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In-situ study of the hydrogen peroxide photoproduction in seawater on carbon dot-based metal-free catalyst under operation condition

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Nano Research 2024年第7期17卷 5956-5964页

作者： Jiaxuan Wang Jiacheng Li Zenan Li Jie Wu Honglin Si Yangbo Wu Zhiyong Guo Xuepeng Wang Fan Liao Hui Huang Mingwang Shao Yang Liu Zhenhui Kang Institute of Functional Nano and Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Faculty of Electrical Engineering and Computer science Ningbo UniversityNingbo 315211China State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products School of Material Science and Chemical EngineeringNingbo UniversityNingbo 315211China macao Institute of Materials science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyTaipa 999078MacaoChina

Hydrogen peroxide(H_(2)O_(2))photoproduction in seawater with metal-free photocatalysts derived from biomass materials is a green,sustainable,and ultra environmentally friendly ***,most photocatalysts are always corroded or poisoned in seawater,resulting in a significantly reduced catalytic ***,we report the metal-free photocatalysts(RUT-1 to RUT-5)with in-situ generated carbon dots(CDs)from biomass materials(Rutin)by a simple microwave-assisted pyrolysis *** visible light(λ≥420 nm,81.6 mW/cm^(2)),the optimized catalyst of RUT-4 is stable and can achieve a high H_(2)O_(2)yield of 330.36μmol/L in seawater,1.78 times higher than that in normal *** transient potential scanning(TPS)tests are developed and operated to in-situ study the H_(2)O_(2)photoproduction of RUT-4 under operation ***-4 has strong oxygen(O_(2))absorption capacity,and the O_(2)reduction rate in seawater is higher than that in *** cations in seawater further promote the photo-charge separation and facilitate the photo-reduction *** RUT-4,the conduction band level under operating conditions only satisfies the requirement of O_(2)reduction but not for hydrogen(H2)*** work provides new insights for the in-situ study of photocatalyst under operation condition,and gives a green and sustainable path for the H_(2)O_(2)photoproduction with metal-free catalysts in seawater.

关键词： carbon dots hydrogen peroxide photocatalysis transient potential scanning in-situ study operation condition

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动态全场光学相干断层扫描结合深度学习在肿瘤患者术中诊断的应用:一项乳腺癌患者的前瞻性队列研究

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science Bulletin 2024年第11期69卷 1748-1756页

作者：张舒玮杨滨杨后圃赵进张原媛高元绪 Olivia Monteiro 张康刘博王殊 Breast Center Peking University People’s HospitalBeijing 100044China China ESG Institute Capital University of Economics and BusinessBeijing 100070China Faculty of Information technology Beijing University of TechnologyBeijing 100124China Department of Pathology Peking University People’s HospitalBeijing 100044China Center for Biomedicine and Innovations Faculty of MedicineMacao University of Science and TechnologyMacao 999078China College of Future technology Peking UniversityBeijing 100091China School of Mathematical and Computational sciences Massey UniversityAuckland 0745New Zealand

An intraoperative diagnosis is critical for precise cancer surgery. However, traditional intraoperative assessments based on hematoxylin and eosin(H&E) histology, such as frozen section, are time-,resource-, and labor-intensive, and involve specimen-consuming concerns. Here, we report a near-real-time automated cancer diagnosis workflow for breast cancer that combines dynamic full-field optical coherence tomography(D-FFOCT), a label-free optical imaging method, and deep learning for bedside tumor diagnosis during surgery. To classify the benign and malignant breast tissues, we conducted a prospective cohort trial. In the modeling group(n = 182), D-FFOCT images were captured from April 26 to June 20, 2018, encompassing 48 benign lesions, 114 invasive ductal carcinoma(IDC), 10 invasive lobular carcinoma, 4 ductal carcinoma in situ(DCIS), and 6 rare tumors. Deep learning model was built up and fine-tuned in 10,357 D-FFOCT patches. Subsequently, from June 22 to August 17, 2018, independent tests(n = 42) were conducted on 10 benign lesions, 29 IDC, 1 DCIS, and 2 rare tumors. The model yielded excellent performance, with an accuracy of 97.62%, sensitivity of 96.88% and specificity of 100%;only one IDC was misclassified. Meanwhile, the acquisition of the D-FFOCT images was non-destructive and did not require any tissue preparation or staining procedures. In the simulated intraoperative margin evaluation procedure, the time required for our novel workflow(approximately 3 min)was significantly shorter than that required for traditional procedures(approximately 30 min). These findings indicate that the combination of D-FFOCT and deep learning algorithms can streamline intraoperative cancer diagnosis independently of traditional pathology laboratory procedures.

关键词： Cancer diagnosis Breast neoplasms Dynamic full-field optical coherence tomography Deep learning Image classification

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High-performance magnesium/sodium hybrid ion battery based on sodium vanadate oxide for reversible storage of Na^(+)and Mg^(2+)

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Journal of Energy Chemistry 2024年第9期96卷 79-88页

作者： Xiaoke Wang Titi Li Xixi Zhang Yaxin Wang Hongfei Li Hai-Feng Li Gang Zhao Cuiping Han Institute of Applied Physics and Materials Engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078China School of Physics and technology University of JinanJinan 250022ShandongChina Songshan Lake Materials Laboratory Dongguan 523808GuangdongChina Faculty of Materials science and Energy Engineering Shenzhen University of Advanced TechnologyShenzhen 518055GuangdongChina Institute of technology for Carbon Neutrality Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055GuangdongChina

Magnesium ion batteries(MIBs)are a potential field for the energy storage of the future but are restricted by insufficient rate capability and rapid capacity ***-sodium hybrid ion batteries(MSHBs)are an effective way to address these ***,we report a new type of MSHBs that use layered sodium vanadate((Na,Mn)V_(8)O_(20)·5H_(2)O,Mn-NVO)cathodes coupled with an organic 3,4,9,10-perylenetetracarboxylic diimide(PTCDI)anode in Mg^(2+)/Na^(+)hybrid *** electrochemical cycling,Mg^(2+)and Na^(+)co-participate in the cathode reactions,and the introduction of Na^(+)promotes the structural stability of the Mn-NVO cathode,as cleared by several ex-situ ***,the Mn-NVO cathode presents great specific capacity(249.9 mA h g^(−1)at 300 mA g^(−1))and cycling(1500 cycles at 1500 mA g^(−1))in the Mg^(2+)/Na^(+)hybrid ***,full battery displays long lifespan with 10,000 cycles at 1000 mA g^(−1).The rate performance and cycling stability of MSHBs have been improved by an economical and scalable method,and the mechanism for these improvements is discussed.

关键词： Aqueous battery Hybrid ion battery Mg^(2+)/Na^(+)co-intercalation High-rate performance Organic-water hybrid electrolyte

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An Enhanced GAN for Image Generation

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Computers, Materials & Continua 2024年第7期80卷 105-118页

作者： Chunwei Tian Haoyang Gao Pengwei Wang Bob Zhang PAMI Research Group University of MacaoMacao999078China School of Software Northwestern Polytechnical UniversityXi’an710129China Yangtze River Delta Research Institute Northwestern Polytechnical UniversityTaicang215400China Research&development Institute Northwestern Polytechnical UniversityShenzhen518057China

Generative adversarial networks(GANs)with gaming abilities have been widely applied in image ***,gamistic generators and discriminators may reduce the robustness of the obtained GANs in image generation under varying *** the relation of hierarchical information in a generation network and enlarging differences of different network architectures can facilitate more structural information to improve the generation effect for image *** this paper,we propose an enhanced GAN via improving a generator for image generation(EIGGAN).EIGGAN applies a spatial attention to a generator to extract salient information to enhance the truthfulness of the generated *** into relation the context account,parallel residual operations are fused into a generation network to extract more structural information from the different ***,a mixed loss function in a GAN is exploited to make a tradeoff between speed and accuracy to generate more realistic *** results show that the proposed method is superior to popular methods,i.e.,Wasserstein GAN with gradient penalty(WGAN-GP)in terms of many indexes,i.e.,Frechet Inception Distance,Learned Perceptual Image Patch Similarity,Multi-Scale Structural Similarity Index Measure,Kernel Inception Distance,Number of Statistically-Different Bins,Inception Score and some visual images for image generation.

关键词： Generative adversarial networks spatial attention mixed loss image generation

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Sulfonated carbon dots modified IrO_(2)nanosheet as durable and high-efficient electrocatalyst for boosting acidic oxygen evolution reaction

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Nano Research 2024年第9期17卷 8017-8024页

作者： Mengjie Ma Wenxiang Zhu Fan Liao Kui Yin Hui Huang Kun Feng Dongdong Gao Jinxin Chen Zenan Li Jun Zhong Lai Xu Yang Liu Mingwang Shao Zhenhui Kang Institute of Functional Nano and Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-based Functional Materials and DevicesSoochow UniversitySuzhou 215123China macao Institute of Materials science and Engineering(MIMSE) Macao University of Science and TechnologyTaipaMacao 999078China

Oxygen evolution reaction(OER)plays a crucial role in developing energy conversion and adjusting electronic structure of the electrocatalysts can effectively improve the catalytic activity and ***,it is a challenge to adjust the electronic structure on two-dimensional iridium dioxide nanosheets(IrO_(2)NS),which have the advantages of high atom ***,we regulate the surface properties of IrO_(2)NS through sulfonated carbon dots(SCDs)to promote the OER catalytic *** catalyst IrO_(2)NS/SCDs-2 exhibited excellent catalytic activity with a lower overpotential of 180 mV than IrO_(2)NS(230 mV)at the current density of 10 mA·cm^(-2)in a 0.5 M H_(2)SO_(4) *** after 160 h of stability testing,the overpotential of IrO_(2)NS/SCDs-2 only decreased by 4 ***,transient potential scanning test can visually demonstrate that the addition of SCDs improves the conductivity of the catalyst and increases the electron transfer rate.

关键词： sulfonated carbon dots oxygen evolution reaction electrocatalysis transient potential scanning

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Medium-energy electron spectrometers on macao science Satellite-1

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science China Technological sciences 2024年第11期67卷 3324-3343页

作者： YE YuGuang LIU Ying ZOU Hong ZONG QiuGang CHEN JiaLi YU XiangQian SHI WeiHong OU JiaMing LIU JianBin YU LiJia ZHOU Jun HUANG He YUAN ShiGeng SU Wen SUO Le State Key Laboratory of Lunar and Planetary sciences Macau University of Science and TechnologyCNSA Macao Center for Space Exploration and Science School of Earth and Space sciences Peking University Shandong Aerospace Electro-technology School of Astronautics Northwestern Polytechnical University DFH Satellite Co.Ltd. Institute of Remote Sensing Satellite China Academy of Space Technology

The macao science Satellite-1 is a two-satellite constellation specifically designed to study the geomagnetic field and particle radiation environment in low Earth orbit, particularly in the South Atlantic Anomaly region, with a low inclination orbit. Each of the two MSS-1 satellites carries a medium-energy electron spectrometer(MES). The MES sensor heads are based on pinhole imaging technology, which can simultaneously measure 50-600 keV electrons incident from nine directions with a field of view(FOV) of 180° × 30°. The two MESs can realize the pitch angle coverage of medium energy electrons at most positions in the orbit. The MSS-1 A/B MESs can realize direct observation of precipitating electrons and electrons near their loss cones. It can help to study the electron generation mechanism in the inner radiation belt and quantify the precipitation of magnetospheric energetic electrons. Combined with the geomagnetic index, solar wind parameters, interplanetary magnetic field conditions, etc.,it can also help to build a dynamic evolution model of energetic electrons in the near-Earth space, to realize the early warning and prediction of space weather based on the observation data, which can provide safety for spacecraft and astronauts in the nearEarth space.

关键词： macao science Satellite-1 medium-energy electron spectrometer inner radiation electrons Southern Atlantic Anomaly pitch angle distribution

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Integrated Clustering and Routing Design and Triangle Path Optimization for UAV-Assisted Wireless Sensor Networks

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China Communications 2024年第4期21卷 178-192页

作者： Shao Liwei Qian Liping Wu Mengru Wu Yuan College of Information Engineering Zhejiang University of TechnologyHangzhou 310014China State Key Laboratory of Internet of Things for Smart City University of MacaoMacaoChina Department of Computer and Information science University of MacaoMacaoChina

With the development of the Internet of Things(IoT),it requires better performance from wireless sensor networks(WSNs),such as larger coverage,longer lifetime,and lower ***,a large amount of data generated from monitoring and long-distance transmission places a heavy burden on sensor nodes with the limited battery *** this,we investigate an unmanned aerial vehicles assisted mobile wireless sensor network(UAV-assisted WSN)to prolong the network lifetime in this ***,we use UAVs to assist the WSN in collecting *** the current UAV-assisted WSN,the clustering and routing schemes are determined ***,such a separate consideration might not maximize the lifetime of the whole WSN due to the mutual coupling of clustering and *** efficiently prolong the lifetime of the WSN,we propose an integrated clustering and routing scheme that jointly optimizes the clustering and routing *** the whole network space,it is intractable to efficiently obtain the optimal integrated clustering and routing ***,we propose the Monte-Las search strategy based on Monte Carlo and Las Vegas ideas,which can generate the chain matrix to guide the algorithm to find the solution *** point-to-point collection leads to long collection paths,so a triangle optimization strategy is then proposed that finds a compromise path to shorten the collection path based on the geometric distribution and energy of sensor *** avoid the coverage hole caused by the death of sensor nodes,the deployment of mobile sensor nodes and the preventive mechanism design are *** emergency data transmission mechanism is further proposed to reduce the latency of collecting the latency-sensitive data due to the absence of *** with the existing schemes,the proposed scheme can prolong the lifetime of the UAVassisted WSN at least by 360%,and shorten the collection path of UAVs by 56.24%.

关键词： Monte-Las search strategy triangle path optimization unmanned aerial vehicles wireless sensor networks

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THE SPARSE REPRESENTATION RELATED WITH FRACTIONAL HEAT EQUATIONS

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Acta Mathematica Scientia 2024年第2期44卷 567-582页

作者：曲伟钱涛梁应德李澎涛 College of sciences China Jiliang UniversityHangzhou310018China macao Center for Mathematical science Macao University of Science and TechnologyMacao999078China Department of Mathematics Faculty of Science and TechnologyUniversity of MacaoMacao999078China School of Mathematics and Statistics Qingdao UniversityQingdao266071China

This study introduces a pre-orthogonal adaptive Fourier decomposition(POAFD)to obtain approximations and numerical solutions to the fractional Laplacian initial value problem and the extension problem of Caffarelli and Silvestre(generalized Poisson equation).As a first step,the method expands the initial data function into a sparse series of the fundamental solutions with fast convergence,and,as a second step,makes use of the semigroup or the reproducing kernel property of each of the expanding *** show the effectiveness and efficiency of the proposed series solutions.

关键词： reproducing kernel Hilbert space dictionary sparse representation approximation to the identity fractional heat equations

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Genome engineering of the human gut microbiome

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Journal of Genetics and Genomics 2024年第5期51卷 479-491页

作者： Linggang Zheng Juntao Shen Ruiyue Chen Yucan Hu Wei Zhao Elaine Lai-Han Leung Lei Dai Dr Neher's Biophysics Laboratory for Innovative Drug Discovery/State Key Laboratory of Quality Research in Chinese Medicine Macao University of Science and TechnologyTaipaMacao 999078China CAS Key Laboratory of Quantitative Engineering Biology Shenzhen Institute of Synthetic BiologyShenzhen Institutes of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China University of Chinese Academy of sciences Beijing 100049China Cancer Center Faculty of Health ScienceUniversity of MacaoMacao 999078China MOE Frontiers science Center for Precision Oncology University of MacaoMacao 999078China

The human gut microbiome,a complex ecosystem,significantly influences host health,impacting crucial aspects such as metabolism and *** enhance our comprehension and control of the molecular mechanisms orchestrating the intricate interplay between gut commensal bacteria and human health,the exploration of genome engineering for gut microbes is a promising ***,the complexities and diversities inherent in the gut microbiome pose substantial challenges to the development of effective genome engineering tools for human gut *** this comprehensive review,we provide an overview of the current progress and challenges in genome engineering of human gut commensal bacteria,whether executed in vitro or in situ.A specific focus is directed towards the advancements and prospects in cargo DNA delivery and high-throughput ***,we elucidate the immense potential of genome engineering methods to enhance our understanding of the human gut microbiome and engineer the microorganisms to enhance human health.

关键词： Non-model gut commensals Genomeediting reagents Cargo delivery High-throughput genome engineering

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Transcriptomic and Macroscopic Architectures of Multimodal Covariance Network Reveal Molecular–Structural–Functional Co-alterations

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Research 2024年第1期2023卷 471-487页

作者： Lin Jiang Yueheng Peng Runyang He Qingqing Yang Chanlin Yi Yuqin Li Bin Zhu Yajing Si Tao Zhang Bharat B.Biswal Dezhong Yao Lan Xiong Fali Li Peng Xu The Clinical Hospital of Chengdu Brain science Institute MOE Key Lab for NeuroinformationUniversity of Electronic Science and Technology of ChinaChengdu 611731China School of Life science and technology Center for Information in BioMedicineUniversity of Electronic Science and Technology of ChinaChengdu 611731China School of Psychology Xinxiang Medical UniversityXinxiang 453003China School of science Xihua UniversityChengdu 610039China Department of Biomedical Engineering New Jersey Institute of TechnologyNewarkNJUSA School of Electrical Engineering Zhengzhou UniversityZhengzhou 450001China Research Unit of NeuroInformation Chinese Academy of Medical Sciences2019RU035ChengduChina Montreal Neurological Institute and Hospital McGill UniversityMontrealQCCanada Department of Electrical and Computer Engineering Faculty of Science and TechnologyUniversity of MacaoMacaoChina Radiation Oncology Key Laboratory of Sichuan Province 610041 ChengduChina Rehabilitation Center Qilu Hospital of Shandong UniversityJinan 250012China

Human cognition is usually underpinned by intrinsic structure and functional neural co-activation in spatially distributed brain *** to lacking an effective approach to quantifying the covarying of structure and functional responses,how the structural–functional circuits interact and how genes encode the relationships,to deepen our knowledge of human cognition and disease,are still ***,we propose a multimodal covariance network(MCN)construction approach to capture interregional covarying of the structural skeleton and transient functional activities for a single *** further explored the potential association between brain-wide gene expression patterns and structural–functional covarying in individuals involved in a gambling task and individuals with major depression disorder(MDD),adopting multimodal data from a publicly available human brain transcriptomic atlas and 2 independent *** analysis showed a replicable cortical structural–functional fine map in healthy individuals,and the expression of cognition-and disease phenotype-related genes was found to be spatially correlated with the corresponding MCN *** analysis of cell type-specific signature genes suggests that the excitatory and inhibitory neuron transcriptomic changes could account for most of the observed correlation with task-evoked MCN differences.

关键词： alterations evoked spatially

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