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Forward modeling and inversion of the relation model between the gas content of plume and its seismic attribute

Acta Oceanologica Sinica 2021年第5期40卷 120-128页

作者： Canping Li Jiachun You Yanchun Tan Fengying Chen Yilin Liu zihao guo Xinyu Tian School of Electronics and Information Engineering Guangdong Ocean UniversityZhanjiang 524088China Southern Marine Science and Engineering Guangdong Laboratory(Zhanjiang) Zhanjiang 524006China School of Geophysics Chengdu University of TechnologyChengdu 610059China

The methane bubble plume attracts interest because it offers direct evidence of seafloor gas leakage and plays an indirect role in the exploration and identification of natural gas *** this study,based on established plume models and their migration sections,three amplitude-class attributes were extracted from three formations for the migration sections of five plumes,and the correlation between the gas content and seismic attribute was *** the gas content increases,the amplitude attribute correspondingly increases,and the linear correlation is relatively ***,correlation coefficients between gas content and amplitude attributes are close to *** using linear fitting,the relation model between the gas content of the plume and the seismic attribute was *** relation model was subsequently used to invert the gas content from a real databearing *** of the gas content section of the plume with the attribute section and real seismic section reveals common distribution characteristics,namely,the color of the section in the lower right corner is *** the amplitude value is large in the seismic section of the real plume,the amplitude attribute value is also large in the corresponding attribute section,and the inverted value of the gas content is also large(because gas content and amplitude are linearly correlated),which indicates that the plume bubbles of the section in the lower right corner is intensively ***,the obtained gas content section of the plume can reflect the distribution of the plume bubble content more simply and intuitively,from which the distribution law of seafloor bubbles can be deduced,and this lays a foundation for the further estimation of the gas content of the plume and hydrate reserves.

关键词： methane plume natural gas hydrate gas content seismic attribute linear fitting

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An active learning workflow for predicting hydrogen atom adsorption energies on binary oxides based on local electronic transfer features

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Green Energy & Environment 2024年第10期9卷 1489-1496页

作者： Wenhao Jing zihao Jiao Mengmeng Song Ya Liu Liejin guo International Research Center for Renewable Energy State Key Laboratory of Multiphase Flow in Power Engineering Xi'an Jiaotong University Department of Energy and Power Engineering Shandong University of Technology

Machine learning combined with density functional theory（DFT） enables rapid exploration of catalyst descriptors space such as adsorption energy, facilitating rapid and effective catalyst screening. However, there is still a lack of models for predicting adsorption energies on oxides,due to the complexity of elemental species and the ambiguous coordination environment. This work proposes an active learning workflow（Le NN） founded on local electronic transfer features（e） and the principle of coordinate rotation invariance. By accurately characterizing the electron transfer to adsorption site atoms and their surrounding geometric structures, Le NN mitigates abrupt feature changes due to different element types and clarifies coordination environments. As a result, it enables the prediction of *H adsorption energy on binary oxide surfaces with a mean absolute error（MAE） below 0.18 e V. Moreover, we incorporate local coverage（θl） and leverage neutral network ensemble to establish an active learning workflow, attaining a prediction MAE below 0.2 e V for 5419 multi-*H adsorption structures. These findings validate the universality and capability of the proposed features in predicting *H adsorption energy on binary oxide surfaces.

关键词： Machine learning Adsorption energy Binary oxide Electron transfer Active learning

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Human Machine Interface with Wearable Electronics Using Biodegradable Triboelectric Films for Calligraphy Practice and Correction

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Nano-Micro Letters 2022年第12期14卷 630-644页

作者： Shen Shen Jia Yi Zhongda Sun zihao guo Tianyiyi He Liyun Ma Huimin Li Jiajia Fu Chengkuo Lee Zhong Lin Wang Jiangsu Engineering Technology Research Center for Functional Textiles Jiangnan UniversityNo.1800 Lihu AvenueWuxiP.R.China Department of Electrical and Computer Engineering National University of Singapore4 Engineering Drive 3Singapore 117576Singapore CAS Center for Excellence in Nanoscience Beijing Key Laboratory of Micro-Nano Energy and SensorBeijing Institute of Nanoenergy and NanosystemsChinese Academy of SciencesBeijing 100083P.R.China China National Textile and Apparel Council Key Laboratory of Natural Dyes Soochow UniversitySuzhou 215123People’s Republic of China School of Material Science and Engineering Georgia Institute of TechnologyAtlantaGA 30332-0245USA

Letter handwriting,especially stroke correction,is of great importance for recording languages and expressing and exchanging ideas for individual behavior and the *** this study,a biodegradable and conductive carboxymethyl chitosan-silk fibroin(CSF)film is prepared to design wearable triboelectric nanogenerator(denoted as CSF-TENG),which outputs of V_(oc)≈165 V,I_(sc)≈1.4μA,and Q_(sc)≈72 mW cm^(−2).Further,in vitro biodegradation of CSF film is performed through trypsin and *** results show that trypsin and lysozyme have stable and favorable biodegradation properties,removing 63.1%of CSF film after degrading for 11 ***,the CSF-TENG-based human-machine interface(HMI)is designed to promptly track writing steps and access the accuracy of letters,resulting in a straightforward communication media of human and *** CSF-TENG-based HMI can automatically recognize and correct three representative letters(F,H,and K),which is benefited by HMI system for data processing and *** CSF-TENG-based HMI can make decisions for the next stroke,highlighting the stroke in advance by replacing it with red,which can be a candidate for calligraphy practice and ***,various demonstrations are done in real-time to achieve virtual and real-world controls including writing,vehicle movements,and healthcare.

关键词： Letter handwriting Triboelectric nanogenerator Biodegradable Human-machine interface Calligraphy practice

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Planar Graphs whose Second Largest Eigenvalue Smaller than ■

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Journal of Mathematical Research with Applications 2024年第1期44卷 1-6页

作者： zihao GENG Jiming guo Department of Mathematics East China University of Science and Technology

A graph G is said to be planar if G can be drawn on the plane in such a way that its edges intersect only at their *** this paper,all the planar graphs without isolated vertices whose second largest eigenvalue smaller... 详细信息

关键词： planar graph the second largest eigenvalue complete product

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High temperature superconductor Na_(2)B_(2)H stabilized by hydrogen intercalation under ambient pressure

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Science China(Physics,Mechanics & Astronomy) 2024年第11期67卷 141-148页

作者： Wendi Zhao Defang Duan Zhengtao Liu zihao Huo Shumin guo Decheng An Maosheng Miao Tian Cui State Key Laboratory of Superhard Materials Key Laboratory of Material Simulation Methods&Software of Ministry of EducationCollege of PhysicsJilin UniversityChangchun 130012China Department of Chemistry and Biochemistry California State UniversityNorthridgeCalifornia 91330USA Department of Earth Science University of CaliforniaSanta BarbaraCalifornia 93106USA Institute of High Pressure Physics School of Physical Science and TechnologyNingbo UniversityNingbo 315211China

Hydrogenated metal borides have attracted much attention due to their potential high-temperature ***,we propose a new strategy for hydrogen intercalation tuning the stability and superconductivity of the boron honeycomb sublattice,and predict an unprecedented layered compound Na_(2)B_(2)H,which hosts excellent ***,the superconducting transition temperature(Tc)of Na_(2)B_(2)H reaches 42 K at ambient *** Tcvalue can be further increase to 63 K under 5%biaxial tensile *** excellent superconductivity originates from the strong electron-phonon coupling between theσ-bonding bands near the Fermi level and the B-B stretching optical E *** interstitial electron localization and crystal orbitals of the H-intercalated Na ion layer well match the boron honeycomb lattice and act as a chemical template to stabilize the B ***,the introduction of hydrogen tuned the Fermi level,and the coupling vibration of Na and H ions effectively enhanced the dynamic stability of the ***_(2)B_(2)H represents a new family of layered high-temperature superconductors,and the strategy of stabilizing the honeycomb boron sublattice via chemical template hosts great potential for application to more layered compounds.

关键词： superconductivity hydrogenation metal borides electron-phonon coupling

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Revealing the Multifunctional Electrocatalysis of Indium-Modulated Phthalocyanine for High-Performance Lithium-Sulfur Batteries

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Energy & Environmental Materials 2024年第1期7卷 1-8页

作者： Yang guo Zhaoqing Jin Jianhao Lu Zilong Wang zihao Song Anbang Wang Weikun Wang Yaqin Huang Beijing Key Laboratory of Electrochemical Process and Technology for Materials Key Laboratory of Biomedical Materials of Natural MacromoleculesMinistry of EducationBeijing University of Chemical TechnologyBeijing 100029China Research Institute of Chemical Defense Beijing Key Laboratory of Advanced Chemical Energy Storage Technology and MaterialsBeijing 100191China

The sluggish kinetics of complicated multiphase conversions and the severe shuttling effect of lithium polysulfides(LiPSs)significantly hinder the applications of Li-S battery,which is one of the most promising candidates for the next-generation energy storage ***,a bifunctional electrocatalyst,indium phthalocyanine self-assembled with carbon nanotubes(InPc@CNT)composite material,is proposed to promote the conversion kinetics of both reduction and oxidation processes,demonstrating a bidirectional catalytic effect on both nucleation and dissolution of Li_(2)S *** theoretical calculation shows that the unique electronic configuration of InPc@CNT is conducive to trapping soluble polysulfides in the reduction process,as well as the modulation of electron transfer dynamics also endows the dissolution of Li_(2)S in the oxidation reaction,which will accelerate the effectiveness of catalytic conversion and facilitate sulfur ***,the InPc@CNT modified separator displays lower overpotential for polysulfide transformation,alleviating polarization of electrode during *** integrated spectroscopy analysis,HRTEM,and electrochemical study reveal that the InPc@CNT acts as an efficient multifunctional catalytic center to satisfy the requirements of accelerating charging and discharging ***,the Li-S battery with InPc@CNT-modified separator obtains a discharge-specific capacity of 1415 mAh g^(-1)at a high rate of 0.5 ***,the 2 Ah Li-S pouch cells deliver 315 Wh kg^(-1)and achieved 80%capacity retention after 50 cycles at 0.1 C with a high sulfur loading of 10 mg cm^(-2).Our study provides a practical method to introduce bifunctional electrocatalysts for boosting the electrochemical properties of Li-S batteries.

关键词： bidirectional catalyst indium phthalocyanine lithium-sulfur batteries pouch cells

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Polyoxometalate as the assembly material to self-assembled Ni(OH)_(2) nanosheets with electrocatalytic performance

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Nano Research 2024年第8期17卷 7061-7067页

作者： Danyang He Tianyang Li Luozhen Jiang Fei Wang zihao Xing Nan Wang Zhiyu Jia guo-Yu Yang Key Laboratory of Cluster Science Ministry of EducationSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China Shanghai Advanced Research Institute Chinese Academy of ScienceShanghai 201210China Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Facluty of ChemistryNortheast Normal UniversityChangchun 130024China

Developing non-noble metal-based electrocatalyst with high catalytic activity is essential for advancing hydrogen energy *** study introduces a hydrothermal method for synthesizing order Ni(OH)_(2) nanosheets,with H_(3)O_(40)PW_(12)(denoted as PW_(12))loaded onto reduced graphene oxide(rGO)coated on nickel foam(referred to as PW_(12)-Ni(OH)_(2)/rGO).This method contrasts with the electrodeposition of Ni(OH)_(2),where PW_(12) is added to the synthetic system to direct the assembly and morphology of the Ni(OH)_(2) through a hydrothermal *** this work,the nickel foam acts dual roles as both the substrate and the source of nickel for the formation of Ni(OH)_(2).The PW_(12)-Ni(OH)_(2)/rGO nanosheets,when successfully prepared and loaded onto the nickel foam(NF),exhibited superior electrocatalytic activity for the hydrogen evolution reaction(HER)in an alkaline electrolyte,achieving a current density of 10 mA·cm^(-2) at an overpotential of 69 ***,we endeavored to expand the application of this material towards the oxygen evolution reaction(OER)by preparing PW_(12)-(Fe/Co)Ni(OH)_(2)/rGO through the addition of metal *** nanocomposite displayed outstanding electrocatalytic activity in alkaline electrolytes,with a current density of 10 mA·cm^(-2)at an overpotential of 211 mV,and demonstrated excellent stability over a 50 h period in a 1 M KOH *** results presented in this paper offer an effective strategy for the preparation of polyoxometalate-based inorganic materials with diverse functionalities,applicable to both HER and OER.

关键词： polyoxometalate Ni(OH)_(2) assembly hydrogen evolution reaction oxygen evolution reaction

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Numerical Simulation Model of Dioxin Production in Grate Furnace-based Municipal Solid Waste Incineration Process

Numerical Simulation Model of Dioxin Production in Grate Fur...

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第37届中国控制会议

作者： zihao guo Jian Tang Junfei Qiao Faculty of Information Technology Beijing University of Technology Beijing Key Laboratory of Computational Intelligence and Intelligent System

Municipal solid waste incineration（MSWI） is the most widely used solid waste treatment techniques. Dioxin（DXN） is a highly toxic and persistent pollutant discharged from MSWI process. The mechanism model of DXN is difficult to establish because of the complex physical and chemical characteristics. In the practical industrial process, DXN emission concentration is off-line detected for monthly or seasonal periods, which cannot be used to operational optimization and feedback control of the MSWI process. In this paper, a numerical simulation model of DXN production based on commercial process simulation soft ware is constructed for a practical MSWI plant. At first, the production mechanism of DXN and a practical MSWI heat and mass balance process are given out. Then, the sensitive analysis of DXN production with several key variables is made based on the constructed numerical model. It shows the constructed numerical simulation model is effective. More detailed works should be done in the future.

关键词： Municipal solid waste incineration (MSWI) Dioxins (DXN) emission concentration Mechanism analysis Numerical simulation Heat and mass balance

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Nanocomposite: Keggin-type Co_(4)-polyoxometalate@cobaltporphyrin linked graphdiyne for hydrogen evolution in seawater

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Nano Research 2024年第3期17卷 1281-1287页

作者： Jiejie Ping Danyang He Fei Wang Nan Wang Yi-cheng Fu zihao Xing Zhiyu Jia guo-Yu Yang Key Laboratory of Cluster Science Ministry of EducationSchool of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 100081China Key Laboratory of Polyoxometalate and Reticular Material Chemistry of Ministry of Education Facluty of Chmeistry Northeast Normal UniversityChangchun 130024China Peking University Third Hospital Beijing 100190China

Polyoxometalate-based nanocomposites with electrocatalytic activity have been applied in hydrogen evolution reactions(HER).Seawater as the main water resource on the earth should be developed as the water electrolysis to prepare high-purity *** this paper,we used two synthesis strategies to prepare the nanocomposite Co_(4)-POM@Co-PGDY(Co_(4)-POM:the Kegging-type microcrystals of K_(10)[Co_(4)(PW_(9)O_(3)4)2]and Co-PGDY:cobalt-porphyrin linked graphdiyne)with excellent activity for ***-PGDY as the porous material is applied not only as the protection of microcrystals towards the metal ion in seawater but also as the co-electrocatalyst of Co_(4)-***_(4)-POM@Co-PGDY exhibits excellent HER performance in seawater electrolytes with low overpotential and high stability at high ***,we have observed a key H_(3)O+intermediate emergence on the surface of nanocomposite during hydrogen evolution process in seawater by Raman synchrotron radiation-based Fourier transform infrared(SR-FTIR).The results in this paper provide an effective strategy for preparing polyoxometalate-based electrocatalysts with high-performance toward hydrogen evolution reaction.

关键词： polyoxometalate graphdiyne seawater hydrogen evolution reaction

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Alignment error modeling and control of a double-sided microlens array during precision glass molding

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Microsystems & Nanoengineering 2024年第2期10卷 311-322页

作者： zihao Zeng Tianfeng Zhou Qian Yu Jia Zhou Gang Wang Qiuchen Xie Zifan Wang Xiaoqiang Yao Yubing guo School of Medical Technology Beijing Institute of TechnologyNo.5 Zhongguancun South StreetHaidian DistrictBeijing100081China School of Mechanical Engineering Beijing Institute of TechnologyNo.5 Zhongguancun South StreetHaidian DistrictBeijing100081China

Double-sided microlens arrays(DSMLAs)include combinations of two single-sided MLAs to overcome positioning errors and greatly improve light transmissivity compared to other types of *** glass molding(PGM)is used to fabricate DSMLAs,but controlling alignment errors during this process is *** this paper,a mold assembly was manufactured with a novel combination of materials to improve the alignment accuracy of mold cores during PGM by using the nonlinear thermal expansion characteristics of the various materials to improve the DSMLA alignment *** establishing a mathematical model of the DSMLA alignment error and a thermal expansion model of the mold-sleeve pair,the relationship between the maximum alignment error of the DSMLA and the mold-sleeve gap was *** research provides a method to optimize the mold-sleeve gap and minimize the alignment error of the *** measured DSMLA alignment error was 10.56μm,which is similar to the predicted maximum alignment *** measurements showed that the uniformity of the homogenized beam spot was 97.81%,and the effective homogeneous area accounted for 91.66%of the total *** proposed method provides a novel strategy to improve the performance of DSMLAs.

关键词： sided alignment error

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