 300 mV,3.84-fold that of Ni_(3)Fe *** is revealed that the catalyst–support interaction between Ni_(3)Fe oxide and PANI support enhances the Ni–O covalency via the interfacial Ni–N bond,thus promoting the charge and mass transfer on Ni_(3)Fe *** the excellent activity and stability,rechargeable Zn-air batteries with optimum Ni_(3)Fe oxide/PANI are assembled,delivering a low charge voltage of 1.95 V to cycle for 400 h at 10 mA cm^(-2).The regulation of the effect of catalyst–support interaction on catalytic activity provides new possibilities for the future design of highly efficient OER catalysts.

关键词： Catalyst-support interaction supported catalysts Heterointerface Oxygen evolution reaction Zn-air batteries

Recent Advances in Fibrous Materials for Hydroelectricity Generation

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Nano-Micro Letters 2025年第2期17卷 109-133页

作者： Can Ge Duo Xu Xiao Feng Xing Yang Zheheng Song Yuhang Song Jingyu Chen Yingcun Liu Chong Gao Yong Du Zhe Sun Weilin Xu Jian Fang College of Textile and Clothing Engineering Soochow UniversitySuzhou 215123People’s Republic of China National Engineering Laboratory for Modern Silk Soochow UniversitySuzhou 215123People’s Republic of China State Key Laboratory of New Textile Materials and Advanced Processing Technologies Wuhan Textile UniversityWuhan 430200People’s Republic of China Institute of Functional Nano&Soft Materials(FUNSOM) Soochow UniversitySuzhou 215123People’s Republic of China Department of Electrical and Computer Engineering University of MassachusettsAmherstMA 01003USA Department of Materials Imperial College LondonSouth Kensington CampusLondon SW72AZUK College of Textile science and Engineering Zhejiang Sci-Tech UniversityHangzhou 310018People’s Republic of China School of Materials science and Engineering Shanghai Institute of Technology100 Haiquan RoadShanghai 201418People’s Republic of China

Depleting fossil energy sources and conventional polluting power generation pose a threat to sustainable *** generation from ubiquitous and spontaneous phase transitions between liquid and gaseous water has been considered a promising strategy for mitigating the energy *** materials with unique flexibility,processability,multifunctionality,and practicability have been widely applied for fibrous materials-based hydroelectricity generation(FHG).In this review,the power generation mechanisms,design principles,and electricity enhancement factors of FHG are first ***,the fabrication strategies and characteristics of varied constructions including 1D fiber,1D yarn,2D fabric,2D membrane,3D fibrous framework,and 3D fibrous gel are ***,the advanced functions of FHG during water harvesting,proton dissociation,ion separation,and charge accumulation processes are analyzed in ***,the potential applications including power supply,energy storage,electrical sensor,and information expression are also ***,some existing challenges are considered and prospects for future development are sincerely proposed.

关键词： Hydroelectricity Fibrous material Streaming potential Ion diffusion

Feasibility evaluation of failure models for predicting forming limit of metal foils

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Chinese Journal of Aeronautics 2020年第9期33卷 2461-2471页

作者： Bao MENG Jiejie SHI Yiyun ZHANG Cheng CHENG Bolin MA Min WAN School of Mechanical Engineering and Automation Beihang UniversityBeijing 100083China

Forming limit of metal foil is an important index to evaluate its formability,and is of considerable significance to improve the quality of *** ductile fracture(DF)behavior in microscale plastic deformation is remarkably affected by the geometry and grain *** explore the size-dependent forming limit curve(FLC),the Holmberg and Marciniak tests of SUS304 foils with the thicknesses of less than 0.1 mm and diverse grain sizes were *** addition,the validity and feasibility of three types of existing failure models including Swift/Hill,MarciniakKuczynski(M-K)and DF criteria for predicting the micro-scaled FLCs were *** is found that the Swift/Hill model possesses the worst accuracy with predicting deviation above 50%.Four classical DF criteria including Freudenthal,Ayada,Brozzo and Oh show great difference,and Oh model considering plastic anisotropy presents the best *** predicted deviation of M-K model is aggravated with increasing grain size and decreasing foil thickness,which is attributed to the intensified free surface roughening and transformation of fracture mechanism with *** research thus provides a deeper understanding and valuable reference for the widespread application of FLC in microforming.

关键词： Failure criteria Forming limit Metal foil Microforming Size effect

Design, Characterization, and 3D Printing of Cardiovascular Stents with Zero Poisson’s Ratio in Longitudinal Deformation

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Engineering 2021年第7期7卷 979-990页

作者： Chengjin Wang Lei Zhang Yongcong Fang Wei Sun Biomanufacturing Center Department of Mechanical EngineeringTsinghua UniversityBeijing 100084China Biomanufacturing and Rapid Forming Technology Key Laboratory of beijing Beijing 100084China “Biomanufacturing and Engineering Living Systems”Innovation International Talents Base(111 Base) Beijing 100084China Department of Mechanical Engineering Drexel UniversityPhiladelphiaPA 19104USA

Inherent drawbacks associated with drug-eluting stents have prompted the development of bioresorbable cardiovascular *** manufacturing(3-dimentional(3D)printing)has been widely applied in medical *** this study,we develop a novel screw extrusion-based 3D printing system with a new designed mini-screw extruder to fabricate stents.A stent with a zero Poisson’s ratio(ZPR)structure is designed,and a preliminary monofilament test is conducted to investigate appropriate fabrication parameters.3D-printed stents with different geometric structures are fabricated and analyzed by observation of the surface *** evaluation of the mechanical properties and a preliminary biological evaluation of 3D-printed stents with different parameters are carried *** conclusion,the screw extrusion-based 3D printing system shows potential for customizable stent fabrication.

关键词： Additive manufacturing 3D printing Screw extrusion Cardiovascular stent Zero Poisson’s ratio

Study on jet formation behavior and optimization of trunconical hypercumulation shaped charge structure

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Defence Technology（防务技术） 2023年第3期21卷 196-206页

作者： Chao Ge Zhuojun Qu Jin Wang Die Hu Yong Zhang School of Mechatronical Engineering Beijing Institute of TechnologyBeijing100081China

Combining the methods of theoretical,numerical and experimental,this research focuses on the jet formation behavior and optimization of trunconical hypercumulation shaped charge *** the three-stage division,formation theory of trunconical hypercumulation shaped charge jet is established based on micro element *** dimensional analysis,main control parameters are identified and their effect on jet formation are *** numerical modelling and orthogonal optimization method,influence of the factors and their levels over the indicators of jet tip velocity and jet length as well as order of the significance of each factor and level are *** experiments of trunconical hypercumulation shaped charge based on the orthogonal optimization reveals its advantage over traditional conical shaped charge structure,and finally determines the optimal influence factor level *** research and results would provide useful guide for the design and application of trunconical hypercumulation shaped charge structure.

关键词： structure shaped charge

Angiotensin-converting enzyme 2(ACE2):SARS-CoV-2 receptor and RAS modulator

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Acta Pharmaceutica Sinica B 2021年第1期11卷 1-12页

作者： Jingwei Bian Zijian Li Department of Cardiology and Institute of Vascular Medicine Peking University Third HospitalKey Laboratory of Cardiovascular Molecular Biology and Regulatory PeptidesMinistry of HealthKey Laboratory of Molecular Cardiovascular SciencesMinistry of EducationBeijing Key Laboratory of Cardiovascular Receptors ResearchBeijing 100191China Department of Pharmacy Peking University Third HospitalBeijing 100191China

The coronavirus disease 2019(COVID-19)outbreak is caused by severe acute respiratory syndrome coronavirus 2(SARS-CoV-2).Angiotensin-converting enzyme 2(ACE2)was rapidly identified as the critical functional receptor for ***2 is well-known as a counter-regulator of the renin-angiotensin system(RAS)and plays a key role in the cardiovascular *** that ACE2 functions as both a SARS-CoV-2 receptor and a RAS modulator,the treatment for COVID-19 presents a dilemma of how to limit virus entry but protect ACE2 physiological ***,an in-depth summary of the recent progress of ACE2 research and its relationship to the virus is urgently needed to provide possible solution to the ***,we summarize the complexity and interplay between the coronavirus,ACE2 and RAS(including anti-RAS drugs).We propose five novel working modes for functional receptor for SARS-CoV-2 infection and the routes of ACE2-mediated virus entering host cells,as well as its regulatory *** the controversy of anti-RAS drugs application,we also give theoretical analysis and discussed for drug *** will contribute to a deeper understanding of the complex mechanisms of underlying the relationship between the virus and ACE2,and provide guidance for virus intervention strategies.

关键词： SARS-CoV-2 Angiotensin-converting enzyme 2 Renin-angiotensin system Receptor Modulator COVID-19 Anti-RAS drug Drug target