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Journal of Rare Earths 2024年第5期42卷 987-994,I0006页

作者： Dongsheng Zhao Wenqian Li Rongmei Wen Wencui Li Xin Liu Xiutang Zhang Liming Fan Shanxi Key Laboratory of Advanced Carbon Electrode Materials Shanxi Coal Mine Water Treatment Technology Innovation CenterSchool of Chemistry and Chemical EngineeringNorth University of ChinaTaiyuan030051China Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education) College of ChemistryNankai UniversityTianjin300071China

By anchoring Tb^(3+)ions on its free carboxyl groups of the nanocaged NiMOF,a dual-emission self-calibrating sensor of Tb^(3+)@NiMOF was fabricated through coordination post-synthetic modification(PSM)*** Tb^(3+)ions as the secondary fluorescent signal and sensing active sites,Tb^(3+)@NiMOF presents great potentials in visually and efficiently monitoring EPI in serum,with high sensitivity and selectivity,fast response,excellent recyclable,and the low detection limit(LOD,3.06 ng/mL).Furthermore,a tandem combinational logic gate based intelligent detection system was constructed to improve the practicability and convenience of epinephrine(EPI)detection in serum by comparing the light emitted colour with the series standard colour cards preset in the *** work provides a promising approach of developing metal-organic frameworks(MOFs)based self-calibrating sensors for intelligent detection of bioactive molecules.

关键词： Metal-organic framework Post-synthetic modification Self-calibrating sensor Logic gate operation Epinephrine detection Rare earths

Hybrid electromechanical properties of hetero-doped and homogeneously bonded dual-mode pressure sensor for indoor body area network node

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Science china(Information Sciences) 2024年第1期67卷 240-253页

作者： Junbin YU Shuai XIAN Jinbiao MU Min WANG Yin WANG Xiaojuan HOU Le ZHANG Jian HE Jiliang MU Xiujian CHOU Science and Technology on Electronic Test and Measurement Laboratory North University of China Sichuan Aerospace Fenghuo Servo Control Technology Corporation

Pressure sensors are considerably important for continuous monitoring of human movement and the surrounding environment to construct a caregiving system for the elderly living *** challenge for pressure sensors that still remains is combining self-driven,comfort,and ***,an all-in-one conformal pressure sensor(ACPS) based on a homogeneous integrated triboelectric-piezoelectric hybrid sensor is *** ACPS has dual-mode sensing properties due to coupling triboelectrification and piezoelectric effect ensuring a stable response to various external ***-coated glass microspheres and polyacrylonitrile were uniformly filleted into the silicone rubber substrate using a hetero-doping method to create a stretchable electrode layer with flexible conformal characteristics and a piezoelectric layer with excellent piezoelectric properties,***,the triboelectric layer was fabricated using the same silicone rubber,allowing ACPS to be homogeneously bonded into an all-in-one structure with reliable *** allowed various functional layers to have outstanding interface characteristics and thus improve the electrical transmission *** developed ACPS had outstanding sensitivity(1.04 V/104Pa),high linearity(about 0.984),a wide measurement range(10–700 k Pa),and can accurately and continuously distinguish multiple ***,using a homemade signal processing circuit,ACPSs can be deployed in the human body and the room as indoor body area network *** successfully applied to the remote tracking of daily dynamic home life and the remote operation of small electrical equipment,these ACPSs can achieve real-time caregiving for the elderly living *** an application area desperately needed by society,this study envisions a caregiving system for the elderly living alone without violating personal privacy.

关键词： dual-mode pressure sensor homogeneous bonding all-in-onestructure indoor body area network node elderly caregiving microsystem

A proteomic landscape of pharmacologic perturbations for functional relevance

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Journal of Pharmaceutical Analysis 2024年第1期14卷 128-139页

作者： Zhiwei Liu Shangwen Jiang Bingbing Hao Shuyu Xie Yingluo Liu Yuqi Huang Heng Xu Cheng Luo Min Huang Minjia Tan Jun-Yu Xu State Key Laboratory of Drug Research Shanghai Institute of Materia MedicaChinese Academy of SciencesShanghai201203China School of Chinese Materia Medica Nanjing University of Chinese MedicineNanjing210023China Zhongshan Institute for Drug Discovery Shanghai Institute of Materia MedicaChinese Academy of SciencesZhongshanGuangdong528400China State Key Laboratory of Pharmaceutical Biotechnology Nanjing UniversityNanjing210023China

Pharmacological perturbation studies based on protein-level signatures are fundamental for drug discovery. In the present study, we used a mass spectrometry (MS)-based proteomic platform to profile the whole proteome of the breast cancer MCF7 cell line under stress induced by 78 bioactive compounds. The integrated analysis of perturbed signal abundance revealed the connectivity between phenotypic behaviors and molecular features in cancer cells. Our data showed functional relevance in exploring the novel pharmacological activity of phenolic xanthohumol, as well as the noncanonical targets of clinically approved tamoxifen, lovastatin, and their derivatives. Furthermore, the rational design of synergistic inhibition using a combination of histone methyltransferase and topoisomerase was identified based on their complementary drug fingerprints. This study provides rich resources for the proteomic landscape of drug responses for precision therapeutic medicine.

关键词： Proteomics Drug Perturbation Drug target Drug combination

Roadmap for rechargeable batteries:present and beyond

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Science china Chemistry 2024年第1期67卷 13-42页

作者： Sen Xin Xu Zhang Lin Wang Haijun Yu Xin Chang Yu-Ming Zhao Qinghai Meng Pan Xu Chen-Zi Zhao Jiahang Chen Huichao Lu Xirui Kong Jiulin Wang Kai Chen Gang Huang Xinbo Zhang Yu Su Yao Xiao Shu-Lei Chou Shilin Zhang Zaiping Guo Aobing Du Guanglei Cui Gaojing Yang Qing Zhao Liubing Dong Dong Zhou Feiyu Kang Hu Hong Chunyi Zhi Zhizhang Yuan Xianfeng Li Yifei Mo Yizhou Zhu Dongfang Yu Xincheng Lei Jianxiong Zhao Jiayi Wang Dong Su Yu-Guo Guo Qiang Zhang Jun Chen Li-Jun Wan CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China university of Chinese Academy of Sciences.Beijing 100049 China Institute of Advanced Battery Materials and Devices Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China Key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of TechnologyBeijing 100124China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China State Key Laboratory of Chemistry and Utilization of Carbon-Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChangchun 130022China Institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China School of Chemical Engineering and Advanced Materials The University of AdelaideAdelaide 5000Australia Qingdao Industrial Energy Storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Frontiers Science Center for New Organic Matter Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China College of Chemistry and Materials Science Jinan UniversityGuangzhou 511443China Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen 518055China Department of Materials Science and Engineering City University of Hong KongHong Kong 999077China Division of Energy Storage Dalian National Laboratory for Clean Energy(DNL)Dalian Institute of Chem

Rechargeable batteries currently hold the largest share of the electrochemical energy storage market,and they play a major role in the sustainable energy transition and industrial decarbonization to respond to global climate *** to the increased popularity of consumer electronics and electric vehicles,lithium-ion batteries have quickly become the most successful rechargeable batteries in the past three decades,yet growing demands in diversified application scenarios call for new types of rechargeable *** efforts are made to developing the next-generation post-Li-ion rechargeable batteries,which include,but are not limited to solid-state batteries,lithium–sulfur batteries,sodium-/potassium-ion batteries,organic batteries,magnesium-/zinc-ion batteries,aqueous batteries and flow *** the great achievements,challenges persist in precise understandings about the electrochemical reaction and charge transfer process,and optimal design of key materials and interfaces in a *** roadmap tends to provide an overview about the current research progress,key challenges and future prospects of various types of rechargeable *** computational methods for materials development,and characterization techniques will also be discussed as they play an important role in battery research.

关键词： energy storage rechargeable batteries battery materials electrochemistry

A multiscale transform denoising method of the bionic polarized light compass for improving the unmanned aerial vehicle navigation accuracy

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Chinese Journal of Aeronautics 2022年第4期35卷 400-414页

作者： Donghua ZHAO Jun TANG Xindong WU Jing ZHAO Chenguang WANG Chong SHEN Jun LIU Key Laboratory of Instrumentation Science&Dynamic Measurement Ministry of EducationSchool of Instrument and ElectronicsNorth University of ChinaTaiyuan 03005JPR China School of Information and Communication Engineering North University of ChinaTaiyuan 030051PR China

In recent years, the bionic polarized light compass has been widely studied for the unmanned aerial vehicle navigation. However, it is found from the obtained investigation results that a polarized light compass with a sensitive and high dynamic range polarimeter still provides inferior output precision of the heading angle due to the presence of the noise generating from the *** noise is existed not only in the angle of the polarization image acquired by polarimeters but also in the output heading data, which leads to a sharp reduction in the accuracy of a polarized light compass. Herein, we present noise analysis and a novel multiscale transform denoising method of a polarized light compass used for the unmanned aerial vehicle navigation. Specifically, a multiscale principle component analysis utilizing one-dimensional image entropy as classification criterion is directly implemented to suppress the noise in the acquired polarization image. Subsequently, a multiscale time–frequency peak filtering method using the sample entropy as classification criterion is applied for the output heading data so as to further increase the heading measurement accuracy from the denoised image above. These two approaches are combined to significantly reduce the heading error affected by different types of noises. Our experimental results indicate the proposed multiscale transform denoising method exhibits high performance in suppressing the noise of a polarized light compass used for the unmanned aerial vehicle navigation compared to existing prior arts.

关键词： Denoising Multi-scale transform Orientation Polarized light compass UAV navigation

Synergistic piezoelectricity enhanced BaTiO_(3)/polyacrylonitrile elastomer-based highly sensitive pressure sensor for intelligent sensing and posture recognition applications

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Nano Research 2023年第4期16卷 5490-5502页

作者： Junbin Yu Shuai Xian Zhenpeng Zhang Xiaojuan Hou Jian He Jiliang Mu Wenping Geng Xiaojun Qiao Le Zhang Xiujian Chou Science and Technology on Electronic Test and Measurement Laboratory North University of ChinaTaiyuan 030051China

Designing stretchable and skin-conformal self-powered sensors for intelligent sensing and posture recognition is ***,based on a multi-force mixing and vulcanization process,as well as synergistically piezoelectricity of BaTiO_(3)and polyacrylonitrile,an all-in-one,stretchable,and self-powered elastomer-based piezo-pressure sensor(ASPS)with high sensitivity is *** ASPS presents excellent sensitivity(0.93 V/104 Pa of voltage and 4.92 nA/104 Pa of current at a pressure of 10-200 kPa)and high durability(over 10,000 cycles).Moreover,the ASPS exhibits a wide measurement range,good linearity,rapid response time,and stable frequency *** components were fabricated using silicone,affording satisfactory skinconformality for sensing *** cooperation with a homemade circuit and artificial intelligence algorithm,an information processing strategy was proposed to realize intelligent sensing and *** home-made circuit achieves the acquisition and wireless transmission of ASPS signals(transmission distance up to 50 m),and the algorithm realizes the classification and identification of ASPS signals(accuracy up to 99.5%).This study proposes not only a novel fabrication method for developing self-powered sensors,but also a new information processing strategy for intelligent sensing and recognition,which offers significant application potential in human-machine interaction,physiological analysis,and medical research.

关键词： flexible pressure sensor synergistic piezoelectricity all-in-one structure high sensitivity intelligent sensing and recognition

A non-contact flexible pyroelectric sensor for wireless physiological monitoring system

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Science china(Information Sciences) 2022年第2期65卷 162-172页

作者： Jian HE Sen LI Xiaojuan HOU Yongjun ZHOU Hao LI Min CUI Tao GUO Xiangdong WANG Jiliang MU Wenping GENG Xiujian CHOU Science and Technology on Electronic Test and Measurement Laboratory North University of China Science and Technology on Near-Surface Detection Laboratory china Institute of Sport Science

Recently, human physiological information wireless monitoring in real-time is particularly important in health analysis. As a solution, a non-contact wireless physiological monitoring system based on pyroelectric generator(Py G), whose core part consists of a wireless circuit processing module and a polyvinylidene fluoride(PVDF) film, has been successfully designed. Owing to the temperature change under the stimulation of an external heat source, the output voltage of the Py G self-powered flexible sensor increases with the heat source temperature variation in the range of 295–355 K. Furthermore, based on the natural temperature oscillation between the living body and surrounding environment, the sensor can realize human physiological information assessment, for example, temperature monitoring of the palms, fingers, respiratory heat signals from mouth or nose or non-contact spatial heat mapping recognition of finger movement via sensor array. On this basis, a portable wireless monitoring system was designed by integrating the intelligent sensor with a signal conditioning circuit, data conversion storage module, Bluetooth module,and power module. This system can acquire real-time human oral or nasal breathing signals in the personal mobile app to evaluate the physiological state of individuals. Additionally, the wireless monitoring system can be activated within 10 m, demonstrating the application of Py G sensors in remote data transmission.

关键词： non-contact pyroelectric generator human body heat environmental thermal energy wireless monitoring system

三维电极反应器中活性炭电化学强化吸附As(V)

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Transactions of Nonferrous Metals Society of china 2022年第6期32卷 2080-2090页

作者：罗永健王云燕徐慧杜嘉丽朱明飞张李敏孙竹梅中南大学冶金与环境学院长沙410083 中南大学国家重金属污染防治工程技术研究中心长沙410083 中北大学环境与安全工程学院太原030051

采用自制三维电极反应器对溶液中的As(V)进行电吸附去除,而粒子电极选用活性炭颗粒(GAC)。在最佳条件下,As(V)的去除率为84%,溶液中As(V)的残留浓度为0.08mg/L。从动力学研究中得到,整个过程的速率控制步骤可能涉及两个以上的过程:膜扩... 详细信息

采用自制三维电极反应器对溶液中的As(V)进行电吸附去除,而粒子电极选用活性炭颗粒(GAC)。在最佳条件下,As(V)的去除率为84%,溶液中As(V)的残留浓度为0.08mg/L。从动力学研究中得到,整个过程的速率控制步骤可能涉及两个以上的过程:膜扩散、物质扩散和物理/化学吸附过程。在脱附过程中,As(V)可以从GAC中解吸出来,且GAC在解吸后能再次电吸附As(V),这表明该电极具有良好的循环性能。

关键词：除砷活性炭电吸附三维电极反应器

Inhibition of ASCT2 induces hepatic stellate cell senescence with modified proinflammatory secretome through an IL-1α/NF-κB feedback pathway to inhibit liver fibrosis

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Acta Pharmaceutica Sinica B 2022年第9期12卷 3618-3638页

作者： Feixia Wang Zhanghao Li Li Chen Ting Yang Baoyu Liang Zili Zhang Jiangjuan Shao Xuefen Xu Guoping Yin Shijun Wang Hai Ding Feng Zhang Shizhong Zheng Jiangsu Key Laboratory for Pharmacology and Safety Evaluation of Chinese Materia Medica School of PharmacyNanjing University of Chinese MedicineNanjing 210023China Department of General Surgery Nanjing Hospital Affiliated to Nanjing University of Chinese MedicineNanjing 210003China Department of Anesthesiology Nanjing Hospital Affiliated to Nanjing University of Chinese MedicineNanjing 210003China College of Traditional Chinese Medicine Shandong University of Traditional Chinese MedicineJinan 250035China

Senescence of activated hepatic stellate cells(aHSCs) is a stable growth arrest that is implicated in liver fibrosis *** cells often accompanied by a multi-faceted senescence-associated secretory phenotype(SASP).But little is known about how alanine-serine-cysteine transporter type-2(ASCT2),a high affinity glutamine transporter,affects HSC senescence and SASP during liver ***,we identified ASCT2 is mainly elevated in aHSCs and positively correlated with liver fibrosis in human and mouse fibrotic *** first discovered ASCT2 inhibition induced HSCs to senescence in vitro and in *** proinflammatory SASP were restricted by ASCT2 inhibition at senescence initiation to prevent paracrine ***,ASCT2 was a direct target of glutaminolysisdependent proinflammatory SASP,interfering IL-1α/NF-κB feedback loop via interacting with precursor IL-1α at *** a translational perspective,atractylenolide Ⅲ is identified as ASCT2 inhibitor through directly bound to Asn230 of *** presence of -OH group in atractylenolide Ⅲ is suggested to be favorable for the inhibition of ***,atractylenolide Ⅲ could be utilized to treat liver fibrosis *** together,ASCT2 controlled HSC senescence while modifying the proinflammatory *** ASCT2 by atractylenolide Ⅲ could be a therapeutic candidate for liver fibrosis.

关键词： Hepatic stellate cells Senescence SASP ASCT2 Precursor IL-1α NF-κB Atractylenolide III Liver fibrosis

Schisanlactone G,a new 3,4-seco-lanostane triterpenoid from Schisandra sphenanthera

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Chinese Chemical Letters 2009年第5期20卷 601-603页

作者： Rong Ren Guo Jun Luo Hong Mei Li Zhao Yuan Wu Hai Zhou Li Rong Tao Li The College of Life Science and Technology Kunming University of Science and Technology Kunming 650224 PR China

A new 3,4-seco-lanostane triterpenoid, schisanlactone G （1）, was isolated from the fruits of Schisandra sphenanthera. Its structure was established on the basis of extensive spectroscopic analysis.

关键词： Schisandra sphenanthera Triterpenoid Schisanlactone G