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Energy & Environmental materials 2024年第4期7卷 413-421页

作者： Liangping Xiao Rusen Zhou Tianqi Zhang Xiaoxiang Wang Renwu Zhou Patrick J.Cullen Kostya (Ken) Ostrikov Department of Physics Research Institute for Biomimetics and Soft Matter Fujian Provincial Key Laboratory for Soft Functional Materials Jiujiang Research Institute Xiamen University School of Chemistry and Physics QUT Centre for Materials Science and QUT Centre for a Waste-Free World Queensland University of Technology(QUT) School of Chemical and Biomolecular Engineering University of Sydney

Ever-increasing emissions of anthropogenic carbon dioxide （CO2） cause global environmental and climate *** by biological photosynthesis,developing effective strategies NeuNlto up-cycle CO2into high-value organics is *** CO2reduction reaction （CO2RR） is highly promising to convert CO2into economically viable carbon-based chemicals or fuels under mild process conditions.

关键词： CO2RR conductive network electrocatalysts formate

Frontiers in high entropy alloys and high entropy functional materials

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Rare Metals 2024年第10期43卷 4639-4776页

作者： Wen-Tao Zhang Wen Huang Fu-Jie Yu Qi Zhao Xin-Dong Zhu Tao Feng Yao Jiang Xiao-Ming Li Xue-Fei Miao He Zhu Si Lan Xue-Qian Wang Bao-Long Shen Zhe Jia Feng-Qi Zhang Wei Wang Qi Liu Yang Ren Xun-Li Wang Xiao-Ya Cui Xiao-Yang Wang Ya-Nan Chen Bing-Bing Fan Meng-Ru Li Qi-Long Gao Jia-Ming Guo Zeng-Bao Jiao Zhi-Min Guo Yu-Ping Zhao Qian Yu Rui Huang Ling-Kun Zhang Yi-Ping Lu Xu-Bo Li Huai-Jun Lin Yan Ma Wei-Ming Yang Zhi-Hua Shen Hai-Yan He Yong-Gang Sun Yong-Jiang Huang De-Zhuang Wang Qing-Feng Liu Fei-Yang Wang Hui Liu Hong-Hui Wu Li-Qiang Wang Yang Lu Nan Wang Tian-Li Wang Wei-Bing Liao Yi-Han Wang Yuan Wu Yu-Zhen Yin Jie Pan Yi Zhang Qing Wang Jian-Yang Zhang Tao Yang Yasir Sohail Jin-Yu Zhang Hua Ji Qiang Li Wei-Di Liu Zhi-Gang Chen Xiong-Jun Liu Wen Ma Liang Mao Zhen-Duo Wu School of materials science and Engineering Nanjing University of Science and Technology Jiangsu Key Laboratory for Advanced Metallic materials School of Materials Science and Engineering Southeast University Department of Physics City University of Hong Kong School of materials science and Engineering Tianjin University School of Physics and Microelectronics Zhengzhou University Department of Mechanical Engineering Research Institute for Advanced Manufacturing The Hong Kong Polytechnic University Center of Electron Microscopy and State Key Laboratory of Silicon materials School of Materials Science and Engineering Zhejiang University Key Laboratory of Solidification Control and Digital Preparation Technology (Liaoning Province) School of Materials Science and Engineering Dalian University of Technology Institute of Advanced Wear & Corrosion Resistance and Functional materials Jinan University School of Mechanics and Civil Engineering China University of Mining and Technology School of Physical sciences Great Bay University School of materials science andEngineering Harbin Institute of Technology State Key Laboratory of materials-Oriented Chemical Engineering College of Chemical Engineering Nanjing Tech University Beijing Advanced Innovation Center for materials Genome Engineering Research Institute for Carbon Neutrality University of Science and Technology Beijing Department of Mechanical Engineering The University of Hong Kong School of Computing Macquarie University Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong Province College of Physics and Optoelectronic Engineering Shenzhen University State Key Laboratory for Advanced Metals and materials University of Science and Technology Beijing State Key Laboratory of materials Processing and Die & Mould Technology School of Materials Science and Engineering Huazhong University of Science and Technology Institute of materials Shanghai University Department of materials science and Engineering C

Owing to their exceptional properties, high-entropy alloys(HEAs) and high-entropy materials have emerged as promising research areas and shown diverse applications. Here,the recent advances in the field are comprehensively reviewed,organized into five sections. The first section introduces the background of HEAs, covering their definition, significance,application prospects, basic properties, design principles, and microstructure. The subsequent section focuses on cutting-edge high-entropy structural materials, highlighting developments such as nanostructured alloys, grain boundary engineering,eutectic systems, cryogenic alloys, thin films, micro-nano-lattice structures, additive manufacturing, high entropy metallic glasses, nano-precipitate strengthened alloys, composition modulation, alloy fibers, and refractory systems. In the following section, the emphasis shifts to functional materials, exploring HEAs as catalysts, magneto-caloric materials, corrosion-resistant alloys, radiation-resistant alloys, hydrogen storage systems, and materials for biomedicine. Additionally, the review encompasses functional high-entropy materials outside the realm of alloys, including thermoelectric, quantum dots, nanooxide catalysts, energy storage materials, negative thermal expansion ceramics,and high-entropy wave absorption materials. The paper concludes with an outlook, discussing future directions and potential growth areas in the field. Through this comprehensive review,researchers, engineers, and scientists may gain valuable insights into the recent progress and opportunities for further exploration in the exciting domains of high-entropy alloys and functional materials.

关键词： Cutting-edge structural materials Cutting-edgefunctional materials High entropy alloys

Recent advances towards aqueous hydrogen peroxide formation in a direct current plasma-liquid system

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High Voltage 2022年第3期7卷 405-419页

作者： Qiang Chen Junshuai Li Qiang Chen Kostya(Ken)Ostrikov Shenzhen Research Institute of Xiamen University Institute of Electromagnetics and AcousticsFujian Provincial Key Laboratory of Plasma and Magnetic ResonanceKey Laboratory of Electromagnetic Wave Science and Detection TechnologyXiamen UniversityXiamenChina LONGi Institute of Future Technology and School of materials&Energy Lanzhou UniversityLanzhouChina Laboratory of Plasma Physics and materials Beijing Institute of Graphic CommunicationBeijingChina School of Chemistry and Physics and qut centre for materials science Queensland University of Technology(QUT)BrisbaneQueenslandAustralia

The aqueous phase hydrogen peroxide(H_(2)O_(2aq))produced from the plasma-liquid interactions can directly or synergistically(with other substances)affect the liquid chemistry,and therefore it is important to unfold the H_(2)O_(2aq)formation ***,up to now,a consensus on the H_(2)O_(2aq)formation mechanism is not *** review aims to survey the recent advances on the understanding of the H_(2)O_(2aq)formation mechanism in the system of a direct current discharge plasma operated over a liquid *** and experimental analyses indicate that the recombination of dissolved OH radicals(OHaq)is the dominant process for the H_(2)O_(2aq)formation,while the purported plasma-induced photolysis of water and the dissolution of gaseous H_(2)O_(2)are ruled out.

关键词： hydrogen liquid system

Chlorine-anion doping induced multi-factor optimization in perovskites for boosting intrinsic oxygen evolution

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Journal of Energy Chemistry 2021年第1期30卷 115-120,I0004页

作者： Yinlong Zhu Qian Lin Zhenbin Wang Dongchen Qi Yichun Yin Yu Liu Xiwang Zhang Zongping Shao Huanting Wang Department of Chemical Engineering Monash UniversityClaytonVIC 3800Australia Department of Physics Technical University of Denmark2800 Kongens LyngbyDenmark School of Chemistry and Physics Centre for Materials ScienceQueensland University of TechnologyBrisbaneQueensland 4001Australia Department of Chemical Engineering Curtin UniversityPerthWestern Australia 6845Australia

The oxygen evolution reaction(OER) plays a crucial role in many electrochemical energy technologies,and creating multiple beneficial factors for OER catalysis is desirable for achieving high catalytic ***,we highlight a new halogen-chlorine(Cl)-anion doping strategy to boost the OER activity of perovskite *** a proof-of-concept,proper Cl doping at the oxygen site of LaFeO3(LFO) perovskite can induce multiple favorable characteristics for catalyzing the OER,including rich oxygen vacancies,increased electrical conductivity and enhanced Fe-O *** from these factors,the LaFeO2.9-δCl0.1(LFOCl) perovskite displays significant intrinsic activity enhancement by a factor of around three relative to its parent *** work uncovers the effect of Cl-anion doping in perovskites on promoting OER performance and paves a new way to design highly efficient electrocatalysts.

关键词： Anion doping Halogen chlorine Multiple beneficial factors Oxygen evolution reaction Perovskite oxide

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High energy superstable hybrid capacitor with a self-regulated Zn/electrolyte interface and 3D graphene-like carbon cathode

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InfoMat 2022年第10期4卷 62-77页

作者： Nilesh R.Chodankar Swati J.Patil Sangjin Lee Jaeho Lee Seung-Kyu Hwang Pragati A.Shinde Indrajit V.Bagal Smita V.Karekar Ganji Seeta Rama Raju Kugalur Shanmugam Ranjith Deepak P.Dubal Yun-Suk Huh Young-Kyu Han Department of Energy and Material Engineering Dongguk University-SeoulSeoulRepublic of Korea Department of Biological Engineering NanoBio High-Tech Materials Research CenterInha UniversityIncheonRepublic of Korea Department of Biological sciences and Bioengineering Inha UniversityIncheonRepublic of Korea Research Institute of sciences and Engineering University of SharjahSharjahUnited Arab Emirates Department of Physics Chonnam National UniversityGwangjuRepublic of Korea School of Chemistry and Physics Centre for Materials ScienceQueensland University of Technology(QUT)BrisbaneQueenslandAustralia

Rechargeable aqueous zinc ion hybrid capacitors(ZIHCs),as an up-and-comer aqueous electrochemical energy storage system,endure in their infancy because of the substandard reversibility of Zn anodes,structural deterioration of cathode materials,and narrow electrochemical stability ***,a scalable approach is described that addresses Zn-anode/electrolyte interface and cathode materials associated deficiencies and boosts the electrochemical properties of *** Zn-anode/electrolyte interface is self-regulated by alteration of the traditional Zn2+electrolyte with Na-based supporting salt without surrendering the cost,safety,and green features of the Zn-based system which further validates the excellent reversibility over 1100 h with suppressed hydrogen *** deficits of cathode materials were overcome by using a high-mass loaded,oxygen-rich,3D,multiscaled graphene-like carbon(3D MGC)*** to the multiscaled texture,high electronic conductivity,and oxygen-rich functional groups of 3D MGC,reversible redox capacitance was obtained with a traditional adsorption/desorption *** ZIHCs containing the modified electrolyte and an oxygen-rich 3D MGC cathode resulted in battery-like specific energy(203 Wh kg1 at 1.6 A g^(-1))and supercapacitor-type power capability(4.9 kW kg1 at 8 A g^(-1))with outstanding cycling durability(96.75%retention over 30000 cycles at 10 A g^(-1)).These findings pave the way toward the utilization of highly efficient ZIHCs for practical applications.

关键词： electrolyte additive graphene-like carbon interface multivalent ion capacitor zinc

Nanocarbon-Enhanced 2D Photoelectrodes:A New Paradigm in Photoelectrochemical Water Splitting

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Nano-Micro Letters 2021年第2期13卷 45-73页

作者： Jun Ke Fan He Hui Wu Siliu Lyu Jie Liu Bin Yang Zhongjian Li Qinghua Zhang Jian Chen Lecheng Lei Yang Hou Kostya Ostrikov Key Laboratory of Biomass Chemical Engineering of Ministry of Education College of Chemical and Biological EngineeringZhejiang UniversityHangzhou 310012People’s Republic of China School of Chemistry and Environmental Engineering Wuhan Institute of Technology206 Guanggu 1st RoadWuhan 430205People’s Republic of China Department of Environmental science and Engineering North China Electric Power University619 Yonghua N StBaoding 071003People’s Republic of China Institute of Zhejiang University-Quzhou Quzhou 324000People’s Republic of China Ningbo Research Institute Zhejiang UniversityHangzhou 315100People’s Republic of China State Key Laboratory of Industrial Control Technology College of Control Science and EngineeringZhejiang UniversityHangzhou 310012People’s Republic of China School of Chemistry and Physics and centre for materials science Queensland University of TechnologyBrisbaneQLD 4000Australia

Solar-driven photoelectrochemical(PEC)water splitting systems are highly promising for converting solar energy into clean and sustainable chemical *** such PEC systems,an integrated photoelectrode incorporates a light harvester for absorbing solar energy,an interlayer for transporting photogenerated charge carriers,and a co-catalyst for triggering redox ***,understanding the correlations between the intrinsic structural properties and functions of the photoelectrodes is *** we critically examine various 2D layered photoanodes/photocathodes,including graphitic carbon nitrides,transition metal dichalcogenides,layered double hydroxides,layered bismuth oxyhalide nanosheets,and MXenes,combined with advanced nanocarbons(carbon dots,carbon nanotubes,graphene,and graphdiyne)as co-catalysts to assemble integrated photoelectrodes for oxygen evolution/hydrogen evolution *** fundamental principles of PEC water splitting and physicochemical properties of photoelectrodes and the associated catalytic reactions are *** strategies for the assembly of 2D photoelectrodes with nanocarbons to enhance the PEC performances are *** mechanisms of interplay of 2D photoelectrodes and nanocarbon co-catalysts are further *** challenges and opportunities in the field are identified to guide future research for maximizing the conversion efficiency of PEC water splitting.

关键词： Advanced nanocarbons Co-catalysts 2D layered structure Integrated photoelectrodes Photoelectrochemical water splitting

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Plasma-enabled synthesis of ordered PtFe alloy nanoparticles encapsulated with ultrathin N-doped carbon shells for efficient methanol electrooxidation

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Nano Research 2023年第2期16卷 2065-2075页

作者： Xuxu Sun Zhijian Mao Ruiqi Wang Xiaohu Pi Changle Chen Junbo Zhong Qi Wang Kostya(Ken)Ostrikov Institute of Plasma Physics Hefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China University of science and Technology of China Hefei 230026China Rutgers Preparatory School New Jersey1345 Easton AveSomersetNJ 08873USA Institute of Intelligent Machines Hefei Institutes of Physical ScienceChinese Academy of SciencesHefei 230031China College of Chemical Engineering Sichuan University of Science and EngineeringZigong 643000China School of Chemistry and Physics and qut centre for materials science Queensland University of Technology(QUT)BrisbaneQLD 4000Australia

Methanol oxidation reaction(MOR),the key reaction for clean energy generation in fuel cells,is kinetically sluggish and short-lasting because of insufficient catalytic activity and stability of the common Pt-based *** Pt alloy structures which promise to surmount these issues,are challenging and impractical to fabricate using common high-temperature *** address the urgent need for simple and rapid synthesis methods for such alloys,here we report the versatile plasma-assisted thermal annealing synthesis of a robust electrocatalyst with PtFe alloys supported on N-doped carbon nanotubes(denoted as PtFe@NCNT-P).Benefiting from the reactive plasma-specific effects,the PtFe@NCNT-P electrocatalyst features ultrafine PtFe alloy nanoparticles(mean size~2.88 nm,ordered degree~87.07%)and ultrathin N-doped carbon(NC)shells(0.3–0.7 nm),leading to the excellent catalytic activity and stability toward *** catalyst shows the specific and mass activities of 3.99 mA/cm^(2)and 2,148.5 mA/mg,which are 7.82 and 7.41 times higher than those for commercial Pt/C(0.51 mA/cm^(2),290 mA/mg),and 2.18 and 2.59 times higher compared to the plasma-untreated PtFe@NCNT(1.83 mA/cm2,829.5 mA/mg),*** PtFe@NCNT-P further exhibits extraordinary stability during the long-term chronoamperometry test and 1,000-cycle cyclic voltammetry scanning,much better compared to PtFe@NCNT samples even after the longer thermal *** findings show great potential of the plasma-enabled synthesis of high-performance carbon-supported metallic electrocatalysts for the emerging clean energy technologies.

关键词： methanol oxidation reaction highly ordered PtFe alloy nanoparticles ultrathin N-doped carbon shell N-doped carbon support plasma nanotechnology

Multidimensional Ni-Co-sulfide heterojunction electrocatalyst for highly efficient overall water splitting

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science China materials 2022年第9期65卷 2421-2432页

作者： Wenxia Chen Yingjie Hu Peng Peng Jinhai Cui Junmei Wang Wei Wei Yongya Zhang Kostya(Ken)Ostrikov Shuang-Quan Zang School of Chemistry and Chemical Engineering Henan Engineering Center of New Energy Battery MaterialsShangqiu Normal UniversityShangqiu 476000China Henan Key Laboratory of Crystalline Molecular Functional materials Henan International Joint Laboratory of Tumor Theranostical Cluster MaterialsGreen Catalysis Center and College of ChemistryZhengzhou UniversityZhengzhou 450001China Key Laboratory of Advanced Functional materials of Nanjing Nanjing Xiaozhuang UniversityNanjing 211171China School of Chemistry and Physics and centre for materials science Queensland University of TechnologyBrisbaneQLD 4000Australia

Heterostructure engineering holds exceptional promise for the development of high-performance electrocatalysts for overall water ***,production of inexpensive and high-efficiency bifunctional electrocatalysts remains a ***,we demonstrate a simple method to synthesize a paper-mulberry(Broussonetia papyrifera)-inspired Co_(9)S_(8)@CoNi_(2)S_(4)/nickel foam(Co_(9)S_(8)@CoNi_(2)S_(4)/NF)heterojunction with high catalytic activity and *** process involves in situ growth of NiCo layered double hydroxide and in situ derivatization of ZIF-67,followed by the S heteroatom *** Co_(9)S_(8)@CoNi_(2)S_(4)/NF benefits from the heterostructure and functional advantages of multidimensional building blocks including one-dimensional(1D)nanowires,2D nanosheets and *** optimized Co_(9)S_(8)@CoNi_(2)S_(4)/NF heterojunction with 10% sulphur content reveals excellent electrocatalytic activity with the lower overpotentials of 68 mV for hydrogen evolution reaction(HER)and 170 mV for oxygen evolution reaction(OER)at 10 mA cm^(-2) in the 1.0 mol L^(-1) KOH solution,which is superior to the recently reported transition metal based *** outstanding performance is attributed to the strong interface coupling between CoNi_(2)S_(4) and Co_(9)S_(8),the advantage of multidimensional structure and the customized electronic *** density functional theory suggests that the interface between Co_(9)S_(8) and CoNi_(2)S_(4) optimizes the adsorption of the multiple intermediates and further facilitates water splitting *** work offers a generic approach for heterostructure engineering design of highperformance catalytic system applications.

关键词： heterojunction heteroatom doping multidimensional nanostructure electrocatalysts overall water splitting

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