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study on preparation,characterization and application of mixed-colorants thermochromic microcapsules

Particuology 2024年第5期88卷 89-97页

作者： Lan Zhou Jingpeng Ye Qinze Cai Guojin Liu Mehran Dadgar Guocheng Zhu Guoqing Zhang College of textile science and Engineering (international Institute of silk) Zhejiang Sci-Tech UniversityHangzhou310018China school of Materials science& Engineering Zhejiang Sci-Tech UniversityHangzhou310018China Department of textile University of NeyshaburAdib BoulevardKhorasan Razavi ProvinceIran Zhejiang Charming Dyeing and Finishing Co. LtdJiaxing314500China Zhejiang Provincial innovation Center of Advanced textile technology Shaoxing312000China

In order to expand the color-change range and make the discoloration temperature suitable for the daily textiles,a new formulation of mixed-colorants thermochromic core material is designed,in which crystal violet lactone(CVL)is the basic color former,bisphenol A(BPA)is the developer,especially the solvent-based dye and dodecyl dedecanoate are used as the extended dye and the solvent,*** electron microscope(sEM),differential scanning calorimeter(DsC)and thermogravimetric analyzer(tGA)were applied to study the morphology,encapsulation rate,non-isothermal crystallization behavior and thermal stability of the mixed-colorant thermochromic microcapsules(MCtMs)prepared by in-situ *** results show that MCtMs have good sphericity,uniform particle size,good thermal stability and the encapsulation rate can reach 86.73%.Under the non-isothermal conditions,the encapsulation of formaldehyde-melamine resin wall material can slightly reduce the crystallization rate of the solvent,but does not affect the relative crystallinity,thermal properties and discoloration sensitivity of the core *** the variety of ambient temperatures in the range of 20–35℃,the printed cotton fabrics with MCtMs could change color reversibly between different tones with good reliability and durability,and exhibit more gorgeous colors than the common thermochromic materials.

关键词： thermochromic microcapsule Color-change range Phase-change material Crystallization behavior

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structure engineering of cathode host materials for Li-s batteries

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Rare Metals 2024年第4期43卷 1370-1389页

作者： Jia-Jun Long Hua Yu Wen-Bo Liu school of New Energy and Materials Southwest Petroleum UniversityChengdu610500China school of Mechanical Engineering Sichuan UniversityChengdu610065China

Although lithium-sulfur batteries are one of the favorable candidates for next-generation energy storage devices,a few key challenges that have not been addressed have limited its *** challenges include lithium dendrite growth in the anode side,volume change of the active material,poor electrical conductivity,dissolution and migration of poly sulfides,and slow rate of solid-state reactions in the cathode *** the electrochemical performance of lithium-sulfur batteries is greatly affected by the design of the cathode host material,it has also been widely discussed in addressing the abovementioned *** this paper,three design ideas of cathode host materials in terms of microstructure,crystal structure and electronic structure are introduced and ***,the current progress of these three structural design strategies and their effects on the electrochemical performance of lithium-sulfur batteries are discussed in ***,future directions in the structural design of cathode materials for lithium-sulfur batteries are discussed and further perspectives are provided.

关键词： Lithium-sulfur batteries structure engineering Cathode Host materials

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Modeling of ion cyclotron resonance frequency heating of proton-boron plasmas in EHL-2 spherical tokamak

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Plasma science and technology 2024年第10期26卷 39-48页

作者： Xianshu WU Jingchun LI Jiaqi DONG Yuejiang sHI Guoqing LIU Yong LIU Zhiqiang LONG Buqing ZHANG Baoshan YUAN Y.K.Martin PENG Minsheng LIU shenzhen key Laboratory of Nuclear and Radiation safety Institute for Advanced Study in Nuclear Energy&SafetyCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen 510640People’s Republic of China Department of Earth and space sciences Southern University of Science and TechnologyShenzhen 518055People’s Republic of China ENN science and technology Development Co. Ltd.and Hebei Key Laboratory of Compact FusionLangfang 065001People’s Republic of China siemens shenzhen Magnetic Resonance Ltd. Shenzhen 518057People’s Republic of China

Ion cyclotron resonance heating(ICRH)stands out as a widely utilized and cost-effective auxiliary method for plasma heating,bearing significant importance in achieving high-performance discharges in p-^(11)B *** light of the specific context of p-^(11)B plasma in the EHL-2 device,we conducted a comprehensive scan of the fundamental physical parameters of the antenna using the full-wave simulation program *** preliminary result indicated that for p-^(11)B plasma,optimal ion heating parameters include a frequency of 40 MHz,with a high toroidal mode number like N_(?)=28 to heat the majority H *** addition,we discussed the impact of concentration of minority ion species on ion cyclotron resonance heating when^(11)B serves as the heavy minority *** significant difference in charge-to-mass ratio between boron and hydrogen ions results in a considerable distance between the hybrid resonance layer and the tow inverted cyclotron resonance layer,necessitating a quite low boron ion concentration to achieve effective minority *** also considered another method of direct heating of hydrogen ions in the presence of boron ion *** is found that at appropriate boron ion concentrations(X(^(11)B)~17%),the position of the hybrid resonance layer approaches that of the hydrogen ion cyclotron resonance layer,thereby altering the polarization at this position and significantly enhancing hydrogen ion fundamental absorption.

关键词： ICRF hydrogen-boron fusion mode conversion fundamental absorption

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Cascading Failures in Power Grids: A Load Capacity Model with Node Centrality

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Complex system Modeling and simulation 2024年第1期4卷 1-14页

作者： Chaoyang Chen Yao Hu Xiangyi Meng Jinzhu Yu Department of Information and Electrical Engineering Hunan University of Science and TechnologyXiangtan 411100China Department of Physics and Astronomy Northwestern UniversityEvanstonIL 60208USA Department of Civil Engineering University of TexasArlingtonTX 22201USA

Power grids,due to their lack of network redundancy and structural interdependence,are particularly vulnerable to cascading failures,a phenomenon where a few failed nodes—having their loads exceeding their capacities—can trigger a widespread collapse of all ***,we extend the cascading failure(Motter-Lai)model to a more realistic perspective,where each node’s load capacity is determined to be nonlinearly correlated with the node’s *** analysis encompasses a range of synthetic networks featuring small-world or scale-free properties,as well as real-world network configurations like the IEEE bus systems and the Us power *** find that fine-tuning this nonlinear relationship can significantly enhance a network’s robustness against cascading failures when the network nodes are under ***,the selection of initial nodes and the attack strategies also impact overall network *** findings offer valuable insights for improving the safety and resilience of power grids,bringing us closer to understanding cascading failures in a more realistic context.

关键词： load capacity complex network node centrality cascading failures robustness of power grids

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Composite structure Al_(2)O_(3)/Al_(2)O_(3)-YAG:Ce/YAG ceramics with high color spatial uniformity for white laser lighting

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Journal of Advanced Ceramics 2024年第2期13卷 189-197页

作者： Pengfei sang Le Zhang Jian Kang Mingzhou Li shiwei Chen Peng Yang Bingheng sun Yang Li Wieslaw strek Hao Chen Jiangsu key Laboratory of Advanced Laser Materials and Devices School of Physics and Electronics EngineeringJiangsu Normal UniversityXuzhou 221116China Jiangsu Xiyi Advanced Materials Research Institute of Industrial technology Xuzhou 221400China Xuzhou EAGLED technology Co. Ltd.Xuzhou 221116China Xuzhou Kangna Advanced Materials technology Co. Ltd.Xuzhou 221116China Xuzhou Fuchang Electronic technology Co. Ltd.Xuzhou 221116China shanghai Institute of Optics Fine Mechanics Chinese Academy of SciencesShanghai 201800China school of Material science and Engineering Shanghai Institute of TechnologyShanghai 201418China state key Laboratory of Crystal Materials Shandong UniversityJinan 250100China Institute of Low temperature and structure Research Polish Academy of SciencesWroclaw 50-422Poland

Composite ceramic phosphor(CCP)is a candidate light-conversion material to obtain the high-quality laser lighting *** based on the transmissive configuration model could not simultaneously meet the requirements of angular color uniformity and high thermal *** this study,a novel composite structure ceramic was designed,including Al_(2)O_(3)-YAG:Ce/YAG layered ceramic with a size of 1 mm×1 mm for lighting,and Al_(2)O_(3) ceramic(φ=16.0 mm)was used as the wrapping material due to its outstanding thermal *** prepared ceramics exhibited excellent thermal performance and no yellow ring *** this design,we achieved the match of the intensity distribution of the blue and yellow lights,resulting in a high angular color uniformity of 0.9 with a view angle of±80°.All ceramics showed no luminous saturation phenomenon,even the laser power density was increased up to 47.51 W/mm^(2).A high-brightness white-light source with a luminous flux of 618 lm,a luminous efficiency of 126 lm/W,a CCt of 6615 K,and a CRI of 69.9 was obtained in the transmissive *** particular,the surface temperature of the ceramic was as low as 74.1℃ under a high laser radiation(47.51 W/mm^(2)).these results indicate that Al_(2)O_(3)/Al_(2)O_(3)-YAG:Ce/YAG composite structure ceramic is a promising luminescent material in the high-power laser lighting applications.

关键词： Al_(2)O_(3)/Al_(2)O_(3)-YAG:Ce/YAG angular color uniformity high thermal stability high-power laser lighting

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High recorded color rendering performance of single-structured Ce,Mn:Y_(3)(Al,sc)_(2)Al_(3)O_(12)phosphor ceramics for high-power white LEDs/LDs

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Journal of Advanced Ceramics 2024年第6期13卷 810-820页

作者： Xuanchu Liu Congcong Yang Yanbin Li Chang Min Jian Kang tianyuan Zhou Chunming Zhou Chaofan shi Cen shao Bingheng sun Wieslaw strek Hao Chen Le Zhang Jiangsu key Laboratory of Advanced Laser Materials and Devices School of Physics and Electronics EngineeringJiangsu Normal UniversityXuzhou 221116China Jiangsu Xiyi Advanced Materials Research Institute of Industrial technology Xuzhou 221400China Xuzhou EAGLED technology Co. Ltd.Xuzhou 221116China Xuzhou Kangna Advanced Materials technology Co. Ltd.Xuzhou 221116China shanghai Institute of Optics Fine Mechanics Chinese Academy of SciencesShanghai 201800China Institute of Low temperature and structure Research Polish Academy of SciencesWroclaw 50-422Poland state key Laboratory of Crystal Materials Shandong UniversityJinan 250100China

Achieving a high color rendering index(CRI)and luminous stability in single-structured Ce:Y_(3)Al_(5)O_(12)(Ce:YAG)phosphor ceramics(PCs)is crucial for high-power white light-emitting diodes or laser diodes(LEDs/LDs).However,cyan valleys and insufficient amounts of the red component in the Ce:YAG emission spectra significantly limit their real *** this work,a series of Ce,Mn:Y_(3)(Al,sc)_(2)Al_(3)O_(12)(Ce,Mn:YsAG)PCs were fabricated by vacuum sintering,and efficient spectral regulation was realized for full-color *** cyan valley was filled by the blueshifted emission peak of Ce^(3+)via sc^(3+)*** orange‒red emission at approximately 580 nm was effectively supplemented via Mn^(2+)*** particular,CRI of Ce,Mn:YsAG increased from 56.4 to 85.8,a 52%increase compared with that of Ce:YAG under high-power LED excitation,and the operating temperature was stable at approximately 50℃for long working ***,CRI of 80.9 could still be obtained for PC-based white *** results indicated that Ce,Mn:YsAG PC,which has excellent CRI and luminous stability,is an extremely promising color convertor for high-power white LEDs/LDs.

关键词： color rendering index(CRI) color converter Ce:Y_(3)Al_(5)O_(12)(Ce:YAG)phosphor ceramics(PCs) high-power white light-emitting diodes or laser diodes(LEDs/LDs) luminous stability

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CEPC technical Design Report

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Radiation Detection technology and Methods 2024年第1期8卷 I0003-I0016,1-1091页

作者： Waleed Abdallah tiago Carlos Adorno de Freitas Konstantin Afanaciev shakeel Ahmad Ijaz Ahmed Xiaocong Ai Abid Aleem Wolfgang Altmannshofer Fabio Alves Weiming An Rui An Daniele Paolo Anderle stefan Antusch Yasuo Arai Andrej Arbuzov Abdesslam Arhrib Mustafa Ashry sha Bai Yu Bai Yang Bai Vipul Bairathi Csaba Balazs Philip Bambade Yong Ban tripamo Bandyopadhyay shou-shan Bao Desmond P.Barber Ayse Bat Varvara Batozskaya subash Chandra Behera Alexander Belyaev Michele Bertucci Xiao-Jun Bi Yuanjie Bi tianjian Bian Fabrizio Bianchi thomas Biekotter Michela Biglietti shalva Bilanishvili Deng Binglin Denis Bodrov Anton Bogomyagkov serge Bondarenko stewart Boogert Maarten Boonekamp Marcello Borri Angelo Bosotti Vincent Boudry Mohammed Boukidi Igor Boyko Ivanka Bozovic Giuseppe Bozzi Jean-Claude Brient Anastasiia Budzinskaya Masroor Bukhari Vladimir Bytev Giacomo Cacciapaglia Hua Cai Wenyong Cai Wujun Cai Yijian Cai Yizhou Cai Yuchen Cai Haiying Cai Huacheng Cai Lorenzo Calibbi Junsong Cang Guofu Cao Jianshe Cao Antoine Chance Xuejun Chang Yue Chang Zhe Chang Xinyuan Chang Wei Chao Auttakit Chatrabhuti Yimin Che Yuzhi Che Bin Chen Danping Chen Fuqing Chen Fusan Chen Gang Chen Guoming Chen Hua-Xing Chen Huirun Chen Jinhui Chen Ji-Yuan Chen Kai Chen Mali Chen Mingjun Chen Mingshui Chen Ning Chen shanhong Chen shanzhen Chen shao-Long Chen shaomin Chen shiqiang Chen tianlu Chen Wei Chen Xiang Chen Xiaoyu Chen Xin Chen Xun Chen Xurong Chen Ye Chen Ying Chen Yukai Chen Zelin Chen Zilin Chen Gang Chen Boping Chen Chunhui Chen Hok Chuen Cheng Huajie Cheng shan Cheng tongguang Cheng Yunlong Chi Pietro Chimenti Wen Han Chiu Guk Cho Ming-Chung Chu Xiaotong Chu Ziliang Chu Guglielmo Coloretti Andreas Crivellin Hanhua Cui Xiaohao Cui Zhaoyuan Cui Brunella D'Anzi Ling-Yun Dai Xinchen Dai Xuwen Dai Antonio De Maria Nicola De Filippis Christophe De La taille Francesca De Mori Chiara De sio Elisa Del Core shuangxue Deng Wei-tian Deng Zhi Deng Ziyan Deng Bhupal Dev tang Dewen Biagio Di Micco Ran Ding siqin Dingl Yadong Ding Haiyi Dong Jianin AGH University of science and technology Faculty of Physics and Applied Computer ScienceKrakow Anhui University HefeiAnhui Applied Physics Department Federal Urdu University of ArtsScience and TechnologyIslamabad Banaras Hindu University Institute of ScienceVaranasi Bandirma Onyedi Eylul University Bandirma Beihang University Beijing Beijing Computational science Research Center Beijing Beijing Conveyi LtD Beijing Beijing Glass Research Institute Co. LtdBeijing Beijing Institute of technology Beijing Beijing Normal University Beijing Brown University ProvidenceRI Budker Institute of Nuclear Physics Novosibirsk Cadi Ayyad University Laboratory of Fundamental and Applied PhysicsPolydisciplinary FacultyMarrakech Cairo University Giza Center for theory and Computation National Tsing Hua UniversityHsinchu Central China Normal University WuhanHubei Central south University ChangshaHunan Centro de Fisica teorica de Particulas Universidade Tecnica de LisboaLisboa Chengdu Kaitengsifang Digital Radio&tV Equipment Co. LtdChengduSichuan China academy of engineering physics MianyangSichuan China building materials academy Beijing China Center of Advanced science and technology Beijing China Institute of Atomic Energy Beijing China Jiliang University HangzhouZhejiang China Nuclear Instrument CO. LTDBeijing China University of Geosciences Beijing China University of Geosciences WuhanHubei China University of Mining and technology XuzhouJiangsu China West Normal University NanchongSichuan Chongqing University Department of PhysicsChongqing Chulalongkorn University Bangkok City University of Hong Kong Department of PhysicsHong Kong Cockcroft Institute Daresbury Cornell University IthacaNY CPPM(AMU/IPhU&CNRs/INP) Marseille Dalian Minzu University DalianLiaoning Dalian University of technology Department of PhysicsDalian Deutsches Elektronen-synchrotron DEsY Hamburg Dzhelepov Laboratory of Nuclear Problems of Joint Institute for Nuclear Research(DLNP JINR) Dubna East China University Of science And technol

the Circular Electron Positron Collider(CEPC)is a large scientific project initiated and hosted by China,fostered through extensive collaboration with international *** complex comprises four accelerators:a 30 GeV Linac,a 1.1 GeV Damping Ring,a Booster capable of achieving energies up to 180 GeV,and a Collider operating at varying energy modes(Z,W,H,and tt).the Linac and Damping Ring are situated on the surface,while the subterranean Booster and Collider are housed in a 100 km circumference underground tunnel,strategically accommodating future expansion with provisions for a potential super Proton Proton Collider(sPPC).the CEPC primarily serves as a Higgs *** its baseline design with synchrotron radiation(sR)power of 30 MW per beam,it can achieve a luminosity of 5×10^(34)cm^(-2)s^(-1)per interaction point(IP),resulting in an integrated luminosity of 13 ab^(-1)for two IPs over a decade,producing 2.6 million Higgs *** the sR power to 50 MW per beam expands the CEPC's capability to generate 4.3 million Higgs bosons,facilitating precise measurements of Higgs coupling at sub-percent levels,exceeding the precision expected from the HL-LHC by an order of *** technical Design Report(tDR)follows the Preliminary Conceptual Design Report(Pre-CDR,2015)and the Conceptual Design Report(CDR,2018),comprehensively detailing the machine's layout,performance metrics,physical design and analysis,technical systems design,R&D and prototyping efforts,and associated civil engineering ***,it includes a cost estimate and a preliminary construction timeline,establishing a framework for forthcoming engineering design phase and site selection *** is anticipated to begin around 2027-2028,pending government approval,with an estimated duration of 8 *** commencement of experiments and data collection could potentially be initiated in the mid-2030s.

关键词： initiated exceeding precise

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金属离子和油酰肌氨酸钠对锂云母和长石浮选分离的协同作用机理(英文)

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transactions of Nonferrous Metals society of China 2024年

作者：向国源范瑞华朱文韬孙伟郑仁基高志勇中南大学资源加工与生物工程学院中南大学金属资源开发利用碳减排教育部工程研究中心中南大学战略含钙矿物资源清洁高效利用湖南省重点实验室中南大学湖南省关键金属矿产资源高效清洁利用国际联合研究中心

铝硅酸盐矿物锂云母和长石的高效分离一直是个难题。本研究首次将油酰肌氨酸钠与不同金属离子（钙、镁、铜和铅）结合，用来提高这两种矿物的浮选分离效率。通过接触角测量、原子力显微镜、傅立叶变换红外光谱、物种分布计算和密度函数... 详细信息

铝硅酸盐矿物锂云母和长石的高效分离一直是个难题。本研究首次将油酰肌氨酸钠与不同金属离子（钙、镁、铜和铅）结合，用来提高这两种矿物的浮选分离效率。通过接触角测量、原子力显微镜、傅立叶变换红外光谱、物种分布计算和密度函数理论计算研究其协同作用机理。结果表明，钙离子对活化锂云母的选择性最大，其次是镁、铜和铅离子。此外，油酰肌氨酸钠能在钙离子活化的锂云母表面形成多层和强烈的化学吸附，吸附能高达-1248.91 kJ/mol。相比之下，油酰肌氨酸钠在钙离子活化的长石上的吸附作用则不明显，吸附能低至-598.84 kJ/mol。因此，油酰肌氨酸钠和钙离子兼具强捕收能力和高选择性，它们的组合使用为全面和高效地回收锂资源提供新策略。

关键词：浮选锂云母长石油酰肌氨酸钠金属离子

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sulfone-functionalized stable molecular single crystals for photocatalytic hydrogen evolution

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susMat 2024年第3期4卷 240-250页

作者： Xunliang Hu Xiaoju Yang Bingyi song Zhen Zhan Ruixue sun Yantong Guo Li-Ming Yang Xuan Yang Chun Zhang Irshad Hussain Xiaoyan Wang Bien tan key Laboratory of Material Chemistry for Energy Conversion and storage Ministry of Education Hubei Key Laboratory of Material Chemistry and Service FailureSchool of Chemistry and Chemical EngineeringHuazhong University of Science and TechnologyWuhanChina Department of Applied Physics The Hong Kong Polytechnic UniversityKowloonHong KongChina College of Life science&technology Huazhong University of Science and TechnologyWuhanChina Department of Chemistry and Chemical Engineering SBA School of Science and EngineeringLahore University of Management SciencesLahorePakistan

Highly crystalline organic semiconductors are ideal materials for photocatalytic hydrogen evolution in water ***,the instability and complex synthesis processes of most reported organic molecule-based photocatalysts restrict their *** this study,we introduce benzo[1,2-b:4,5-bʹ]bis[1]benzothiophene-3,9-dicarboxylic acid,5,5,11,11-tetraoxide(FsOCA),a highly crystalline,stable molecular crystal that is easy to synthesize and serves as an efficient photocatalyst for the hydrogen evolution *** exhibits high efficiency in sacrificial hydrogen evolution reaction(760μmol h^(−1),76 mmol g^(−1)h^(−1)at 330 mW cm^(−2);570μmol h^(−1),57 mmol g^(−1)h^(−1)at 250 mW cm^(−2)),and FsOCA remains stable during photocatalysis for up to 400 *** and theoretical studies confirmed the presence of hydrogen bonds between the sulfone group and the sacrificial agent(ascorbic acid).this interaction significantly improved the oxidation reaction kinetics and boosted the photocatalytic *** study presents a scalable and convenient approach to synthesize highly crystalline,active,and stable organic photocatalysts with potential applications in large-scale photocatalysis.

关键词： exceptional durability molecular single crystals photocatalytic water splitting

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Roadmap for rechargeable batteries:present and beyond

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science China Chemistry 2024年第1期67卷 13-42页

作者： sen Xin Xu Zhang Lin Wang Haijun Yu Xin Chang Yu-Ming Zhao Qinghai Meng Pan Xu Chen-Zi Zhao Jiahang Chen Huichao Lu Xirui Kong Jiulin Wang Kai Chen Gang Huang Xinbo Zhang Yu su Yao Xiao shu-Lei Chou shilin Zhang Zaiping Guo Aobing Du Guanglei Cui Gaojing Yang Qing Zhao Liubing Dong Dong Zhou Feiyu Kang Hu Hong Chunyi Zhi Zhizhang Yuan Xianfeng Li Yifei Mo Yizhou Zhu Dongfang Yu Xincheng Lei Jianxiong Zhao Jiayi Wang Dong su Yu-Guo Guo Qiang Zhang Jun Chen Li-Jun Wan CAs key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of sciences.Beijing 100049 China Institute of Advanced Battery Materials and Devices Faculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China key Laboratory of Advanced Functional Materials Ministry of EducationBeijing University of TechnologyBeijing 100124China Beijing key Laboratory of Green Chemical Reaction Engineering and technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China state key Laboratory of Chemistry and Utilization of Carbon-Based Energy Resources College of ChemistryXinjiang UniversityUrumqi 830046China Department of Chemical Engineering Shanghai Jiao Tong UniversityShanghai 200240China state key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied ChemistryChangchun 130022China Institute for Carbon Neutralization College of Chemistry and Materials EngineeringWenzhou UniversityWenzhou 325035China school of Chemical Engineering and Advanced Materials The University of AdelaideAdelaide 5000Australia Qingdao Industrial Energy storage Research Institute Qingdao Institute of Bioenergy and Bioprocess TechnologyChinese Academy of SciencesQingdao 266101China Frontiers science Center for New Organic Matter Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China College of Chemistry and Materials science Jinan UniversityGuangzhou 511443China tsinghua shenzhen international Graduate school Tsinghua UniversityShenzhen 518055China Department of Materials science and Engineering City University of Hong KongHong Kong 999077China Division of Energy storage Dalian National Laboratory for Clean Energy(DNL)Dalian Institute of Chem

Rechargeable batteries currently hold the largest share of the electrochemical energy storage market,and they play a major role in the sustainable energy transition and industrial decarbonization to respond to global climate *** to the increased popularity of consumer electronics and electric vehicles,lithium-ion batteries have quickly become the most successful rechargeable batteries in the past three decades,yet growing demands in diversified application scenarios call for new types of rechargeable *** efforts are made to developing the next-generation post-Li-ion rechargeable batteries,which include,but are not limited to solid-state batteries,lithium–sulfur batteries,sodium-/potassium-ion batteries,organic batteries,magnesium-/zinc-ion batteries,aqueous batteries and flow *** the great achievements,challenges persist in precise understandings about the electrochemical reaction and charge transfer process,and optimal design of key materials and interfaces in a *** roadmap tends to provide an overview about the current research progress,key challenges and future prospects of various types of rechargeable *** computational methods for materials development,and characterization techniques will also be discussed as they play an important role in battery research.

关键词： energy storage rechargeable batteries battery materials electrochemistry

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