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An Unprecedented Efficiency with Approaching 21%Enabled by Additive‑Assisted Layer‑by‑Layer Processing in Organic Solar Cells

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Nano-Micro Letters 2025年第2期17卷 372-375页

作者： Shuai Xu Youdi Zhang Yanna Sun Pei Cheng Zhaoyang Yao Ning Li Long Ye Lijian Zuo Ke Gao Key Laboratory of Advanced Green Functional Materials College of ChemistryChangchun Normal UniversityChangchun 130032People’s Republic of China Shandong Provincial Key Laboratory for Science of Material Creation and Energy Conversion School of Chemistry and Chemical EngineeringShandong UniversityQingdao 266237People’s Republic of China College of Polymer Science and Engineering Sichuan UniversityChengdu 610065People’s Republic of China State Key Laboratory and Institute of Elemento‑Organic Chemistry Centre of Nanoscale Science and Technology and Key Laboratory of Functional Polymer MaterialsRenewable Energy Conversion and Storage Center(RECAST)College of ChemistryNankai UniversityTianjin 300071People’s Republic of China Institute of Polymer Optoelectronic Materials and Devices State Key Laboratory of Luminescent Materials and Devices South China University of TechnologyGuangzhou 510640People’s Republic of China Tianjin Key Laboratory of Molecular Optoelectronic Sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300350People’s Republic of China State Key Laboratory of Silicon Materials MOE Key Laboratory of Macromolecular Synthesis and FunctionalizationDepartment of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027People’s Republic of China

Recently published in Joule,Feng Liu and colleagues from Shanghai Jiaotong university reported a record-breaking 20.8%power conversion efficiency in organic solar cells(OSCs)with an interpenetrating fibril network active layer morphology,featuring a bulk p-in structure and proper vertical segregation achieved through additive-assisted layer-by-layer *** optimized hierarchical gradient fibrillar morphology and optical management synergistically facilitates exciton diffusion,reduces recombination losses,and enhances light capture *** approach not only offers a solution to achieving high-efficiency devices but also demonstrates the potential for commercial applications of OSCs.

关键词： Organic solar cells Additive-assisted layer-by-layer processing Three-dimensional fibril morphology Bulk p-i-n structure Optical management

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Weak KAM theory for two classes of almost periodic Hamiltonian systems

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Science china Mathematics 2025年

作者： Xun Niu Kaizhi Wang Yong Li School of Mathematics and Statistics Center for Mathematics and Interdisciplinary SciencesNortheast Normal University School of Mathematical Sciences Shanghai Frontier Science Center of Modern Analysis (CMA-Shanghai)Shanghai Jiao Tong University Institute of Mathematics Jilin University

The purpose of this paper is to investigate the dynamics of Bohr almost periodic and Levitan almost periodic Hamiltonian systems via the weak KAM theory. We obtain minimal measures and weak KAM solutions in both cases. The weak KAM solution is a weak solution to the Hamilton-Jacobi equation, which formally transforms the original Hamiltonian systems into an integrable one. Consequently, we get the existence of an invariant torus in the aforementioned weak sense.

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Perfluoropentane-based oxygen-loaded nanodroplets reduce microglial activation through metabolic reprogramming

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Neural Regeneration research 2025年第4期20卷 1178-1191页

作者： Wanxian Luo Chuanhui Xu Linxi Li Yunxiang Ji Yezhong Wang Yingjia Li Yongyi Ye Department of Medicine Ultrasonics Nanfang HospitalSouthern Medical UniversityGuangzhouGuangdong ProvinceChina Institute of Neuroscience Department of NeurosurgeryThe Second Affiliated Hospital of Guangzhou Medical UniversityGuangzhouGuangdong ProvinceChina

Microglia,the primary immune cells within the brain,have gained recognition as a promising therapeutic target for managing neurodegenerative diseases within the central nervous system,including Parkinson’s *** perfluorocarbon droplets have been reported to not only possess a high oxygen-carrying capacity,but also exhibit remarkable anti-inflammatory ***,the role of perfluoropentane in microglia-mediated central inflammatory reactions remains poorly *** this study,we developed perfluoropentane-based oxygen-loaded nanodroplets(PFP-OLNDs)and found that pretreatment with these droplets suppressed the lipopolysaccharide-induced activation of M1-type microglia in vitro and in vivo,and suppressed microglial activation in a mouse model of Parkinson’s *** suppression led to a reduction in the inflammatory response,oxidative stress,and cell migration capacity in ***,the neurotoxic effects were mitigated,which alleviated neuronal ***,ultrahigh-performance liquid chromatography–tandem mass spectrometry showed that the anti-inflammatory effects of PFP-OLNDs mainly resulted from the modulation of microglial metabolic *** further showed that PFP-OLNDs regulated microglial metabolic reprogramming through the AKT-mTOR-HIF-1α***,our findings suggest that the novel PFP-OLNDs constructed in this study alleviate microglia-mediated central inflammatory reactions through metabolic reprogramming.

关键词： metabolic reprogramming microglia microglial migration nanotherapy neurodegenerative diseases neuroinflammation oxygen-loaded nanodroplets Parkinson’s disease perfluoropentane ultra-performance liquid chromatography–mass spectrometry

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2D free-standing ultra-large ferromagnetic nanosheets via a topotactic transformation strategy

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Science china Chemistry 2025年

作者： Haofeng Sun Minghao Wang Wenjie Li Yang Liu Xinyu Sun Wenjie Wang Yuqiao Guo Yi Xie Changzheng Wu Key Laboratory of Precision and Intelligent Chemistry University of Science&Technology of China National Synchrotron Radiation Laboratory University of Science and Technology of China

Considerable progress has been made in synthesizing two-dimensional （2D） materials by exfoliating layered ***,for tremendous non-layered inorganic materials,especially magnet solids,usually with closely packed bulk phases by strong chemical bonds,it is challenging to obtain their high-quality 2D ***,we highlighted a new structure of free-standing ferromagnetic nanosheets featuring （111） *** magnet,Fe3O4,its inversed spinel crystalline has limited abilities to exfoliate into 2D forms and rarely exists as free-standing nanosheets owing to aggregation induced by magnetic *** realized a breakthrough in achieving free-standing ferromagnetic nanosheets with dramatically surpassing size limitations via topotactic conversion from layered *** Fe3O4nanosheets exhibited a maximum width of 60μm while only～4 nm thick,prominently exposing （111） facets.2D Fe3O4behaved anisotropic magnetism,which displayed a 4.6 emu g-1moment（H=500 Oe） in the （111） plane but 2.1 emu g-1out of the （111） plane,indicating a （111） in-plane easy *** anticipated our topotactic conversion strategy would inspire the creation of 2D non-layered materials and enrich the 2D materials family.

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Synthesis and characteristics of large-scale ZnO rods by wet chemical method

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中国有色金属学会会刊：英文版 2008年第5期18卷 1089-1093页

作者：魏素凤蒋青连建设 Key Laboratory of Automobile Materials Ministry of EducationCollege of Materials Science and EngineeringJilin University

The large-scale ZnO rods of submicrometer were prepared on the bare glass using a wet chemical method under different experimental parameters,such as the reactant concentration and the growth *** microstructure of the ZnO rods was characterized by X-ray diffractometry(XRD) and field emission scanning electron microscopy (FESEM) with the energy dispersive X-ray spectroscopy(EDX),and the optical property was investigated by the room-temperature photoluminescence (PL) *** and FESEM results show that the wurtzite structure and rod-like ZnO is *** length (3-8 μm) and the diameter (400 nm-3 μm) vary with the experimental parameters.A strong UV emission at 384 nm and a weak visible yellow-green emission around 570 nm are observed in the PL *** annealing at 600 ℃ in air,the UV peak intensity increases obviously and the yellow-green peak intensity decreases *** near-band-edge UV emission is attributed to the exciton recombination; the yellow-green emission can be associated with the defect recombination; and some defect complexes may be responsible for the latter emission.

关键词：氧化锌湿化学法光致发光退火方法

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Dispersive Liquid-liquid Microextraction for Simultaneous Determination of Six Parabens in Aqueous Cosmetics

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Chemical research in Chinese Universities 2014年第3期30卷 368-373页

作者： WEI Hongmin YANG Jinjuan ZHANG Hanqi SHI Yuhua College of Chemistry Jilin University Changehun 130012 P. R. China

A simple and rapid sample preparation method of dispersive liquid-liquid microextraction（DLLME） was applied in the simultaneous determination of six parabens in the aqueous cosmetics. The analysis was performed on gas chromatography coupled with a flame ionization detection（GC-FID）. The mixed solution containing 30 μL of chloroform（extraction solvent） and 300 μL of tetrahydrofuran（dispersive solvent） was rapidly injected into the sample solution for the purpose of microextraction. After that, the solution mentioned above was centrifuged at 4000 r/min for 10 min, and then the organic sediment phase was detected by GC-FID. The effects of experimental parameters, such as the extraction solvent and the volume of it, and the dispersive solvent and the volume of it, on the yield of the extraction were studied in detail. Under the optimum conditions, the enrichment factors of the target analytes range from 87 to 214. Linearity ranges are 0.05-10.0μg/mL for methylparaben and 0.025--5.0 μg/mL for the other five parabens. The relative standard deviations（RSDs） are lower than 8.2%（n=6）. The proposed method was applied to the analysis of six parabens in eleven aqueous cosmetics. The recoveries of the target analytes in the spiked real samples are in the range of 81.0%-103%.

关键词： Dispersive liquid-liquid microextraction Parabens Aqueous cosmetic Gas chromatography-flame ionization detector

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Influence of preparation methods on photoluminescence properties of ZnO films on quartz glass

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中国有色金属学会会刊：英文版 2008年第1期18卷 145-149页

作者：赵磊连建设刘玉华蒋青 Key Laboratory of Automobile Materials Ministry of EducationCollege of Materials Science and EngineeringJilin University

The influence of preparation methods on the photoluminescence properties of ZnO film was *** methods were applied to fabricate ZnO films in a conventional pulsed laser deposition *** is high temperature(500-700 ℃)oxidation of the metallic zinc film that is obtained by pulsed laser *** other is pulse laser ablation of Zn target in oxygen atmosphere at low temperature(100-250 ℃).The photoluminescence property was detected by PL *** room temperature PL spectra of the ZnO films obtained by oxidation method show single violet luminescence emission centered at 424 nm(or 2.90 eV)without any accompanied deep-level emission and UV *** violet emission is attributed to interstitial zinc in the *** ZnO film with c-axis(002)orientation is obtained by pulsed laser *** ZnO film deposited at 200 ℃ shows single strong ultraviolet *** excellent UV emission is attributed to the good crystalline quality of the film and low intrinsic defects at such low temperature.

关键词： ZnO薄膜脉冲激光光激发光石英玻璃

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Microstructure and property of zinc phosphate coating on die-casting magnesium alloy AZ91D

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中国有色金属学会会刊：英文版 2006年第A02期16卷 70-74页

作者：李光玉连建设牛丽媛江中浩 Key Laboratory of Automobile Materials Ministry of Education College of Materials Science and Engineering Jilin University Changchun 130025 China

A surface treatment method was described, which can form a uniform and dense phosphate conversion coating on the die-casting magnesium alloy AZ91D in a non-chromate and non-nitrite bath. The coating consists of Zn-3(PO4)(2)(.)4H(2)O, Zn, AlPO4 and MgZn2(PO4)(2) analyzed by XRD. The SEM results show that the microstructure of the zinc phosphate coating transfers from flower-like to stab-like crystals with the increase of immersion time of magnesium alloy samples in the phosphating bath. The zinc phosphate coating formed in the bath with immersion time of 1 min is denser because metallic Zn and insoluble phosphate crystals co-deposit on the magnesium alloy surface and the growth of the crystals are restricted by each others. The zinc phosphate coating on the magnesium alloy is used as the base layer for further cataphoric and powder paintings. The cataphoric painting on AZ91D alloy based on phosphate coating has similar adhesion and corrosion-resistance to that based on the chromate conversion coating. But for powder painting, the former exhibits better adhesion property than the latter, due to the uneven microstructure and the enough thickness of the phosphate coating.

关键词：模铸镁合金 AZ91D 磷酸锌涂层显微结构耐蚀性能

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Absorption and dispersion control in a five-level M-type atomic system

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Chinese Physics B 2012年第11期21卷 260-265页

作者：杨红严冬张梅房博张岩吴金辉 College of Physics Jilin University

We investigate the steady optical response of a coherently driven five-level M-type atomic system in three different situations. When all three coupling fields have the same zero detuning, we just find one deep transparency window accompanied by a steep normal dispersion in the probe absorption and dispersion spectra. When two coupling fields are detuned from the relevant transitions to the same extent, however, a second deep transparency window may be observed in the presence of a narrow absorption line of linewidth - 50 kHz. In this case, two single-photon far-detuned transitions can be replaced by a two-photon resonant transition, so the five-level M system in fact reduces into a four-level quasi-A system. Finally, we note that no deep transparency windows and no narrow absorption lines can be found when all three coupling fields have unequal detunings.

关键词： electromagnetically induced transparency absorption and dispersion control narrowspectral linewidth

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Deciphering the role of mtH2O2 in hepatic ischemia-reperfusion injury mechanisms with low-background super-resolution fluorogenic probe

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Science china Chemistry 2025年第01期 297-307页

作者： Bin Fang Limin Wang Haoqin Li Jiaxin Zhang Yang Ding Pan Pan Li Bo Peng Hua Bai Lin Li Frontiers Science Center for Flexible Electronics Xi'an Institute of Flexible Electronics (IFE) and Xi'an Institute of Biomedical Materials &Engineering Northwestern Polytechnical University Institute of Flexible Electronics (IFE Future Technologies) Xiamen University

Hepatic ischemia-reperfusion injury（HIRI） is characterized by mitochondrial dysfunction and oxidative stress. Monitoring mitochondrial hydrogen peroxide（mtH2O2） levels in real-time through super-resolution imaging is crucial for elucidating its distribution in live cells and its mechanism of action during HIRI. However, low-background fluorogenic probes have been overlooked in the context of super-resolution imaging. In this study, we developed a low-background fluorogenic probe（MitoWG） with the potential for super-resolution morphology-correlated mitochondrial identification to track the fluctuates of mtH2O2in HIRI. Activation of the desirable fluorescence properties of the probe by mtH2O2was confirmed using structural illumination microscopy（SIM）, enabling high-quality mitochondrial imaging with exceptional specificity and *** in mtH2O2levels were successfully observed in both cellular and rat models of HIRI. Furthermore, we associated the decline in mitochondrial redox homeostasis with accelerated mtH2O2production during HIRI, which triggered mitophagy deficiency and led to cell death. In conclusion, Mito-WG possesses excellent photophysical and low-background properties for SIM imaging, making it a promising tool for mtH2O2tracking in HIRI research and clinical diagnosis.

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