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Progress in Natural Science:Materials International 2024年第03期34卷 512-523页

作者： Xin Tong Hao Ye Yunrou Wu Xinxing Zhan Manqi Gu Shixia Luo Jiangning Gong Juan Tiana Yadian Xie School of Chemistry and Material Science Guizhou Normal University Center for the Physics of Low-Dimensional Materials School of Physics and Electronics School of Future Technology Henan University Key Laboratory of Low-Dimensional Materials and Big Data Guizhou Minzu University

High-entropy alloy nanoparticles(HEA-NPs) have recently sparked great interest in materials science. Their solidsolution states, derived from distinct HEA configurations, make them promising candidates for catalysts with exceptional activity, stability, and tunable performance. However, a comprehensive understanding of the underlying mechanisms governing their electrocatalytic behavior is still lacking, hindering the rational design of HEA electrocatalysts. This review summarizes the fundamental knowledge of HEA-NPs, including the structureactivity correlations of HEA-NPs, diverse synthesis strategies, and applications in electrochemical catalysis. The design strategies for guiding improvements in tunable performance were highlighted. The article concludes with insights, perspectives, and future directions, encapsulating the state-of-the-art knowledge and paving the way for further exploration in this dynamic field.

关键词： High-entropy alloy nanoparticles Structure-activity correlations Synthesis strategies Electrochemical catalysis

BioTreasury:a community-based repository enabling indexing and rating of bioinformatics tools

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Science China(Life Sciences) 2024年第2期67卷 221-229页

作者： Qi Zhao Xin Zhou Jingxing Wu Jieyi Cai Xiaoqiong Bao Lin Tang Chaoye Wang Chunlei Liu Yukai Wang Yuyan Teng Mohan Zheng Weiping Mu Zhixiang Zuo Yubin Xie Xiaotong Luo Jian Ren School of Life Sciences State Key Laboratory of Oncology in South ChinaCancer CenterGuangdong Provincial Clinical Research Center for CancerSun Yat-sen UniversityGuangzhou 510060China Institute of Precision Medicine The First Affiliated HospitalSun Yat-sen UniversityGuangzhou 510080China Guangdong Institute of Gastroenterology Department of General SurgeryGuangdong Provincial Key Laboratory of Colorectal and Pelvic Floor DiseasesThe Sixth Affiliated HospitalSun Yat-sen UniversityGuangzhou 510275China

The exponential growth of bioinformatics tools in recent years has posed challenges for scientists in selecting the most suitable one for their data analysis ***,to aid scientists in making informed choices,a community-based platform that indexes and rates bioinformatics tools is urgently *** this study,we introduce Bio Treasury(http://***),an integrated communitybased repository that provides an interactive platform for users and developers to share their experiences in various bioinformatics *** Treasury offers a comprehensive collection of well-indexed bioinformatics software,tools,and databases,totaling over 10,000 *** the past two years,we have continuously improved and maintained Bio Treasury,adding several exciting features,including creating structured homepages for every tool and user,a hierarchical category of bioinformatics tools and classifying tools using large language model(LLM).Bio Treasury streamlines the tool submission process with intelligent ***,Bio Treasury provides a wide range of social features,for example,enabling users to participate in interactive discussions,rate tools,build and share tool collections for the *** believe Bio Treasury can be a valuable resource and knowledge-sharing platform for the biomedical *** empowers researchers to effectively discover and evaluate bioinformatics tools,fostering collaboration and advancing bioinformatics research.

关键词： bioinformatics tools index tool database rating system large language model tool collections shari

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Recent advances and trends of single-atom catalysts for proton exchange membrane fuel cell cathodes

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ChemPhysMater

ChemPhysMater 2024年第2期3卷 143-156页

作者： Zihao Wan Feng Liu Hongfei Xu Shuaili Zhao Zhen An Zizai Ma Zhonghua Zhang Yun Wu Xiaoguang Wang Laboratory of Advanced Materials and Energy Electrochemistry Institute of New Carbon MaterialsCollege of Material Science and EngineeringTaiyuan University of TechnologyTaiyuan 030024China Datong Innoreagen Power Technology Co. LtdDatong 037000China College of Chemistry Taiyuan University of TechnologyTaiyuan 030024China Shanxi Key Laboratory of Gas Energy Efficient and Clean Utilization Taiyuan University of TechnologyTaiyuan 030024China Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan250061China Department of Materials Science and Engineering Guangdong University of Petrochemical TechnologyMaoming 525000China

Proton exchange membrane fuel cells(PEMFCs),which have the advantages of high-power density,zero emission,and low noise,are considered ideal electrochemical conversion systems for converting hydrogen(H2)and oxy-gen(O_(2))/air into ***,the oxygen reduction reaction(ORR),which is accompanied by multiple electrons,results in voltage loss and low conversion efficiency of ***,PEMFCs mainly use high-load precious platinum(Pt)to promote the ORR process;however,the high cost of Pt hinders the widespread commercialization of *** the past few years,metal-nitrogen-carbon single-atom catalysts(M-N-C SACs)have attracted considerable attention and have been recognized as potential Pt-based catalysts owing to their outstanding ORR *** review briefly introduces the components of ***,we discuss the catalytic mechanisms of the M-N-C SACs for the ***,the latest advances in noble,non-noble,and heteroatom-doped M-N-C SACs used as ORR and PEMFCs cathode catalysts are systematically *** sum-mary,we have outlined the current challenges and proposed a future perspective of M-N-C SACs for PEMFCs cathodes.

关键词： Proton exchange membrane fuel cells Oxygen reductionreaction Cathode Platinum-based catalysts Metal-nitrogen-carbon single-atom catalysts

Boosting Li-ion storage kinetics via constructing layered TiO_(2) anode

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Particuology 2024年第10期93卷 22-29页

作者： Jiyue Hou Fei Wang Enfeng Zhang Ying Wang Peng Dong Yunxiao Wang Yiyong Zhang Xue Li Yingjie Zhang national and Local Joint Engineering Research Center of Lithium-ion Batteries and Materials Preparation Technology Faculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming650093China College of Electrical Information Engineering Panzhihua UniversityPanzhihua617000China University Wollongong Australian Inst Innovat MatInst Superconducting&Elect MatInnovat Campus Squires WayWollongongNSW2500Australia

Due to the typical intercalation-deintercalation mechanism,TiO_(2) holds great promise as a sustainable anode for next-generation lithium-ion batteries(LIBs).However,commercial TiO_(2)(C–TiO_(2))is granular and shows slow ionic conductivity,which greatly hinders its development due to sluggish kinetics,leading to low reversible capacity and inferior rate *** this study,a two-dimensional layered TiO_(2)(L-TiO_(2))anode is prepared via a one-step calcination process,which can effectively shorten the lithium ions diffusion path and improve its lithium ions *** elucidated the enhanced electrochemical performance of L-TiO_(2) as an anode in LIBs through pseudocapacitive acceleration of lithium ions intercalation and deintercalation using various characterization techniques,including different scan rate cyclic voltammetry tests,in situ electrochemical impedance spectroscopy,in situ Raman spectroscopy,and in situ X-ray *** comparison to C–TiO_(2) material,L-TiO_(2) material showcases remarkable electrochemical performance,achieving a capacity of 166 mAh/g after 100 cycles at 0.1 ***,the lithium-ion diffusion coefficient calculated for the L-TiO_(2) is two orders of magnitude greater,underscoring its potential as a negative electrode material for LIBs.

关键词： Lithium-ionbatteries Anode MXene Layered TiO_(2)

6DOF pose estimation of a 3D rigid object based on edge-enhanced point pair features

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Computational Visual Media 2024年第1期10卷 61-77页

作者： Chenyi Liu Fei Chen Lu Deng Renjiao Yi Lintao Zheng Chenyang Zhu Jia Wang Kai Xu College of Computing National University of Defense TechnologyChangsha410073China Department of Spine Surgery the Second Xiangya HospitalCentral South UniversityChangsha410011China Clinical Nursing Teaching and Research Section the Second Xiangya HospitalChangsha410011China College of Meteorology and Oceanography National University of Defense TechnologyChangsha410073China Beijing Institute of Tracking and Communication Technology Beijing100094China

The point pair feature(PPF)is widely used for 6D pose *** this paper,we propose an efficient 6D pose estimation method based on the PPF *** introduce a well-targeted down-sampling strategy that focuses on edge areas for efficient feature extraction for complex geometry.A pose hypothesis validation approach is proposed to resolve ambiguity due to symmetry by calculating the edge matching *** perform evaluations on two challenging datasets and one real-world collected dataset,demonstrating the superiority of our method for pose estimation for geometrically complex,occluded,symmetrical *** further validate our method by applying it to simulated punctures.

关键词： point pair feature(PPF) pose estimation object recognition 3D point cloud

An integrable generalization of the Fokas–Lenells equation:Darboux transformation, reduction and explicit soliton solutions

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Chinese Physics B 2024年第7期33卷 117-124页

作者：魏姣耿献国王鑫 School of Mathematics and Statistics Zhengzhou UniversityZhengzhou 450001China School of Mathematics and Information Science Zhongyuan University of TechnologyZhengzhou 450007China

Under investigation is an integrable generalization of the Fokas–Lenells equation, which can be derived from the negative power flow of a 2 × 2 matrix spectral problem with three potentials. Based on the gauge transformation of the matrix spectral problem, one kind of Darboux transformation with multi-parameters for the three-component coupled Fokas–Lenells system is constructed. As a reduction, the N-fold Darboux transformation for the generalized Fokas–Lenells equation is obtained, from which the N-soliton solution in a compact Vandermonde-like determinant form is given. Particularly,the explicit one-and two-soliton solutions are presented and their dynamical behaviors are shown graphically.

关键词： Darboux transformation soliton solutions generalized Fokas–Lenells equation

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Ten-Minute Synthesis of a New Redox-Active Aqueous Binder for Flame-Retardant Li-S Batteries

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Energy & Environmental Materials 2024年第2期7卷 48-57页

作者： Tianpeng Zhang Borui Li Zihui Song Wanyuan Jiang Siyang Liu Runyue Mao Xigao Jian Fangyuan Hu School of Materials Science and Engineering State Key Laboratory of Fine ChemicalsFrontiers Science Center for Smart Materials Oriented Chemical Engineering Technology Innovation Center of High Performance Resin Materials(Liaoning Province)Key Laboratory of Energy Materials and Devices(Liaoning Province)Dalian University of TechnologyDalian 116024China State Key Laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringSchool of Chemical Engineering Technology Innovation Center of High Performance Resin Materials(Liaoning Province)Key Laboratory of Energy Materials and Devices(Liaoning Province)Dalian University of TechnologyDalian 116024China

As a critical role in battery systems,polymer binders have been shown to efficiently suppress the lithium polysulfide shuttling and accommodate volume changes in recent ***,preparation processes and safety,as the key criterions for Li-S batteries'practical applications,still attract less ***,an aqueous multifunction binder(named PEI-TIC)is prepared via an easy and fast epoxy-amine ring-opening reaction(10 min),which can not only give the sulfur cathode a stable mechanical property,a strong chemical adsorption and catalytic conversion ability,but also a fire safety *** Li-S batteries based on the PEI-TIC binder display a high discharge capacity(1297.8 mAh g^(-1)),superior rate performance(823.0 mAh g^(-1)at 2 C),and an ultralow capacity decay rate of 0.035%over more than 800 *** under 7.1 mg cm^(-2)S-loaded,the PEI-TIC electrode can also achieve a high areal capacity of 7.2 mA h g^(-1)and excellent cycling stability,confirming its application ***,it is also noted that TG-FTIR test is performed for the first time to explore the flame-retardant mechanism of polymer *** work provides an economically and environmentally friendly binder for the practical application and inspires the exploration of the flame-retardant mechanism of all electrode components.

关键词： 3D cross-linked network environmentally friendly flame retardant Li-S batteries multifunction binder

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Insights into the history and tendency of glycosylation and digestive system tumor:A bibliometric-based visual analysis

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World Journal of Gastrointestinal Oncology 2024年第3期16卷 1059-1075页

作者： Jie Jiang Zai Luo Ren-Chao Zhang Yue-Ling Wang Jun Zhang Ming-Yu Duan Zheng-Jun Qiu Chen Huang Department of Gastrointestinal Surgery Shanghai General HospitalShanghai Jiao Tong University School of MedicineShanghai 200080China Jiangnan University Wuxi School of Medicine Wuxi 214122Jiangsu ProvinceChina Department of Education Shanghai General HospitalShanghai Jiao Tong University School of MedicineShanghai 200080China

BACKGROUND Glycosylation,a commonly occurring post-translational modification,is highly expressed in several tumors,specifically in those of the digestive system,and plays a role in various cellular pathophysiological *** the importance and detection methods of glycosylation in digestive system tumors have garnered increasing attention in recent years,bibliometric analysis of this field remains *** present study aims to identify the developmental trends and research hotspots of glycosylation in digestive system *** To find and identify the developmental trends and research hotspots of glycosylation in digestive system *** We obtained relevant literature from the Web of Science Core Collection and employed VOSviewer 1.6.19 and CiteSpace(version 6.1.R6)to perform bibliometric *** A total of 2042 documents spanning from 1978 to the present were analyzed,with the research process divided into three phases:the period of obscurity(1978-1990),continuous development period(1991-2006),and the rapid outbreak period(2007-2023).These documents were authored by researchers from 66 countries or regions,with the United States and China leading in terms of publication *** Celso A had the highest number of publications,while Pinho SS was the most cited ***-occurrence analysis revealed the most popular keywords in this field are glycosylation,expression,cancer,colorectal cancer,and pancreatic ***,the Journal of Proteome Research was the most prolific journal in terms of publications,while the Journal of Biological Chemistry had the most *** The bibliometric analysis shows current research focus is primarily on basic research in this ***,future research should aim to utilize glycosylation as a target for treating tumor patients.

关键词： Glycosylation Cancer Digestive system Bibliometric analysis CiteSpace VOS viewer

Monolithic integrated optoelectronic chip for vector force detection

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Microsystems & Nanoengineering 2024年第3期10卷 245-257页

作者： Jiansong Feng Zhongqi Wang Mengyuan Zhanghu Xu Zhang Yong Shen Jing Yang Zhibin Li Bin Chen Taihong Wang Xiaolong Chen Zhaojun Liu Department of Electrical and Electronic Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Electrical and Electronic Engineering The University of Hong KongHong KongChina

Sensors with a small footprint and real-time detection capabilities are crucial in robotic surgery and smart wearable *** device footprint while maintaining its high performance is a major challenge and a significant limitation to their ***,we proposed a monolithic integrated micro-scale sensor,which can be used for vector force *** sensor combines an optical source,four photodetectors,and a hemispherical silicone elastomer component on the same sapphire-based AlGaInP *** chip-scale optical coupling is achieved by employing the laser lift-off techniques and the flip-chip bonding to a processed sapphire *** hemispherical structure device can detect normal and shear forces as low as 1mN within a measurement range of 0–220 mN for normal force and 0–15 mN for shear *** packaging,the sensor is capable of detecting forces over a broader range,with measurement capabilities extending up to 10 N for normal forces and 0.2 N for shear *** has an accuracy of detecting a minimum normal force of 25 mN and a minimum shear force of 20 ***,this sensor has been validated to have a compact footprint of approximately 1.5 mm^(2),while maintaining high real-time *** also demonstrate its promising potential by combining this sensor with fine surface texture perception in the fields of compact medical robot interaction and wearable devices.

关键词： robot force smart

Evaluation of the energy budget of thermokarst lake in permafrost regions of the Qinghai-Tibet Plateau

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Advances in Climate Change Research 2024年第4期15卷 636-646页

作者： Ze-Yong GAO Fu-Jun NIU Yi-Bo WANG Jing LUO Guo-An YIN Yun-Hu SHANG Zhan-Ju LIN Key Laboratory of Cryospheric Science and Frozen Soil Engineering Northwest Institute of Eco-Environment and ResourcesChinese Academy of ScienceLanzhou 730000China College of Earth and Environment Science Lanzhou UniversityLanzhou 73000China

Thermokarst lake formation accelerates permafrost degradation due to climate warming,thereby releasing significant amounts of carbon into the atmosphere,complicating hydrological cycles,and causing environmental ***,the energy transfer mechanism from the surface to the sediment of thermokarst lakes remains largely unexplored,thereby limiting our understanding of the magnitude and duration of biogeochemical processes and hydrological ***,herein,a typical thermokarst lake situated in the center of the Qinghai-Tibet Plateau(QTP)was selected for observation and energy budget *** results showed that the net radiation of the thermokarst lake surface was 95.1,156.9,and 32.3 W m^(-2) for the annual,ice-free,and ice-covered periods,respectively,and was approximately 76%of the net radiation consumed by latent heat *** in heat storage in the thermokarst lake initially increased from January to April,then decreased from April to December,with a maximum change of 48.1 W m^(-2) in *** annual average heat fuxes from lake water to sediments were 1.4 W m^(-2);higher heat fluxes occurred during the ice-free season at a range of 4.9-12.0 W m^(-2).The imbalance between heat absorption and release in the millennium scale caused the underlying permafrost of the thermokarst lake to completely *** present,the ground temperature beneath the lake bottom at a depth of 15 m has reached 2.0℃.The temperatures and vapor-pressure conditions of air and lake surfaces control the energy budget of the thermokarst *** findings indicate that changes in the hydrologic regime shifts and biogeochemical processes are more frequent under climate warming and permafrost degradation.

关键词： Qinghai-Tibet Plateau Thermokarst lake Energy budget Permafrost degradation Hydrological cycle