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Molecule‑Level Multiscale Design of Nonflammable Gel Polymer Electrolyte to Build Stable SEI/CEI for Lithium Metal Battery

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Nano-Micro Letters 2025年第1期17卷 404-423页

作者： Qiqi Sun Zelong Gong Tao Zhang Jiafeng Li Xianli Zhu Ruixiao Zhu Lingxu Wang Leyuan Ma Xuehui Li Miaofa Yuan Zhiwei Zhang Luyuan Zhang Zhao Qian Longwei Yin Rajeev Ahuja Chengxiang Wang Key Laboratory for Liquid‑Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan 250061People’s Republic of China Condensed Matter Theory Department of Physics and AstronomyUppsala UniversityUppsala 75120Sweden

The risk of flammability is an unavoidable issue for gel polymer electrolytes(GPEs).Usually,flameretardant solvents are necessary to be used,but most of them would react with anode/cathode easily and cause serious interfacial instability,which is a big challenge for design and application of nonflammable ***,a nonflammable GPE(SGPE)is developed by in situ polymerizing trifluoroethyl methacrylate(TFMA)monomers with flame-retardant triethyl phosphate(TEP)solvents and LiTFSI–LiDFOB dual lithium *** is strongly anchored to PTFMA matrix via polarity interaction between-P=O and-CH_(2)CF_(3).It reduces free TEP molecules,which obviously mitigates interfacial reactions,and enhances flame-retardant performance of TEP *** TEP molecules are also inhibited in solvation of Li^(+),leading to anion-dominated solvation sheath,which creates inorganic-rich solid electrolyte interface/cathode electrolyte interface *** coordination structure changes Li^(+)transport from sluggish vehicular to fast structural transport,raising ionic conductivity to 1.03 mS cm^(-1) and transfer number to 0.41 at 30℃.The Li|SGPE|Li cell presents highly reversible Li stripping/plating performance for over 1000 h at 0.1 mA cm^(−2),and 4.2 V LiCoO_(2)|SGPE|Li battery delivers high average specific capacity>120 mAh g^(−1) over 200 *** study paves a new way to make nonflammable GPE that is compatible with Li metal anode.

关键词： Anchoring effect Nonflammable gel electrolyte In situ cross-linked Electrode-electrolyte interface Li metal battery

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Second harmonic generation from precise diamond blade diced ridge waveguides

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Chinese Physics B 2022年第9期31卷 340-345页

作者： Hui Xu Ziqi Li Chi Pang Rang Li Genglin Li ShAkhmadaliev Shengqiang Zhou Qingming Lu Yuechen Jia Feng Chen School of Physics State Key Laboratory of Crystal MaterialsShandong UniversityJinan 250100China Division of Physics and Applied Physics School of Physical and Mathematical SciencesNanyang Technological UniversitySingapore 637371Singapore Institute of Ion Beam and Materials Research Helmholtz-Zentrum Dresden-RossendorfDresden 01314Germany School of Chemistry and Chemical Engineering Shandong UniversityJinan 250100China

Carbon ion irradiation and precise diamond blade dicing are applied to fabricate Nd∶GdCOB ridge *** propagation properties of the fabricated Nd∶GdCOB waveguides are investigated through experiments and theoret-ical ***-Raman analysis reveals that the Nd∶GdCOB crystal lattice expands during the irradiation ***-second harmonic spectroscopic analysis suggests that the original nonlinear properties of the Nd∶GdCOB crystal are greatly enhanced within the waveguide *** pulsed 1064 nm laser pumping,second harmonic generation(SHG)at 532 nm has been achieved in the fabricated *** maximum SHG conversion efficiencies are determined to be~8.32%·W^(-1) and~22.36%·W^(-1) for planar and ridge waveguides,respectively.

关键词： optical waveguides Nd:GdCOB crystal second harmonic generation

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Quantum dot-enabled infrared hyperspectral imaging with single-pixel detection

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Light(Science & Applications) 2024年第6期13卷 1112-1121页

作者： Heyan Meng Yuan Gao Xuhong Wang Xianye Li Lili Wang Xian Zhao Baoqing Sun School of Information Sciences and Engineering Shandong UniversityQingdaoChina Center for Optics Research and Engineering(CORE) Key Laboratory of Laser&Infrared System(Shandong University)Ministry of EducationShandong UniversityQingdaoChina School of Mechanical Electrical and Information EngineeringShandong UniversityWeihaiChina

Near-infrared(NIR)hyperspectral imaging is a powerful technique that enables the capture of three-dimensional(3D)spectra-spatial information within the NIR spectral range,offering a wide array of ***,the high cost associated with InGaAs focal plane array(FPA)has impeded the widespread adoption of NIR hyperspectral *** this challenge,in this study,we adopt an alternative approach—single-pixel detection for NIR hyperspectral *** investigation reveals that single-pixel detection outperforms conventional FPA,delivering a superior signal-to-noise ratio(SNR)for both spectral and imaging *** implement this strategy,we leverage self-assembled colloidal quantum dots(CQDs)and a digital micromirror device(DMD)for NIR spectral and spatial information multiplexing,complemented by single-pixel detection for simultaneous spectral and image *** experimental results demonstrate successful NIR hyperspectral imaging with a detection window about 600 nm and an average spectral resolution of 8.6 nm with a pixel resolution of 128×*** resulting spectral and spatial data align well with reference instruments,which validates the effectiveness of our *** circumventing the need for expensive and bulky FPA and wavelength selection components,our solution shows promise in advancing affordable and accessible NIR hyperspectral imaging technologies,thereby expanding the range of potential applications.

关键词： spectral Quantum mirror

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Porous and Ultra-Flexible Crosslinked MXene/Polyimide Composites for Multifunctional Electromagnetic Interference Shielding

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Nano-Micro Letters 2022年第4期14卷 59-74页

作者： Zhi-Hui Zeng Na Wu Jing-Jiang Wei Yun-Fei Yang Ting-Ting Wu Bin Li Stefanie Beatrice Hauser Wei-Dong Yang Jiu-Rong Liu Shan-Yu Zhao Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials Ministry of Education and School of Materials Science and EngineeringShandong UniversityJinan 250061People’s Republic of China Department of Chemistry and Applied Biosciences ETH ZurichCH-8093 ZurichSwitzerland Laboratory for Cellulose and Wood Materials Swiss Federal Laboratories for Materials Science and Technology(Empa)8600 DübendorfSwitzerland Laboratory for Building Energy Materials and Components Swiss Federal Laboratories for Materials Science and Technology(Empa)8600 DübendorfSwitzerland School of Aerospace Engineering and Applied Mechanics Tongji UniversityShanghai 200092People’s Republic of China

Lightweight,ultra-flexible,and robust crosslinked transition metal carbide(Ti3C2 MXene)coated polyimide(PI)(C-MXene@PI)porous composites are manufactured via a scalable dip-coating followed by chemical crosslinking *** addition to the hydrophobicity,anti-oxidation and extreme-temperature stability,efficient utilization of the intrinsic conductivity of MXene,the interfacial polarization between MXene and PI,and the micrometer-sized pores of the composite foams are ***,the composites show a satisfactory X-band electromagnetic interference(EMI)shielding effectiveness of 22.5 to 62.5 dB at a density of 28.7 to 48.7 mg cm−3,leading to an excellent surface-specific SE of 21,317 dB cm^(2)g^(−1).Moreover,the composite foams exhibit excellent electrothermal performance as flexible heaters in terms of a prominent,rapid reproducible,and stable electrothermal effect at low voltages and superior heat performance and more uniform heat distribution compared with the commercial heaters composed of alloy ***,the composite foams are well attached on a human body to check their electromechanical sensing performance,demonstrating the sensitive and reliable detection of human motions as wearable *** excellent EMI shielding performance and multifunctionalities,along with the facile and easy-to-scalable manufacturing techniques,imply promising perspectives of the porous C-MXene@PI composites in next-generation flexible electronics,aerospace,and smart devices.

关键词： MXene Polyimide Electromagnetic interference shielding Heater Sensor

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Microstructure,Corrosion and Mechanical Properties of Medium-Thick 6061-T6 Alloy/T2 Pure Cu Dissimilar Joints Produced by Double Side Friction Stir Z Shape Lap-Butt Welding

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Chinese Journal of Mechanical Engineering 2024年第2期37卷 385-400页

作者： Jiuxing Tang Guoxin Dai Lei Shi Chuansong Wu Sergey Mironov Surendra Kumar Patel Song Gao Mingxiao Wu MOE Key Lab for Liquid-Solid Structure Evolution and Materials Processing Shandong UniversityJinan 250061China Laboratory of Mechanical Properties of Nanoscale Materials and Superalloys Belgorod State UniversityBelgorod 308015Russia School of Mechanical Engineering Qilu University of Technology(Shandong Academy of Sciences)Jinan 250353China State Grid Henan Electric Power Research Institute Zhengzhou 450052China

A novel double side friction stir Z shape lap-butt welding(DS-FSZW)process was proposed to achieve excellent mechanical properties of Al/Cu medium-thick dissimilar *** influence of welding parameters on weld microstructure and properties of DS-FSZW joint were systematically *** indicated that defect-free medium-thick Al/Cu DS-FSZW joint could be achieved under an optimal welding ***-FSZW joint was prone to form void defects in the bottom of the second-pass *** recrystallization mechanisms at the top and middle of the weld nugget zone(WNZ)were continuous dynamic recrystallization(CDRX)and geometric dynamic recrystallization(GDRX).While the major recrystallization mechanism at the bottom of the WNZ was ***-FSZW joint of the optimal welding condition with 850 r/min-400 mm/min was produced with a continuous thin and crack-free IMCs layer at the Al/Cu interface,and the maximum tensile strength of this joint is 160.57 MPa,which is equivalent to 65.54%of pure Cu base ***,the corrosion resistance of Al/Cu DS-FSZW joints also achieved its maximum value at the optimal welding parameter of 850 r/min-400 mm/*** demonstrates that the DS-FSZW process can simultaneously produce medium-thick Al/Cu joints with excellent mechanical performance and corrosion resistance.

关键词： DS-FSZW Al/Cu dissimilar joint Corrosion behaviour Intermetallic compounds Microstructure Mechanical properties

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Thickness-dependent highly sensitive photodetection behavior of lead-free all-inorganic CsSnBr_(3) nanoplates

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Rare Metals 2022年第5期41卷 1753-1760页

作者： Dong Liu Yan-Xue Yin Feng-Jing Liu Cheng-Cheng Miao Xin-Ming Zhuang Zhi-Yong Pang Ming-Sheng Xu Ming Chen Zai-Xing Yang School of Physics State Key Laboratory of Crystal MaterialsSchool of MicroelectronicsShandong UniversityJinan 250100China

Non-layered two-dimensional(2D) lead-free all-inorganic perovskites nanoplates have recently attracted considerable attention in photodetectors;however, the indepth investigation of thickness on photodetection performance is still lacking. In this work, by constructing the famous metal-semiconductor-metal photodetectors, the photodetection behaviors of thickness-controlled CsSnBr;nanoplates are investigated systematically. Ni electrodes are adopted for ensuring the good ohmic contact behaviors of as-fabricated photodetectors. With the increase in thickness, the photodetection performances improve accordingly, such as photocurrent increases from 0.22 to 19.40 nA, responsivity increases from 72.9 to 4893.7 mA·W^(-1), rise/decay time decreases from 11/35 to 3/10 ms, respectively. Notability, the dark current also increases with the increase in thickness, making the further investigation on the reduction in dark current *** of the as-fabricated photodetectors are stable, suggesting the careful thickness selection in next-generation high-performance lead-free all-inorganic perovskites photodetectors.

关键词： Thickness Photodetection Lead-free all-inorganic perovskites Non-layered two-dimensional perovskites CsSnBr3 nanoplates

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Progress of organic magnetic materials

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Science China(Physics,Mechanics & Astronomy) 2019年第7期62卷 22-33页

作者： Mengmeng Wei Yingcai Fan Wei Qin State Key Laboratory of Crystal Materials School of Physics Shandong University School of Information and Electronic Engineering Shandong Technology and Business University

Over the past years, the development of magnetic materials has been intensively explored, both for fundamental research and technological applications. Particularly, several materials with large magnetoresistance effect have received significant *** this study, we provide an analysis of the progress of organic magnetic materials and organic magnetoelectric complexes, thus paving the way for the understanding of organic magnetism and magnetoelectric coupling mechanisms. In addition, this analysis provides us a critical guide for future organic magnetic material design and fabrication.

关键词： organic materials magnetism magnetoelectric coupling effect

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Design and development of multi-channel front end electronics based on dual-polarity charge-to-digital converter for SiPM detector applications

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Nuclear Science and Techniques 2023年第2期34卷 1-12页

作者： Yu‑Ying Li Chang‑Yu Li Kun Hu Institute of Frontier and Interdisciplinary Science Shandong UniversityQingdao 266237China

With the development of silicon photomultiplier(SiPM)technology,front-end electronics for SiPM signal processing have been highly sought after in various fields.A compact 64-channel front-end electronics(FEE)system achieved by fieldprogrammable gate array-based charge-to-digital converter(FPGA-QDC)technology was built and *** FEE consists of an analog board and FPGA *** analog board incorporates commercial amplifiers,resistors,and *** FPGA board is composed of a low-cost *** electronics performance of the FEE was evaluated in terms of noise,linearity,and uniformity.A positron emission tomography(PET)detector with three different readout configurations was designed to validate the readout capability of the FEE for SiPM-based *** PET detector was made of a 15×15 lutetium–yttrium oxyorthosilicate(LYSO)crystal array directly coupled with a SiPM array *** experimental results show that FEE can process dual-polarity charge signals from the SiPM *** addition,it shows a good energy resolution for 511-keV gamma photons under the dual-end readout for the LYSO crystal array irradiated by a Na-22 ***,the FEE based on FPGA-QDC shows promise for application in SiPM-based radiation detectors.

关键词： Readout electronics Charge measurement Radiation detector Silicon photomultiplier Field-programmable gate array

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An overview of recent progress in the development of flexible electrochromic devices

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Nano Materials Science 2023年第4期5卷 369-391页

作者： Bin Wang Wu Zhang Feifei Zhao William W.Yu Abdulhakem Y.Elezzabi Linhua Liu Haizeng Li Optics and Thermal Radiation Research Center Institute of Frontier&Interdisciplinary ScienceShandong UniversityQingdao266237China School of Chemistry&Chemical Engineering Shandong UniversityJinan250100China Ultrafast Optics and Nanophotonics Laboratory Department of Electrical and Computer EngineeringUniversity of AlbertaEdmontonAlbertaT6G 2V4Canada

Electrochromic materials are capable of reversibly switching their colors or optical properties through redox reactions under applied voltages,which have shown great potential applications including smart windows,nonemissive displays,optical filters,among *** the current rigid electrochromic devices have shown emerging interest and developed rapidly,many applications(e.g.,wearable/deformable optoelectronics)are blocked due to their inflexible ***,the adaption of rigid electrochromic devices to flexible ones is of particular interest for the new era of smart *** this review,the current state-of-the-art achievements of flexible electrochromic devices(FECDs)are highlighted,along with their design strategies and the choice of electrochromic *** recent research progress of FECDs is reviewed in detail,and the challenges and corresponding solutions for real-world applications of FECDs are ***,we summarize the basic fabrication strategies of FECDs and their potential *** addition,the development trend,the perspectives,and the outlook of FECDs are discussed at the end of this Review,which may provide recommendations and potential directions to advance the practical applications of FECDs.

关键词： Electrochromism Flexible electrochromic devices Optoelectronics Optical materials

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High-performance multifunctional(Hf^(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))C high-entropy ceramic reinforced with low-loading 3D hybrid graphene–carbon nanotube

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Journal of Advanced Ceramics 2023年第2期12卷 341-356页

作者： Jialin SUN Jun ZHAO Yonghui ZHOU Peng ZHAI Xialun YUN Zhifu HUANG Hui ZHANG Guohua ZHANG School of Mechanical Electrical&Information EngineeringShandong University(Weihai)Weihai 264209China State Key Laboratory for Mechanical Behavior of Materials School of Materials Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China Key Laboratory of High Efficiency and Clean Mechanical Manufacture of Ministry of Education School of Mechanical EngineeringShandong UniversityJinan 250061China State Key Laboratory for Manufacturing System Engineering School of Mechanical EngineeringXi’an Jiaotong UniversityXi’an 710049China State Key Laboratory of High Performance Ceramics and Superfine Microstructure Shanghai Institute of CeramicsChinese Academy of SciencesShanghai 200050China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

There has been growing interest in the high-entropy ceramic(HEC)recently owing to its tailorable compositions and microstructures,versatile properties,together with promising structural and functional ***,inferior fracture toughness(KIC)and damage tolerance restricted many practical applications of the ***,we addressed this challenge by incorporating a threedimensional graphene–carbon nanotube(3D G–CNT)as toughening agent in(Hf_(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))*** resulting enhanced 3D G–CNT/(Hf_(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))C featured an outstanding toughness of 8.23 MPa·m^(1/2),while remaining superior strength(763 MPa)and hardness(24.7 GPa).An ultralow friction coefficient(0.15)coupled with an ultralow wear rate(w,2.6×10^(−7) mm^(3)/(N·m))in the 3D G–CNT/(Hf_(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))C was obtained primarily as a function of lubricating scrolls,in which two-dimensional(2D)graphene acted as a tribolayer,and one-dimensional(1D)carbon nanotubes acted as nano ball bearings embedded ***,the 3D G–CNT/(Hf_(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))C exhibited rather low thermal conductivity(κ)yet excellent electrical conductivity(σ,1.3×10^(6) S/m)in comparison with the pure(Hf_(0.2)Nb_(0.2)Ta_(0.2)Ti_(0.2)Zr_(0.2))*** study provided great potential for maximizing the physical and functional properties of the HEC for various applications.

关键词： high-entropy ceramic(HEC) three-dimensional graphene-carbon nanotube(3D G-CNT) toughening lubricating thermal conductivity(κ)/electrical conductivity(σ)

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