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Understanding amorphous PrO_(x)-based N-doped carbon catalyst as an efficient electrocatalyst for oxygen reduction reaction

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Journal of Rare Earths 2025年第1期43卷 73-80,I0003页

作者： Xiao Man Ying Chang Shaohong Guo Meilin Jia Jingchun Jia inner mongolia Key Laboratory of Green Catalysis and inner mongolia Collaborative Innovation Center for Water Environment Safety College of Chemistry and Environmental ScienceInner Mongolia Normal UniversityHohhot010022China

The development of an e fficacious and easily prepared no nprecious metal electrocatalyst is crucial for the oxygen reduction reaction(ORR).This work used a dual template method to prepare the amorphous rare earth-based catalyst PrO_(x)-NC,and optimized the calcination temperature and *** PrO_(x)-NC-900 catalyst has high durability and activity and exhibits superior ORR performance in alkaline electrolytes with an onset potential(E_(0))of 0.96 V and a half-wave potential(E_(1/2))of 0.85 *** research results indicate that the ORR performance of rare earth oxide composite carbon catalysts can be improved by adjusting oxygen vacancies(Ov).In addition,high specific surface area,N rich defect *** oxygen vacancies,and the synergistic effect of oxygen vacancies and N-doped carbon interfacial layer play a significant part in the enhancement of *** performance of the zinc air battery assembled with PrO_(x)-NC-900 is significantly improved,and rare earth oxides and carbon frameworks originating from metal organic frameworks(MOFs)contribute to the oxygen electrocatalyst and electron transfer rate of the zinc air *** catalyst provides promising information for the development of rare earth metal oxide nanostructures as potential candidate materials for ORR in alkaline media.

关键词： Rare earths Metal-organic framework Oxygen reduction reaction Zn-air batteries

Microstructure and electrochemical hydrogen storage properties of nanosized doped La2Ti2O7 solid solutions

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Journal of Rare Earths 2025年第2期43卷 354-361页

作者： Guofang Zhang Jianyi Xu Shilong Sun Yiming Li Zhuocheng Liu Ruihua Guo Zhiyong Yang Lu Bai Yanghuan Zhang School of Materials and Metallurgy Inner Mongolia University of Science and Technology

Hydrothermal-sintering method was employed to obtain pure and Li,Co,Mn,Cu and Zn doped La2Ti2O7solid *** substitution sites of doping ions are discussed.X-ray diffraction（XRD） results indicate that the doped ions were incorporated into the lattice of *** electron microscopy（TEM） measurements prove that the doped ions with smaller radius induce the contraction of *** re sults of UV and photo luminescence（PL） tests show that the doped ions cause the red-shift of band gap energies and enhance the concentrations of oxygen vacancies and *** electrochemical hydrogen storage properties of the samples were measured at 303 and 333 K,*** discharge capacities of the doped samples keep growing by increasing the cycle number at 333 ***,the doped samples possess better kinetic performances than the pure *** the samples,the Mn,Co and Li ions doped samples exhibit better electrochemical hydrogen storage *** hydrogen storage properties are closely related with the characteristics of doped ions,crystallite sizes,the content of the oxygen vacancies and defects in the lattice of La2Ti2O7.

关键词： Discharge capacity Doped La2Ti2O7 Electrochemical hydrogen storage property Oxygen vacancy Rare earths

Some Eigenvalue Properties of Third-order Boundary Value Problems with Distributional Potentials

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Acta Mathematicae Applicatae Sinica 2025年第1期41卷 179-199页

作者： Hai-yan ZHANG Ji-jun AO College of sciences Inner Mongolia University of TechnologyHohhot 010051China

Several eigenvalue properties of the third-order boundary value problems with distributional potentials are ***,we prove that the operators associated with the problems are self-adjoint and the corresponding eigenvalues are ***,the continuity and differential properties of the eigenvalues of the problems are given,especially we find the differential expressions for the boundary conditions,the coefficient functions and the ***,we show a brief application to a kind of transmission boundary value problems of the problems studied here.

关键词： third-order boundary value problems distributional potentials quasi-derivatives eigenvalues

Bilevel Optimal Scheduling of Island Integrated Energy System Considering Multifactor Pricing

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Energy Engineering 2025年第1期122卷 349-378页

作者： Xin Zhang Mingming Yao Daiwen He Jihong Zhang Peihong Yang Xiaoming Zhang School of Automation and Electrical Engineering Inner Mongolia University of Science and TechnologyBaotou014010China

In this paper,a bilevel optimization model of an integrated energy operator(IEO)–load aggregator(LA)is constructed to address the coordinate optimization challenge of multiple stakeholder island integrated energy system(IIES).The upper level represents the integrated energy operator,and the lower level is the electricity-heatgas load *** to the benefit conflict between the upper and lower levels of the IIES,a dynamic pricing mechanism for coordinating the interests of the upper and lower levels is proposed,combined with factors such as the carbon emissions of the IIES,as well as the lower load interruption *** price of selling energy can be dynamically adjusted to the lower LA in the mechanism,according to the information on carbon emissions and load interruption *** benefits and win-win situations are achieved between the upper and lower ***,CPLEX is used to iteratively solve the bilevel optimization *** optimal solution is selected according to the joint optimal discrimination *** results indicate that the sourceload coordinate operation can reduce the upper and lower operation *** the proposed pricingmechanism,the carbon emissions and load interruption power of IEO-LA are reduced by 9.78%and 70.19%,respectively,and the capture power of the carbon capture equipment is improved by 36.24%.The validity of the proposed model and method is verified.

关键词： Bilevel optimal scheduling load aggregator integrated energy operator carbon emission dynamic pricing mechanism

Femtosecond mode-locking and soliton molecule generation based on a GaAs saturable absorber

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Chinese Physics B 2025年第1期34卷 344-349页

作者： Chen-Yan Zhang Xin-He Dou Zhen Chen Jing-Han Zhao Wei Sun Ze-Yu Fan Tao Zhang Hao Teng Zhi-Guo Lv School of Physical science and Technology Inner Mongolia UniversityHohhot 010021China Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China

In the last few years,research on advanced ultrafast photonic devices has attracted great interest from laser *** a semiconductor material with excellent nonlinear saturation absorption characteristics,Ga As has been used in solidstate and fiber lasers as a ***,the pulse widths that have been reported in the searchable published literature are all long and the shortest is tens of *** pulse widths,desired for a variety of applications,have not yet been reported in Ga As-based pulsed *** this work,we further explore the nonlinear characteristics of Ga As that has been magnetron sputtered onto the surface of a tapered fiber and its application in the generation of femtosecond lasing via effective dispersion optimization and nonlinearity *** the enhanced interaction between evanescent waves and Ga As nanosheets,mode-locked soliton pulses as short as 830 fs are generated at repetition rates of 4.64 *** far as we know,this is the first time that femtosecond-level pulses have been generated with a Ga As-based saturable *** addition,soliton molecules,including in the dual-pulse state,are also realized under stronger *** work demonstrates that Ga As-based photonic devices have good application prospects in effective polymorphous ultrashort pulsed laser generation.

关键词： GaAs saturable absorber mode-locking soliton molecule

Boosting hydrocarbon conversion via Cu-doping induced oxygen vacancies on CeO_(2) in CO_(2)electroreduction

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Journal of Energy Chemistry 2025年第1期100卷 66-76页

作者： Lei Xue Tong Shi Chenhui Han Heng Zhang Fenrong Liu Haorun Li Yan Wang Xiaojun Gu Shanghong Zeng inner mongolia Key Laboratory of Chemistry and Physics of Rare Earth Materials School of Chemistry and Chemical EngineeringInner Mongolia UniversityHohhot 010021Inner MongoliaChina State Key Laboratory of Coal Conversion Institute of Coal ChemistryChinese Academy of SciencesTaiyuan 030001ShanxiChina Institute of Catalysis Department of ChemistryZhejiang UniversityHangzhou 310058ZhejiangChina National Key Laboratory of Baiyunobo Rare Earth Resource Research and Comprehensive Utilization Baotou Research Institute of Rare EarthsBaotou 014030Inner MongoliaChina

Conversion of CO_(2)back to hydrocarbons is the most direct way of closing the“carbon cycle”,and its significance is further enlarged if this process is driven by renewable energies such as ***,precisely controlling the product selectivity towards hydrocarbons against the competitive hydrogen evolution remains challenging,especially for Cu-based ***,we report a novel defect engineering strategy,by which Cu-doping-induced oxygen vacancies on CeO_(2)nanorods were effectively created,with adjustable vacancy/Cu *** resulting optimum catalyst shows up to 79%catalytic current density to hydrocarbons(excluding CO),with 49%faradaic efficiency to *** and density functional theory unveil that the ratio between oxygen vacancy and Cu affects significantly the formation of*CHO and activation of H2O,which leads to the following deep hydrogenation to *** findings may spur new insights for designing and developing more controllable chemical process relevant to CO_(2)utilization.

关键词： Cu/CeO_(2)-x Oxygen vacancy Hydrocarbon production Reaction mechanism

Activation of peroxymonosulfate by sustainable biomass-based carbon nanotubes for controlling the spread of plant viruses in water environments

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Journal of Environmental sciences 2025年第3期149卷 99-112页

作者： Jian Tang Yujie Wang JunMa Yujie Chen Ming Chen College of Resources and Environment Yangtze UniversityWuhan 430100China Key Laboratory of Reservoir Aquatic Environment Chongqing Institute of Green and Intelligent TechnologyChinese Academy of SciencesChongqing 400714China Chongqing School University of Chinese Academy of SciencesChongqing 400714China School of Geography and Tourism Chongqing Normal UniversityChongqing 400714China

With the increasing demand for water in hydroponic systems and agricultural irrigation,viral diseases have seriously affected the yield and quality of *** removing plant viruses in water environments,virus transmission can be prevented and agricultural production and ecosystems can be *** so far,there have been few reports on the removal of plant viruses in water ***,in this study,easily recyclable biomass-based carbon nanotubes catalysts were synthesized with varying metal activities to activate peroxymonosulfate(PMS).Among them,the magnetic 0.125Fe@NCNTs-1/PMS system showed the best overall removal performance against pepper mild mottle virus,with a 5.9 log_(10)removal within 1 ***,the key reactive species in the 0.125Fe@NCNTs-1/PMS system is^(1)O_(2),which can maintain good removal effect in real water matrices(river water and tap water).Through RNA fragment analyses and label free analysis,it was found that this system could effectively cleave virus particles,destroy viral proteins and expose their *** capsid protein of pepper mild mottle virus was effectively decomposed where serine may be the main attacking sites by^(1)O_(2).Long viral RNA fragments(3349 and 1642 nt)were cut into smaller fragments(∼160 nt)and caused their *** summary,this study contributes to controlling the spread of plant viruses in real water environment,which will potentially help protect agricultural production and food safety,and improve the health and sustainability of ecosystems.

关键词： Pepper mild mottle virus Removal Plant virus spread Biomass-based carbon nanotubes Water environments

Li,Na,and Cs-based metal-organic frameworks for room temperature phosphorescence applications

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science China Chemistry 2025年

作者： Jiaqi Ma Rui Feng Yanyuan Jia Mingshi Zhang Shuo Guo College of Chemistry and Chemical Engineering Inner Mongolia University School of Materials science and Engineering Smart Sensing Interdisciplinary Science Center Nankai University & TKL of Metal and Molecule Based Material Chemistry Key Laboratory of Advanced Energy Materials Chemistry (Ministry of Education) Nankai University Department of Chemistry and Biochemistry University of California San Diego

The conventional design of metal-organic frameworks (MOFs) with room-temperature phosphorescence (RTP) mostly relies on using heavy metals,as the heavy atom effect can effectively increase the efficiency of intersystem crossing (ISC) to get a better phosphorescence *** the first time,we reported the highly efficient RTP of a lithium-based MOF IMU-101 with a lifetime (τ) of 299 ms and a quantum yield (QY) of 4.91%.In addition,MOFs IMU-102 and IMU-103,with sodium and cesium as metal nodes,were successfully *** phosphorescence properties of this series of alkali metal MOFs were systematically studied and *** crystallography and computational calculation show that the mechanism for achieving RTP for this material lies in the ultrashort coordination bond of Li,which enables the reduction of non-radiative ***-101,as a cheap and environmentally friendly room-temperature phosphorescent material,has been further developed into composite polymer inks and bulk *** makes them promising for applications in anti-counterfeiting and information encryption.

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Using fracture mechanics method to analyze the failure mechanism and equilibrium equation of interfacial loess-mudstone landslides

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Journal of Mountain science 2025年第1期22卷 156-166页

作者： LI Shuanhu LI Chi GAO Yu Key Laboratory of Geological Hazards and Geotechnical Engineering Defense in Sandy and Drought Regions at Universities of inner mongolia Autonomous Region Inner Mongolia University of TechnologyHohhot 010051China inner mongolia Engineering Research Center of Geological Technology and Geotechnical Engineering Inner Mongolia University of TechnologyHohhot 010051China College of Resource and Environmental Engineering Inner Mongolia University of TechnologyHohhot 010051China

Loess-mudstone landslides are common in the Loess *** into the mechanical theory of loess-mudstone landslides have become a challenging undertaking due to the distinctive interfacial properties of loess-mudstone and the unique water sensitivity characteristics of ***,it is imperative to develop innovative mechanical models and mathematical equations specifically tailored to loess-mudstone *** this study,we analyze the fracture mechanism of the loess-mudstone sliding zone using plastic fracture mechanics and develop a unique fracture yield *** calculate the energy release rate during the expansion of the loess-mudstone interface tip region,the shear fracture energy G is applied,which reflects both the yield failure criterion and the fracture failure *** better understand the instability mechanism of loess-mudstone landslides,equilibrium equations based on G are established for tractive,compressive,and tensile loess-mudstone *** on the equilibrium equation,the critical length Lc of the sliding zone can be used for the safety evaluation of loess-mudstone *** this way,this study proposes a new method for determining the failure mechanism and equilibrium equation of loessmudstone landslides,which resolves their starting mechanism,mechanical equilibrium equations,and safety evaluation indicators,thus justifying the scientific significance and practical value of this research.

关键词： Loess-mudstone landslide Failure mechanism Shear fracture energy Equilibrium equation Safety factor