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Luminescence properties and optical sensing behaviors of Sr_(2)GdSbO_(6):Eu^(3+) phosphors

Journal of Rare Earths 2024年第8期42卷 1458-1469,I0002页

作者： Youfa Tai Ruirui Cui Jun Zhang Chunkai Wang Tingyu Zhao Beiqiao Zhang Chaoyong Deng Key Laboratory of Functional Composite Materials of Guizhou Province College of Big Data and Information EngineeringGuizhou UniversityGuiyang550025China College of Computer and Information Engineering Guizhou University of CommerceGuiyang550014China School of Electronics and Information Engineering Guiyang UniversityGuiyang550005China

Novel orange-red Sr_(2)GdSbO_(6):xEu^(3+)(x=0,0.05,0.1,0.2,0.3,0.4,0.5 and 0.6) phospho rs were successfully prepared by the traditional high-temperature solid-state *** results of Rietveld refinement,energy dispersive spectroscopy(EDS) spectrum and elemental mapping demonstrate that Eu^(3+) successfully replaces the Gd^(3+) sites and distributes uniformly in the particles of *** luminescence properties of Sr_(2)GdSbO_(6):Eu_(3+)phosphors were investigated in *** emission spectra of the strongest emission peak is the ^(5)D_(0)→^(7)F_(1)(593 nm) transition,which can emit orange-red light under393 nm *** the doping concentration of Eu3+ions is x=0.2,the luminescence intensity of the phosphors reaches the *** detailed mechanism of concentration quenching is attributed to dipole-dipole *** thermal stability values of Sr_(2)GdSbO_(6):0.2Eu^(3+) phosphors are 87%,82% and114% under 393,467 and 527 nm excitations,*** causes of the abnormal thermal quenching under 527 nm excitation were *** on the abnormal thermal quenching under527 nm excitation,the optical thermometry properties of Sr_(2)GdSbO_(6):0.2Eu^(3+)phosphors were investigated by fluorescence intensity ratio(FIR) technique,and appreciable relative sensitivity was *** results suggest that Sr_(2)GdSbO_(6):0.2Eu^(3+)phosphors can be potentially applied to w-LEDs and optical thermometers.

关键词： Sr_(2)GdSbO_(6):Eu^(3+) Phosphors Luminescence properties Abnormal thermal quenching Rare earths

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Superhydrophilic nickel hydroxide ultrathin nanosheets enable high-performance asymmetric supercapacitors

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Rare Metals 2024年第1期43卷 138-147页

作者： Yi-Ran Wang Fei Zhang Jian-Min Gu Xiao-Yu Zhao Ran Zhao Xing Wang Tian-Hui Wu Jing Wang Ji-Dong Wang De-Song Wang State Key Laboratory of Metastable Materials science and technology(MMST) Hebei Key Laboratory of Applied ChemistryYanshan UniversityQinhuangdao 066004China department of Food and Pharmaceutical Engineering Suihua UniversitySuihua 152000China School of Chemical science and Engineering Tongji UniversityShanghai 200092China School of sciences Hebei University of Science and TechnologyShijiazhuang 050018China

Superhydrophilic surfaces have been applied for supercapacitor;however,during energy storage reaction,how the wettability affects the process of electrochemical reaction specifically is still ***,we demonstrate superhydrophilic surface for promotion of electrochemical reactions by liquid affinity and further explain the mechanism,where the transition of the wettability state caused by the change in surface free energy is the main reason for the obvious increase in specific *** citric acid assistance strategy,an intrinsically hydrophobic Ni(OH)_(2)thick nanosheets(HNHTNs,16 nm)can be transitioned into superhydrophilic Ni(OH)_(2)ultrathin nanosheets(SNHUNs,6.8 nm),where the water contact angle was 0°and the surface free energy increased from 8.6to 65.8 mN·m^(-1),implying *** with HNHTNs,the specific capacitance of SNHUNs is doubled:from 1230 F·g^(-1)(HNHTNs)to 2350 F·g^(-1)(2A·g^(-1))and,even at 20 A·g^(-1),from 833 F·g^(-1)(HNHTNs)to 1670 F·g^(-1).The asymmetric capacitors assembled by SNHUNs and activated carbon show 52.44 Wh·kg^(-1)at 160W·kg^(-1)and excellent stability with~90%retention after5000 cycles(~80%retention after 9500 cycles).The promotion of electrochemical performances is ascribed to the change of surface wettability caused by surface free energy,which greatly increase affinity of electrode to the surrounding liquid environment to reduce the interface resistance and optimize the electron transport path.

关键词： Asymmetric supercapacitor Superhydrophilic interface Transition metal hydroxides Ultrathin nanosheets High specific capacitance

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Giant low-field reversible magnetocaloric effect at liquid helium temperature of niobium and iron co-substituted EuTiO_(3) compounds

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Journal of Rare Earths 2024年第4期42卷 710-715页

作者： Zhihong Hao Quanyi Liu Huicai Xie Yan Zhang Zhaojun Mo School of Rare Earth and New Materials Engineering Ganzhou Innovation Center of Rare Earth Permanent Magnet Material Advanced Manufacturing and Intelligent Equipment TechnologyGannan University of Science and TechnologyGanzhou341000China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou34119China School of Materials science and Engineering Taiyuan University of Science and TechnologyTaiyuan030024China

Giant magnetocaloric effect(MCE)materials in the liquid helium temperature region have attracted a lot of attention in the field of low-temperature magnetic refrigeration(MR).In this study,a series of niobium(Nb)and iron(Fe)co-substituted EuTiO_(3) perovskites with cubic structure(space group pm3m)was successfully fabricated,and their magnetic properties as well as cryogenic magnetocaloric effects were investigated in *** expected,the introduction of Nb and Fe can significantly modulate the magnetic phase transition and magnetocaloric effect of the EuTiO_(3) *** increasing Fe concentration,two local minima corresponding to the AFM-FM magnetic phase transition near 5.0 K and FM-PM transition near 10 K with no hysteresis in the thermomagnetic curves are observed,which is attributed to an enhancement of FM *** the same time,the gradually widened-ΔSM-T curves and the two peaks with a broad shoulder lead to considerable refrigeration capacity(RC).With the field change ofΔH=2 T,the calculated values of-ΔS_(M)^(max) for the EuTi_(0.9375-x)Nb_(0.0625)Fe_(x)O_(3)(x=0.075,0.1,0.125,0.15)compounds are 24.2,17.6,14.5 and 14.0 J/(kg·K),*** corresponding RC values were calculated to be 144.6,138.3,151.2 and 159 J/kg,***,the values of-ΔS_(M)^(max) for EuTi_(0.8625)Nb_(0.0625)Fe_(0.075)O_(3) are 8.6 and 15.1 J/(kg·K)under low field changes of 0.5 and 1 T,*** giant low-field reversible magnetocaloric effect makes them attractive candidates for magnetic refrigeration in the liquid helium temperature region.

关键词： Magnetocaloric effect Refrigeration capacity Magnetic entropy change Rareearths

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An Innovative K-Anonymity Privacy-Preserving Algorithm to Improve Data Availability in the Context of Big Data

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Computers, Materials & Continua 2024年第4期79卷 1561-1579页

作者： Linlin Yuan Tiantian Zhang Yuling Chen Yuxiang Yang Huang Li State Key Laboratory of Public Big Data College of Computer Science and TechnologyGuizhou UniversityGuiyang550025China College of Information Engineering Guizhou Open UniversityGuiyang550025China Guizhou Academy of Tobacco science Guiyang550025China

The development of technologies such as big data and blockchain has brought convenience to life,but at the same time,privacy and security issues are becoming more and more *** K-anonymity algorithm is an effective and low computational complexity privacy-preserving algorithm that can safeguard users’privacy by anonymizing big ***,the algorithm currently suffers from the problem of focusing only on improving user privacy while ignoring data *** addition,ignoring the impact of quasi-identified attributes on sensitive attributes causes the usability of the processed data on statistical analysis to be *** on this,we propose a new K-anonymity algorithm to solve the privacy security problem in the context of big data,while guaranteeing improved data ***,we construct a new information loss function based on the information quantity *** that different quasi-identification attributes have different impacts on sensitive attributes,we set weights for each quasi-identification attribute when designing the information loss *** addition,to reduce information loss,we improve K-anonymity in two ***,we make the loss of information smaller than in the original table while guaranteeing privacy based on common artificial intelligence algorithms,i.e.,greedy algorithm and 2-means clustering *** addition,we improve the 2-means clustering algorithm by designing a mean-center method to select the initial center of ***,we design the K-anonymity algorithm of this scheme based on the constructed information loss function,the improved 2-means clustering algorithm,and the greedy algorithm,which reduces the information ***,we experimentally demonstrate the effectiveness of the algorithm in improving the effect of 2-means clustering and reducing information loss.

关键词： Blockchain big data K-anonymity 2-means clustering greedy algorithm mean-center method

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Synthesis,phase transformation and applications of CeCO_(3)OH:A review

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Journal of Rare Earths 2024年第8期42卷 1403-1420,I0001页

作者： Zhou Zou Weihao Tian Xisong Mao Junqi Li Yuanpei Lan Chaoyi Chen Hong Yong Sohn Junshan Zhang Fengyuan Liu department of Metallurgical Engineering College of Materials and MetallurgyGuizhou UniversityGuiyang55025China Guizhou Province Key Laboratory of Metallurgical Engineering and Process Energy Saving Guiyang550025China Guizhou Provincial University Key Laboratory of High-Performance Battery Materials Guiyang550025China department of Materials science and Engineering University of UtahSalt Lake CityUT84112USA

CeCO_(3)OH has a unique crystal structure and excellent optical,electronic and catalytic properties,which has been widely investigated for many ***,ceria obtained from CeCO_(3)OH has a morphology that is similar to that of the precursor,and the CeO_(2)-based products obtained from CeCO_(3)OH exhibit outstanding properties,such as catalytic performances,owing to their designed morphology and oxygen vacancies(OVs).To introduce CeCO_(3)OH into a wider range of potential researchers,we first systematically review the physico-chemical properties,synthesis,reaction and morphology tuning mechanism of CeCO_(3)OH,and summarize the conversion behavior from CeCO_(3)OH to ***,we thoroughly survey the applications of CeCO_(3)OH and its conversion *** for further investigations of CeCO_(3)OH are also made in this *** is hoped that the exhaustive co mpilation of the valuable properties and considerable potential investigations of CeCO_(3)OH will promote further applications of CeCO_(3)OH and CeO_(2)-based functional materials.

关键词： CeCO_(3)OH Morphology tuning CeO_(2) Catalyst Lanthanide compounds Rare earths

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Deep Insight of Design,Mechanism,and Cancer Theranostic Strategy of Nanozymes

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Nano-Micro Letters 2024年第2期16卷 165-217页

作者： Lu Yang Shuming Dong Shili Gai Dan Yang He Ding Lili Feng Guixin Yang Ziaur Rehman Piaoping Yang Key Laboratory of Superlight Materials and Surface technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001People’s Republic of China Yantai research Institute Harbin Engineering UniversityYantai 264000People’s Republic of China Key Laboratory of Green Chemical Engineering and technology of heilongjiang Province College of Material Science and Chemical EngineeringHarbin University of Science and TechnologyHarbin 150040People’s Republic of China department of Chemistry Quaid-i-Azam UniversityIslamabad 45320Pakistan

Since the discovery of enzyme-like activity of Fe3O4 nanoparticles in 2007,nanozymes are becoming the promising substitutes for natural enzymes due to their advantages of high catalytic activity,low cost,mild reaction conditions,good stability,and suitable for large-scale ***,with the cross fusion of nanomedicine and nanocatalysis,nanozyme-based theranostic strategies attract great attention,since the enzymatic reactions can be triggered in the tumor microenvironment to achieve good curative effect with substrate specificity and low side ***,various nanozymes have been developed and used for tumor *** this review,more than 270 research articles are discussed systematically to present progress in the past five ***,the discovery and development of nanozymes are ***,classification and catalytic mechanism of nanozymes are ***,activity prediction and rational design of nanozymes are focused by highlighting the methods of density functional theory,machine learning,biomimetic and chemical ***,synergistic theranostic strategy of nanozymes are ***,current challenges and future prospects of nanozymes used for tumor theranostic are outlined,including selectivity,biosafety,repeatability and stability,in-depth catalytic mechanism,predicting and evaluating activities.

关键词： Nanozymes Classification Prediction and design Catalytic mechanism Tumor theranostics

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Atropine can induce autophagy independent of the M3 muscarinic acetylcholine receptor

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Traditional Medicine research 2024年第7期9卷 35-41页

作者： Hai-Chang Yin Wen-Zhu Zhuang Xin-Jie Jiang Di Liu Postdoctoral research Workstation Heilongjiang Academy of Agricultural SciencesHarbin 150069China. College of Life science and Agriculture Forestry Qiqihar UniversityQiqihar 161006China.

Background: No other effects of atropine other than as an antagonist of muscarinic acetylcholine receptor (mAChR) have been found. Methods: In this study, human kidneyepithelial cells were treated with different physiological regulators. Results: Subsequently, it was found that atropine could significantly induce autophagy as demonstrated by the appearance of autophagosome-like double- or single-membrane vesicles in the cytoplasm ofhost cells and the number of GFP-LC3 dots. In addition, increased conversion of the autophagy marker protein LC3-I and LC3-II and increased p62/SQSTM1 indicatedincomplete autophagy. In addition, atropine induced autophagosome levels in a dose-dependent manner within a certain concentration range in human kidney epithelial cells. In atropine-treated mouse skeletal muscle cells containing nicotinic acetylcholinereceptors and rat cardiac muscle cells containing mAchR, atropine induced autophagy in mouse skeletal muscle cells but not in rat cardiac muscle cells. Furthermore, atropine did not induce autophagy in tissue cells containing mAchR in vivo but did in tissue cells not containing mAchR. Conclusion: This study expands the application and understanding of atropine’s action mechanism in the field of medicine.

关键词： autophagy atropine acetylcholine receptor cells

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Projected changes in Köppen-Trewartha climate zones under 1.5-4℃global warming targets over mid-high latitudes of Northern Asia using an ensemble of RegCM4 simulations

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Advances in Climate Change research 2024年第2期15卷 185-196页

作者： Jie WU Xue-Jie GAO Xian-Bing TANG Filippo GIORGI School of Geography and Environmental Engineering Gannan Normal UniversityGanzhou 341000China Climate Change research Center Institute of Atmospheric PhysicsChinese Academy of SciencesBeijing 100029China Collaborative Innovation Center on Forecast and Evaluation of Meteorological Disasters Nanjing University of Information Science&TechnologyNanjing 210044China University of Chinese Academy of sciences Beijing 100049China The Abdus Salam International Centre for Theoretical Physics Trieste 34100Italy

Mid-high latitude Northern Asia is one of the most vulnerable and sensitive areas to global warming,but relatively less studied *** used an ensemble of a regional climate model(RegCM4)projections to assess future changes in surface air temperature,precipitation and Köppen-Trewartha(K-T)climate types in Northern Asia under the 1.5-4℃global warming ***4 is driven by five CMIP5 global models over an East Asia domain at a grid spacing of 25 *** of the present day(1986-2005)simulations shows that the ensembles of RegCM4(ensR)and driving GCMs(ensG)reproduce the major characters of the observed temperature,precipitation and K-T climate zones reasonably *** and more realistic spatial detail is found in RegCM4 compared to the driving GCMs.A general warming and overall increases in precipitation are projected over the region,with these changes being more pronounced at higher warming *** projected warming by ensR shows different spatial patterns,and is in general lower,compared to ensG in most months of the year,while the percentage increases of precipitation are maximum during the cold *** future changes in K-T climate zones are characterized by a substantial expansion of Dc(temperature oceanic)and retreat of Ec(sub-arctic continental)over the region,reaching∼20%under the 4℃warming *** most notable change in climate types in ensR is found over Japan(∼60%),followed by Southern Siberia,Mongolia,and the Korean Peninsula(∼40%).The largest change in the K-T climate types is found when increasing from 2 to 3℃.The results will help to better assess the impacts of climate change and in implementation of appropriate adaptation measures over the region.

关键词： Mid-high latitudes of Northern Asia Köppen climate zones Global warming targets Regional climate model

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The Method of Polynomial Particular Solutions for Solving Nonlinear Poisson-Type Equations

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Acta Mechanica Solida Sinica 2024年第1期37卷 155-165页

作者： Zhile Jia Yanhua Cao Xiaoran Wu School of sciences East China Jiaotong UniversityNanchang 330013China

In this paper,the method of polynomial particular solutions is used to solve nonlinear Poisson-type partial differential equations in one,two,and three *** condition number of the coefficient matrix is reduced through the implementation of multiple scale technique,ultimately yielding a stable numerical *** methodological process can be divided into two main parts:first,identifying the corresponding polynomial particular solutions for the linear differential operator terms in the governing equations,and second,employing these polynomial particular solutions as basis function to iteratively solve the remaining nonlinear terms within the governing ***,we investigate the potential improvement in numerical accuracy for equations with singularities in the analytical solution by shifting the computational domain a certain *** experiments are conducted to assess both the accuracy and stability of the proposed method.A comparison of the obtained results with those produced by other numerical methods demonstrates the accuracy,stability,and efficiency of the proposed method in handling nonlinear Poisson-type partial differential equations.

关键词： Nonlinear equation Singularity Polynomial particular solutions Poisson type

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Polyoxometalates for continuous power generation by atmospheric humidity

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Nano research 2024年第3期17卷 1875-1885页

作者： Tuo Ji Weilin Chen Zhenhui Kang Liming Zhang Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of education Northeast Normal UniversityChangchun 130024China Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&Devices DepartmentSoochow UniversitySuzhou 215123China Macao Institute of Materials science and Engineering Macao University of Science and TechnologyTaipaMacao 999078China Institute of Functional State Key Laboratory of Luminescence and Applications Changchun Institute of OpticsFine Mechanics and PhysicsChinese Academy of SciencesChangchun 130033China

Atmospheric humidity is a sustainable low-value energy widely existing in natural environment,which is a promising candidate to solve the noncontinuous and low efficiency of low-value energy power *** the mono-substituted Dawson-type polyoxometalates are constructed to be highly dispersed organic ammonium-polyoxoanion clusters and are assembled into thin films power generators with micropores,working in atmospheric *** optimal polyoxometalates generator with the thickness of 7.2μm and the area of 0.36 cm^(2) produces a voltage of 0.68 V and a current density of 19.5μA·cm^(-2) under simulated natural environment,and works continuously and stably under almost all-natural environments(humidity 10%–90%).The highly dispersed polyoxometalate nanoclusters can form microporous in polyoxometalate films to effectively absorb atmospheric humidity and spontaneously form distribution gradient of water,which is the structural basis of power *** continuous power generation may be maintained by the effective adsorption and utilization of H_(2)O,the huge electrostatic field of organic ammonium-polyoxoanion clusters,and the reasonably designed polyoxometalates containing inorganic small ions with high *** is the first humidity generator designed with polyoxometalates,which may provide a new research direction for polyoxometalates in sustainable utilization of low-value energy.

关键词： atmospheric humidity continuous power generations nanomaterials polyoxoanions polyoxometalates

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