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Nanotechnology and Precision Engineering 2024年第2期7卷 11-24页

作者： Sohaib Raza Chandrakant Nirala Department of Mechanical Engineering Indian Institute of Technology RoparPunjab 140001India

Ultrasonic-assisted micro-electro-discharge machining(EDM)has the potential to enhance processing responses such as material removal rate(MRR)and surface *** understand the reasons for this enhancement,the physical mechanisms responsible for the individual discharges and the craters that they form need to be *** work examines features of craters formed by single discharges at various parameter values in both conventional and ultrasonic-assistedEDM of ***-speed imaging of the plasma channel is performed,and data on the individual discharges are captured in real-time.A 2D axisymmetric model using finite element software is established to model crater *** the basis of simulation and experimental results,a comparative study is then carried out to examine the effects of ultrasonic vibrational assistance on crater *** every set ofEDM parameters,the crater diameter and depth from a single discharge are found to be higher in ultrasonic-assistedEDM than in conventional*** improved crater geometry and the reduced bulge formation at the crater edges are attributed to the increased melt pool velocity and temperature predicted by the model.

关键词： Ultrasonic vibration Discharge crater Plasma diameter Single discharge

Sequential decay analysis of^(235)U(n^(th),f)reaction using fragmentation approach

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Chinese Physics C 2024年第6期48卷 145-154页

作者： Nitin Sharma Ashutosh Kaushik Manoj K.Sharma School of Physics and Materials Science Thapar Institute of Engineering&TechnologyPatiala-147004PunjabIndia

Numerous experimental and theoretical observations have concluded that the probability of the three fragment emission(ternary fission)or binary fission increases when one proceeds towards the heavy mass region of nuclear periodic *** factors affect fragment emission,such as the shell effect,deformation,orientation,and fissility *** and ternary fissions are observed for both ground and excited states of the *** collinear cluster tripartition(CCT)channel of the^(235)U(n^(th),f)reaction is studied,and we observe that the CCT may be a sequential or simultaneous emission *** date,different approaches have been introduced to study the CCT process as a simultaneous or sequential process,but the decay dynamics of these modes have not been not fully *** the three fragments of the sequential process and exploring their related dynamics using an excitation energy dependent approach would be of further ***,in this study,we investigate the sequential decay mechanism of the^(235)U(n^(th),f)reaction using quantum mechanical fragmentation theory(QMFT).The decay mechanism is considered in two steps,where initially,the nucleus splits into an asymmetric *** the second step,the heavy fragment obtained in the first step divides into two *** I analysis is conducted by calculating the fragmentation potential and preformation probability for the spherical and deformed choices of the decaying *** most probable fragment combination of stage I are identified with respect to the dips in the fragmentation structure and the corresponding maxima of the preformation probability(P0).The light fragments of the identified decay channels(obtained in step I)agree closely with the experimentally observed *** excitation energy of the decay channel is calculated using an iteration *** excitation energy is shared using an excitation energy dependent level density *** obtained excitation

关键词： fission cluster radioactivity ternary fission spontaneous fission cluster model total kinetic energy preformation probability

Semitransparent Organic Solar Cells with Superior Thermal/Light Stability and Balanced Efficiency and Transmittance

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Energy & Environmental Materials 2024年第4期7卷 215-222页

作者： Zhipeng Yin Huan Zhao Yang Liu Xunwen Xiao Yong Zhang Huahang Lai Ning Li Hai-Qiao Wang School of Materials Science and Engineering Ningbo Tech University State Key Laboratory of Luminescent Materials and Devices Institute of Polymer Optoelectronic Materials and Devices School of Materials Science and Engineering South China University of Technology Ningbo University of Technology Ningbo Institute of Technology Beihang University Hangna Nanofabrication Equipment Co. Ltd.

Semitransparent organic solar cells show attractive potential in the application of building-integrated photovoltaics,agrivoltaics,floating photovoltaics,and wearable electronics,as their multiple functionalities of e... 详细信息

关键词： organic solar cell semitransparent thermal/light stability

Data-driven Simulations of Magnetic Field Evolution in Active Region 11429:Magneto-frictional Method Using PENCIL CODE

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Research in Astronomy and Astrophysics 2024年第2期24卷 74-82页

作者： P.Vemareddy Jorn Warnecke Ph.A.Bourdin Indian Institute of Astrophysics Sarjapur roadII BlockKoramangalaBengaluru-560034India Max-Planck-Institut für Sonnensystemforschung Justus-von-Liebig-Weg 3D-37077 GöttingenGermany Institute of Physics University of GrazUniversitätsplatz 5A-8010 GrazAustria

Coronal magnetic fields evolve quasi-statically over long timescales and dynamically over short *** of now there exist no regular measurements of coronal magnetic fields,and therefore generating the coronal magnetic field evolution using observations of the magnetic field at the photosphere is a fundamental requirement to understanding the origin of transient phenomena from solar active regions(ARs).Using the magneto-friction(MF)approach,we aim to simulate the coronal field evolution in the solar AR *** MF method is implemented in the open source PENCIL CODE along with a driver module to drive the initial field with different boundary conditions prescribed from observed vector magnetic fields at the *** order to work with vector potential and the observations,we prescribe three types of bottom boundary drivers with varying free-magnetic *** MF simulation reproduces the magnetic structure,which better matches the sigmoidal morphology exhibited by Atmospheric Imaging Assembly(AIA)images at the pre-eruptive *** found that the already sheared field further driven by the sheared magnetic field will maintain and further build the highly sheared coronal magnetic configuration,as seen in AR ***-driven MF simulation is a viable tool to generate the coronal magnetic field evolution,capturing the formation of the twisted flux rope and its eruption.

关键词： Sun corona-Sun evolution-Sun magnetic fields-Sun photosphere

Investigation of 58Ni(n, p)58Co reaction cross-section with covariance analysis

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Chinese Physics C 2024年第2期48卷 78-90页

作者： Akash Hingu S.Mukherjee Siddharth Parashari Arora Sangeeta A.Gandhi Mahima Upadhyay Mahesh Choudhary Sumit Bamal Namrata Singh G.Mishra Sukanya De Saurav Sood Sajin Prasad G.Saxena Ajay Kumar R.G.Thomas B.K.Agrawal K.Katovsky A.Kumar Department of Physics Faculty of ScienceThe M.S.University of BarodaVadodara 390002India Faculty of Electrical Engineering and Communication Brno University of TechnologyBrnoCzech Republic Department of Physics Faculty of ScienceUniversity of ZagrebBijenička c.32Zagreb 10000Croatia Department of Physics University Institute of SciencesChandigarh UniversityGharuanMohali 140413PunjabIndia Department of Physics Banaras Hindu UniversityVaranasi 221005India Horia Hulubei National Institute for Physics and Nuclear Engineering Măgurele 077125Romania Nuclear Physics Division Bhabha Atomic Research CentreMumbai 400085India Health Physics Division Bhabha Atomic Research CentreMumbai 400085India Department of Physics(H&S) Government Women Engineering CollegeAjmer 305002India Saha Institute of Nuclear Physics Kolkata 700064India Homi Bhabha National Institute Anushakti NagarMumbai 400094India

The excitation function of the 58Ni(n,p)58Co reaction was measured using the well-established neutron activation technique andγ-ray *** in the energy range of 1.7 to 2.7 MeV were generated using the 7Li(p,n)*** neutron flux was measured using the standard 115In(n,n’)115mIn monitor *** results of the neutron spectrum averaged cross-section of 58Ni(n,p)58Co reactions were compared with existing cross-section data available in the EXFOR data library as well as with various evaluated data libraries such as ENDF/B-VIII.0,JEFF-3.3,JENDL-4.0,and *** calculations were performed using the nuclear reaction code *** nuclear level density(NLD)models were tested,and their results were compared with the present *** NLDs were also obtained through the spectral distribution method(SDM).The cross-section results,along with the absolute errors,were obtained by investigating the uncertainty propagation and using the covariance *** forγ-ray true coincidence summing,low-energy background neutrons,andγ-ray self attenuation were *** experimental cross-section obtained in the present study is consistent with previously published experimental data,evaluated libraries,and theoretical calculations carried out using the TALYS code.

关键词： nuclear reactions (n,p)reaction cross-section measurement covariance analysis nuclear level density

Advantageous properties of halide perovskite quantum dots towards energy-efficient sustainable applications

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Green Energy & Environment 2024年第6期9卷 949-965页

作者： Qian Zhao Shuo Wang Young-Hoon Kim Shekhar Mondal Qingqing Miao Simiao Li Danya Liu Miao Wang Yaxin Zhai Jianbo Gao Abhijit Hazarika Guo-Ran Li School of Materials Science and Engineering Nankai UniversityTianjin300350China Department of Energy Engineering Hanyang UniversitySeoul04763Republic of Korea Polymers and Functional Materials Division CSIR-Indian Institute of Chemical TechnologyUppal RoadTarnakHyderabad500007India Institute of Process Engineering Chinese Academy of SciencesBeijing100190China Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Department of PhysicsHunan Normal UniversityChangshHunan410081China Department of Chemistry Brock University1812 Sir Isaac WaySt CatharinesOntarioCanada

As lead halide perovskite(LHP)semiconductors have shown tremendous promise in many application fields,and particularly made strong impact in the solar photovoltaic area,low dimensional quantum dot forms of these perovskites are showing the potential to make distinct marks in the fields of electronics,optoelectronics and *** so-called perovskite quantum dots(PQDs)not only possess the most important features of LHP materials,i.e.,the unusual high defect tolerance,but also demonstrate clear quantum size effects,along with exhibiting desirable optoelectronic properties such as near perfect photoluminescent quantum yield,multiple exciton generation and slow hot-carrier ***,we review the advantageous properties of these nanoscale perovskites and survey the prospects for diverse applications which include lightemitting devices,solar cells,photocatalysts,lasers,detectors and memristors,emphasizing the distinct superiorities as well as the challenges.

关键词： Perovskite quantum dot Light-emitting Detector Laser Solar cell

Ionic Liquids Assisted Synthesis of ZnO Nanostructures:Controlled Size,Morphology and Antibacterial Properties

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Journal of Materials Science & Technology 2013年第6期29卷 533-538页

作者： R.Rajiv Gandhi S.Gowri J.Suresh M.Sundrarajan Advanced Green Chemistry Lab Department of Industrial ChemistrySchool of Chemical SciencesAlagappa UniversityKaraikudi 3Tamil NaduIndia

Systematic analysis about the exploitation of imidazolium based ionic liquids （ILs）, [BMIM] BF4 [ILl], [EMIM] BF4 ILL2] and [BMIM] PF6 [IL3] as the morphological template on the basic sol-gel method adopted synthesis of nanostructured zinc oxide （ZnO） is presented. X-ray diffraction （XRD）, particle size analysis （PSA） and scanning electron microscopy （SEM） have been employed for the characterization of structure and morphology of the synthesized ZnO particles. Well-defined capsule like shaped morphology with lower nanosize is observed for the ZnO nanoparticles with ILl than those with IL2 and IL3. This confirms that ILl served as an effective templating material due to their unique properties. Especially the effective aggregation of ZnO particles with a self-organized frame of ILl was the essential factor to produce the lower nanosized ZnO with capsule shaped structure. The synthesized ZnO samples with IL2 and IL3 fabricated the flake like shaped and rod like shaped morphologies in the range of nanoscale. The formed ZnO nanoparticles with IL2 exhibit higher nanosize than the ZnO nanoparticles produced by ILl, owing to shorter length of alkyl group in its cation which restricts steric effect and permits the nanoparticles to grow longer. Even though IL3 produced the discrete ZnO nanorods, the hydrophobic nature of IL3 created the higher nanosize than the ZnO nanoparticles formed by other two ionic liquids. Antibacterial properties of the synthesized ZnO nanostructures were investigated against Staphylococcus aureus （gram positive） and Escherichia coil （gram negative） bacteria by Agar diffusion test method. Microbial experiments indicate that the synthesized ZnO samples show a wide spectrum of antimicrobial activities and performed better against S. aureus than E. coil with the same concentration of ZnO.

关键词： Zinc oxide Ionic liquids Sol-gel method Antibacterial activity

Structural and electrochemical investigations of nanostructured NiTiO3 in acidic environment

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Frontiers of Materials Science 2017年第2期11卷 162-170页

作者： V. CHELLASAMY P. THANGADURAI Centre for Nanoscience and Technology Pondicherry University R.V. Nagar Kalapet Puducherry-605014 India

Electrochemically stable nanostructured nickel titanate （NiTiO3） was prepared by sol-gel method and the structural and electrochemical properties were studied in the presence of H2SO4 ＋ CH3OH electrolyte. XRD and Raman studies confirmed the single phase of NiTiO3 with the rhombohedral structure. Thermal stability was studied by TGA. Microstructure analysis by SEM confirmed the uniformly distributed spherical shaped NiTiO3 particles, and TEM studies showed the spherical shaped particles with an average size of 90 nm. The UV-Vis analysis shows the absorption spectrum of NiTiO3, while the FTIR spectrum showed the vibrations related to Ni-O and Ti-O stretching. Electrochemical tests were carried out by cyclic voltammetry （CV） and polarization studies. The CV measurements were made at room temperature as well as at 60℃： at room temperature, the NiTiO3 did not show any activity towards methanol oxidation whereas there observed an activity at the potential of 0.69 V at the operating temperature of 60℃. The ilmenite structured NiTiO3 has oxygen vacancies, most probably on the surface, which could have also contributed to the methanol oxidation. Thus the nanostructured NiTiO3 is proposed to be an active support material for metal electrocatalysts.

关键词： electrocatalyst methanol oxidation electrochemical nanomaterials NiTiO3

Novel multistage solid-liquid circulating fluidized bed： Hydrodynamic characteristics

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Particuology 2018年第3期16卷 134-142页

作者： Prakash V. Chavan Manjusha A. Thombare Sandip B. Bankar Dinesh V. Kalaga Veena A. Patil-Shinde Department of Chemical Engineering College of Engineering Bharati Vidyapeeth Deemed University Pune 411 043. India Department of Biotechnology and Chemical Technology School of Chemical Technology Alto University P.O. Box 16100. FI-00076 Aalto Finland Department of Chemical Engineering City College of New York CUNY NY USA

The present work proposes a novel radially cross-flow multistage solid-liquid circulating fluidized bed （SLCFB）. The SLCFB primarily consists of a single multistage column （having an inner diameter of 100 mm and length of 1.40 m）, which is divided into two sections wherein both the steps of utilization or loading （e.g., adsorption and catalytic reaction） and regeneration of the solid phase can be carried out simulta- neously in continuous mode. The hydrodynamic characteristics were studied using ion exchange resin as the solid phase and water as the fluidizing medium. The loading and flooding states were determined for three particle sizes; i.e,. 0.30, 0,42, and 0.61 ram. The effects of the superficial liquid velocity and solid feed rate on the solid hold-up were investigated under loading and flooding conditions. The solid hold-up increases with an increase in the solid feed rate and decreases with an increase in the superficial liquid velocity. An artificial-intelligence formalism, namely the multilayer perceptron neural network （MLPNN）, was employed for the prediction of the solid hold-up. The input space of MLPNN-based model consists of four parameters, representing operating and system parameters of the proposed SLCFB. The developed MLPNN-based model has excellent prediction accuracy and generalization capability.

关键词： Solid-liquid fluidized bed Solid-liquid circulating fluidized bed Hydrodynamics Modeling

Investigation of Terminal Group Effect on Electron Transport Through Open Molecular Structures

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Communications in Theoretical Physics 2013年第5期59卷 649-654页

作者： C. Preferencial Kala P. Aruna Priya D. John Thiruvadigal Department of Physics and Nano Technology Center for Materials Science and NanodevicesSRM University Department of Electronics and Communication Engineering Center for Materials Science and NanodevicesSRM University

The effect of terminal groups on the electron transport through metal-molecule-metal system has been investigated using nonequilibrium Green’s function (NEGF) formalism combined with extended Huckel theory (EHT). Au-molecule-Au junctions are constructed with borazine and BCN unit structure as core molecule and sulphur (S), oxygen (O), selenium (Se) and cyano-group (CN) as terminal groups. The electron transport characteristics of the borazine and BCN molecular systems are analyzed through the transmission spectra and the current-voltage curve. The results demonstrate that the terminal groups modifying the transport behaviors of these systems in a controlled way. Our result shows that, selenium is the best linker to couple borazine to Au electrode and oxygen is the best one to couple BCN to Au electrode. Furthermore, the results of borazine systems are compared with that of BCN molecular systems and are discussed. Simulation results show that the conductance through BCN molecular systems is four times larger than the borazine molecular systems. Negative differential resistance behavior is observed with borazine-CN system and the saturation feature appears in BCN systems.

关键词： molecular electronics extended Huckel theory (EHT) nonequilibrium Green’s function (NEGF) quantum transport