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Experimental Study of Liquid Metal Flow for the Development of a Contact-Less Control Technique

Fluid Dynamics & Materials Processing 2024年第7期20卷 1553-1564页

作者： Aleksandr Poluyanov Ilya Kolesnichenko Laboratory of Technological Hydrodynamics Institute of Continuous Media Mechanics of the Ural Branch of Russian Academy of Science(ICMM UB RAS)Perm614018Russia

The article presents an experimental study on the flow of an eutectic gallium alloy in a cylindrical cell,which is placed in an alternating magnetic *** magnetic field is generated by a coil connected to an alternating current *** coil is located at a fixed height in such a way that its plane is perpendicular to the gravity vector,which in turn is parallel to the axis of the *** position of the cylinder can vary in height with respect to the *** forced flow of the considered electrically conductive liquid is generated due to the action of the localized electromagnetic *** is assumed that under the action of the alternating magnetic field,the liquid is heated uniformly,and the resulting heat is quickly absorbed by the forced flow,so that liquid free convection can be *** experiment is carried out using an ultrasonic Doppler *** transducer is installed in the axially located cylinder sluice and the other transducer is placed in the near-wall *** to the results,a velocity profile,corresponding to a two-tori flow pattern can be hardly obtained in the low frequency range of the power ***,this is possible in the high frequency *** average velocity profiles depend essentially on the location of the coil relative to the *** spectral analysis of velocity signals shows that the amplitude of the velocity pulsations is comparable to the average value of the flow *** experimental results and their verification through comparison with numerical calculations are intended to support the development of new methods for reducing the intensity of vortex flows during the electromagnetic separation of impurities through an electromagnetic induction mechanism(able to produce an electromotive force that displaces particles).

关键词： Ultrasonic doppler velocimeter electrically conductive medium azimuthal pinch experiment in liquid metal magnetohydrodynamics

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Early Neoproterozoic Granite-Gneisses of the Junggar Alataw(Southeastern Kazakhstan):Age,Petrogenesis and Tectonic Implications

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Acta Geologica Sinica(English Edition) 2024年第1期98卷 67-82页

作者： Nadezhda KANYGINA Andrey TRETYAKOV Dmitriy ALEXEIEV Kirill DEGTYAREV Anfisa SKOBLENKO Natalia SOLOSHENKO Boris ERMOLAEV Geological Institute Russian Academy of SciencesMoscow 119017Russia A.N.Zavaritsky Institute of Geology and Geochemistry Ural Branch of the Russian Academy of SciencesYekaterinburg 620016Russia

The combined petrographic,petrological,geochemical and geochronological study of the Neoproterozoic gneisses of the Sarychabyn and Baskan complexes of the Junggar Alataw of South Kazakhstan elucidate the Precambrian tectonic evolution of the Aktau–Yili *** is one of the largest Precambrian crustal blocks in the western Central Asian orogenic *** U-Pb single-grain zircon ages indicate that granite-gneisses formed from the same source and crystallised in the early Neoproterozoic ca.930–920 *** chemical composition of gneisses corresponds to A2-type *** whole-rock Nd isotopic characteristics(εNd(t)=−4.9 to−1.0 and TNd(DM-2st)=1.9 to 1.7 Ga)indicate the involvement of Paleoproterozoic crustal rocks in magma *** Neoproterozoic ca.930–920 Ma A-type granitoids in the Aktau–Yili terrane of South and Central Kazakhstan might reflect within-plate magmatism adjacent to the collisional belt or a local extension setting in back-arc areas of the continental arc.

关键词： granitoid magmatism geochemistry geochronology Sm-Nd isotope systematics Neoproterozoic Junggar Alataw Kazakhstan Central Asian orogenic belt

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Influence of Bottom Inclination on the Flow Structure in a Rotating Convective Layer

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Fluid Dynamics & Materials Processing 2024年第4期20卷 739-748页

作者： Andrei Vasiliev Andrei Sukhanovskii Elena Popova Laboratory of Turbulence Institute of Continuous Media Mechanics UB RASPerm614013Russia

The formation of convective flows in a rotating cylindrical layer with an inclined bottom and free surface is *** is driven by localized cooling at the center of the upper free surface and by rim heating at the bottom near the *** horizontal temperature difference in a rotating layer leads to the formation of a convective flow with a complex *** mean meridional circulation,consisting of three cells,provides a strongly non-uniform differential *** a result of the instability of the main cyclonic zonal flow,the train of baroclinic waves appears in the upper *** baroclinic waves provide most of the heat transfer in the middle radii and are responsible for strong temperature and velocity *** is shown that the inclination of the bottom is a crucial factor for the structure of the convective cells and the dynamics of the baroclinic *** increase in the inclination angle leads to a significant increase in the energy of the *** obtained results may be important for heat and mass transfer in various geophysical and industrial systems,including transport of various additives and impurities in rotating crucibles,and crystallization processes.

关键词： Laboratory modeling global atmospheric circulation baroclinic waves beta-effect

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Effect of the anionic composition of sulfolane based electrolytes on the performances of lithium-sulfur batteries

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Journal of Energy Chemistry 2024年第8期95卷 231-240,I0005页

作者： Elena V.Karaseva Elena V.Kuzmina Bo-Quan Li Qiang Zhang Vladimir S.Kolosnitsyn Ufa Institute of Chemistry of the Ufa Federal Research Centre of the russian Academy of science 71Prospect OktyabryaUfa 450054BashkortostanRussia Advanced Research Institute of Multidisciplinary science Beijing Institute of TechnologyBeijing 100081China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China

In lithium-sulfur batteries,cell design,specifically electrolyte design,has a key impact on the battery *** effect of lithium salt anion donor number(DN)(DN[PF_(6)]^(-)=2.5,DN[N(SO_(2)CF_(3))_(2)]^(-)=5.4,DN[ClO_(4)]^(-)=8.4,DN[SO_(3)CF_(3)]^(-)=16.9,and DN[NO_(3)]^(-)=21.1)on the patterns of lithium-sulfur batteries and lithium metal electrode performances with sulfola ne-based electrolytes is *** increase in DN of lithium salt anions leads to an increase in the depth and rate of electrochemical reduction of sulfur and long-chain lithium polysulfides and to a decrease in those for medium-and short-chain lithium *** of lithium salt anions has weak effect on the discharge capacity of lithium-sulfur batteries and the Coulomb efficiency during cycling,with the exception of LiSO_(3)CF_(3)and LiNO_(3).An increase in DN of lithium salt anions leads to an increase in the cycling duration of lithium metal anodes and to a decrease in the presence of lithium *** sulfolane solutions of LiNO_(3)and LiSO_(3)CF_(3),lithium polysulfides do not affect the cycling duration of lithium metal anodes.

关键词： Donor number Lithium salt Sulfolane Lithium polysulfide Electrolyte Lithium-sulfur battery Lithium metal electrode

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Major depressive disorder:hypothesis,mechanism,prevention and treatment

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Signal Transduction and Targeted Therapy 2024年第3期9卷 913-944页

作者： Lulu Cui Shu Li Siman Wang Xiafang Wu Yingyu Liu Weiyang Yu Yijun Wang Yong Tang Maosheng Xia Baoman Li Department of Forensic Analytical Toxicology School of Forensic MedicineChina Medical UniversityShenyangChina Liaoning Province Key Laboratory of Forensic Bioevidence sciences ShenyangChina China Medical University Centre of Forensic Investigation ShenyangChina International Joint Research Centre on Purinergic Signalling/Key Laboratory of Acupuncture for Senile Disease(Chengdu University of TCM) Ministry of Education/School of Health and RehabilitationChengdu University of Traditional Chinese Medicine/Acupuncture and Chronobiology Key Laboratory of Sichuan ProvinceChengduChina Department of Orthopaedics The First HospitalChina Medical UniversityShenyangChina

Worldwide,the incidence of major depressive disorder(MDD)is increasing annually,resulting in greater economic and social ***,the pathological mechanisms of MDD and the mechanisms underlying the effects of pharmacological treatments for MDD are complex and unclear,and additional diagnostic and therapeutic strategies for MDD still are *** currently widely accepted theories of MDD pathogenesis include the neurotransmitter and receptor hypothesis,hypothalamicpituitary-adrenal(HPA)axis hypothesis,cytokine hypothesis,neuroplasticity hypothesis and systemic influence hypothesis,but these hypothesis cannot completely explain the pathological mechanism of *** it is still hard to adopt only one hypothesis to completely reveal the pathogenesis of MDD,thus in recent years,great progress has been made in elucidating the roles of multiple organ interactions in the pathogenesis MDD and identifying novel therapeutic approaches and multitarget modulatory strategies,further revealing the disease features of ***,some newly discovered potential pharmacological targets and newly studied antidepressants have attracted widespread attention,some reagents have even been approved for clinical treatment and some novel therapeutic methods such as phototherapy and acupuncture have been discovered to have effective improvement for the depressive *** this work,we comprehensively summarize the latest research on the pathogenesis and diagnosis of MDD,preventive approaches and therapeutic medicines,as well as the related clinical trials.

关键词： prevention acupuncture hypothesis

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An advanced theoretical approach to study super-multiperiod superlattices:theory vs experiments

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Journal of Semiconductors 2024年第2期45卷 57-66页

作者： Alexander Sergeevich Dashkov Semyon Andreevich Khakhulin Dmitrii Alekseevich Shapran Gennadii Fedorovich Glinskii Nikita Andreevich Kostromin Alexander Leonidovich Vasiliev Sergey Nikolayevich Yakunin Oleg Sergeevich Komkov Evgeniy Viktorovich Pirogov Maxim Sergeevich Sobolev Leonid Ivanovich Goray Alexei Dmitrievich Bouravleuv Saint-Petersburg Electrotechnical University"LETI" Saint Petersburg197022Russian Federation Alferov Saint-Petersburg National Research Academic University of the russian Academy of sciences Saint Petersburg194021RussiaFne deration Saint Petersburg Polytechnic University of Peter the Great Saint Petersburg195251Russian Federation Shubnikov Institute of Crystallography of Federal Scientific Research Centre“Crystallography and Photonics” Russian Academy of SciencesMoscow119333Russian Federation National Research Center‘Kurchatov Institute’ Moscow123182Russian Federation University associated with IA EAEC Saint Petersburg194044Russian Federation Institute for Analytical Instrumentation Saint Petersburg198095Russian Federation Ioffe Institute Saint Petersburg194021Russian Federation

A new theoretical method to study super-multiperiod superlattices has been *** method combines the precision of the 8-band kp-method with the flexibility of the shooting method and the Monte Carlo *** method was applied to examine the finest quality samples of super-multiperiod Al_(0.3)Ga_(0.7)As/GaAs superlattices grown by molecular beam *** express photoreflectance spectroscopy method was utilized to validate the proposed theoretical *** the first time,the accurate theoretical analysis of the energy band diagram of super-multiperiod superlattices with experimental verification has been *** proposed approach highly accurately determines transition peak positions and enables the calculation of the energy band diagram,transition energies,relaxation rates,and gain *** has achieved a remarkably low 5%error compared to the commonly used method,which typically results in a 25%error,and allowed to recover the superlattice *** retrieved intrinsic parameters of the samples aligned with XRD data and growth *** proposed method also accurately predicted the escape of the second energy level for quantum well thicknesses less than 5 nm,as was observed in photoreflectance *** new designs of THz light-emitting devices operating at room temperature were suggested by the developed method.

关键词： super-multiperiod superlattice photoreflectance spectroscopy Kane model kp-method energy band diagram light amplifiers

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Prediction of Moments in the Particles on Demand Method for LBM

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Communications in Computational Physics 2023年第1期33卷 144-173页

作者： Elizaveta Zipunova Anastasia Perepelkina Vadim Levchenko German Zvezdin Keldysh Institute of Applied Mathematics RAS 4 Miusskaya sq.MoscowRussia125047 Moscow State University 1 Ulitsa KolmogorovaMoscowRussia119991

PonD is a method to extend LBM calculations to arbitrary ranges of Mach number and *** current work was motivated by the issue of mass,momentum and energy conservation in the PonD method for *** collision guarantees their conservation,thus,the study involves all aspects of the streaming step:both coordinate and velocity space discretizations,gauge transfer method,resolution of the scheme *** obtaining the expressions for the change of moments in the system in a time update of the scheme,it was found that the scheme can be formulated as explicit in some ***,we found the sufficient conditions to make Pond/RegPonD computations explicit and mass,momentum,and energy *** scheme was implemented in the explicit form,and validated for several test cases.

关键词： LBM compressible off-grid

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Machine learning-driven synthesis of TiZrNbHfTaC_(5) high-entropy carbide

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npj Computational Materials 2023年第1期9卷 2293-2303页

作者： Alexander Ya.Pak Vadim Sotskov Arina A.Gumovskaya Yuliya Z.Vassilyeva Zhanar S.Bolatova Yulia A.Kvashnina Gennady Ya.Mamontov Alexander V.Shapeev Alexander G.Kvashnin National Research Tomsk Polytechnic University 30 Lenin AvenueTomsk 634050Russia Skolkovo Institute of science and Technology Skolkovo Innovation CenterBolshoi Blv.30Building 1Moscow 121205Russia Pirogov russian National Research Medical University 1 Ostrovityanova St.Moscow 117997Russia

Synthesis of high-entropy carbides(HEC)requires high temperatures that can be provided by electric arc plasma ***,the formation temperature of a single-phase sample remains ***,under some temperatures multi-phase structures can *** this work,we developed an approach for a controllable synthesis of HEC TiZrNbHfTaC_(5) based on theoretical and experimental *** used Canonical Monte Carlo(CMC)simulations with the machine learning interatomic potentials to determine the temperature conditions for the formation of single-phase and multi-phase *** full agreement with the theory,the single-phase sample,produced with electric arc discharge,was observed at 2000 *** 1200 K,the sample decomposed into(Ti-Nb-Ta)C,and a mixture of(Zr-Hf-Ta)C,(Zr-Nb-Hf)C,(Zr-Nb)C,and(Zr-Ta)*** results demonstrate the conditions for the formation of HEC and we anticipate that our approach can pave the way towards targeted synthesis of multicomponent materials.

关键词： carbide materials

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Tunable order in colloids of hard magnetic hexaferrite nanoplatelets

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Nano Research 2022年第2期15卷 898-906页

作者： Artem A.Eliseev Lev A.Trusov Evgeny O.Anokhin Andrei P.Chumakov Vladimir V.Korolev Anastasia E.Sleptsova Peter Boesecke Vladimir Ya.Shur Vladimir YaShur Pavel E.Kazin Andrei A.Eliseev Faculty of Chemistry Moscow State UniversityLeninskie Gory lb3Moscow 119991Russia Department of Materials science MSU-BIT UniversityShenzhen 517182China Faculty of Materials science Moscow State UniversityLeninskie Gory lb73Moscow 119991Russia European Synchrotron Radiation Facility Avenue des Martyrs 71Grenoble 38043France School of Natural sciences and Mathematics Ural Federal UniversityLenin Ave 51Ekaterinburg 620000Russia

Structural ordering in the concentrated magnetic colloids containing 50×5 nm hard magnetic disc-like SrFe_(12)O_(19) nanoparticles was investigated by cryogenic scanning electron microscopy,optical microscopy,magnetic measurements,and small-angle X-ray *** was revealed that macroscopically homogeneous magnetic liquid consists of dynamic threads of stacked *** threads align into quasiperiodic arrays with the distances between individual threads of a few *** also can form pseudodomain structures with -90°domain boundaries realized through T-type thread *** effects of magnetic attraction and electrostatic repulsion on the equilibrium interplatelet distance in the threads were *** was demonstrated that this distance can be tuned by the control of the particles charge and electric double layer screening from Stern layer thickness(-1 nm)to tens of *** was shown that the permanent magnetic field is not able to cause any structural changes in the ordered magnetic liquid phase,while alternating field draws particles apart by their *** variation of interparticle distance up to 6%was achieved using an alternating magnetic field of low *** data were complemented by the theoretical models of screened electrostatic interactions between spherical and platelike magnetic *** last model provides good predictive power and correlates with the experimental *** stabilization energy of the condensed phase in the order of 1-10 kBT was derived from the *** approach allows controlling of an equilibrium interparticle distance and interparticle distance distribution by adjusting the magnetization and surface charge of the particles as well as the ionic strength of the solvent.

关键词： hexaferrite ferrofluid self-assembly colloidal solution

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High-performance cascade nanoreactor based on halloysite nanotubes-integrated enzyme-nanozyme microsystem

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Chinese Chemical Letters 2022年第2期33卷 807-811页

作者： Yan Liu Rui Lv Shiyong Sun Daoyong Tan Faqin Dong Yevgeny A.Golubev Xiaoqin Nie Olga B.Kotova Jin Liu Ke Wang School of Environment and Resource Key Laboratory of Solid Waste Treatment and Resource Recycle of Ministry of EducationSouthwest University of Science and TechnologyMianyang 621010China Yushkin’s Institute of Geology Komi Science CenterUral Branch of RASul.Pervomayskaya54Syktyvkar 167982Russia

Various enzymatic reactions or enzymatic cascade reactions occur efficiently in biological microsystems due to space constraints or orderly transfer of intermediate products. Inspired by this, the horseradish peroxidase(HRP)-like nanozyme(Fe-aminoclay) was in situ synthesized on the surface of alkali-activated halloysite nanotubes and the natural enzyme(glucose oxidase, GOx) was immobilized on it to construct a high-efficiency GOx-Fe AC@AHNTs cascade nanoreactor. In which, Fe AC@AHNTs can not only be used as a carrier for immobilized enzymes, but also help its catalytic activity to cooperate with glucose oxidase in a cascade reaction. The microcompartments and substrate channel effect of this enzyme-nanozyme microsystem exhibit a superior catalytic performance than that of natural enzyme system, and exhibits excellent long-term stability and recyclability. Subsequently, the GOx-Fe AC@AHNTs cascade nanoreactor was employed as a glucose colorimetric platform, which displayed a low detection limit(0.47 μmol/L)in glucose detection. This enzyme-nanoenzyme nanoreactor provides a simple and effective example for constructing a multi-enzyme system with limited space, and lays the foundation for subsequent research in the fields of biological analysis and catalysis.

关键词： Halloysite nanotubes Fe-aminoclay Nanozyme Cascade nanoreactor Catalysis enhancement

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