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Immobilization and transformation of co-existing arsenic and antimony in highly contaminated sediment by nano zero-valent iron

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Journal of Environmental Sciences 2022年第2期34卷 152-160页

作者： Jianlong guo Zhipeng Yin Wen zhong Chuanyong Jing State Key Laboratory of Environmental Chemistry and Ecotoxicology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China School of Environmental Science and Engineering Shandong UniversityQingdao 266237China

Arsenic(As)and antimony(Sb)are usually coexistent in mine wastes and pose a great threat to human *** As immobilization by nano zero-valent iron(n ZVI)is promising,however,the stabilization for co-occurring As and Sb is not ***,the immobilization and transformation of As and Sb in n ZVI-treated sediments were evaluated using complementary leaching experiments and characterization *** sediment samples from a gold-antimony deposit revealed the co-existence of ultrahigh As and Sb at 50.3 and 14.9 g/kg,*** results show that As was more efficiently stabilized by n ZVI than Sb,which was primarily due to the soluble fraction that was readily absorbed by n ZVI of As was *** the n ZVI treatment proceeds,the oxidation and reduction of As and Sb occur simultaneously as evidenced by XPS *** primary oxidant,hydroxyl radicals,was detected by EPR studies,proving the occurrence of n ZVI induced Fenton *** study sheds light on differences in the interaction and immobilization of n ZVI with Sb and As in co-contaminated sediments.

关键词： Arsenic Antimony Nano zero-valent iron Immobilization Transformation Leaching

NeurstrucEnergy:A bi-directional GNN model for energy prediction of neural networks in IoT

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Digital Communications and Networks 2024年第2期10卷 439-449页

作者： Chaopeng guo Zhaojin zhong Zexin Zhang Jie Song Software Campus Northeastern UniversityShenyang110000LiaoningChina

A significant demand rises for energy-efficient deep neural networks to support power-limited embedding devices with successful deep learning applications in IoT and edge computing *** accurate energy prediction approach is critical to provide measurement and lead optimization ***,the current energy prediction approaches lack accuracy and generalization ability due to the lack of research on the neural network structure and the excessive reliance on customized training *** paper presents a novel energy prediction model,*** treats neural networks as directed graphs and applies a bi-directional graph neural network training on a randomly generated dataset to extract structural features for energy *** has advantages over linear approaches because the bi-directional graph neural network collects structural features from each layer's parents and *** results show that NeurstrucEnergy establishes state-of-the-art results with mean absolute percentage error of 2.60%.We also evaluate NeurstrucEnergy in a randomly generated dataset,achieving the mean absolute percentage error of 4.83%over 10 typical convolutional neural networks in recent years and 7 efficient convolutional neural networks created by neural architecture *** code is available at https://***/NEUSoftGreenAI/***.

关键词： Internet of things Neural network energy prediction Graph neural networks Graph structure embedding Multi-head attention

Effects of Cultivar on Phenolic Content and Antioxidant Activity of Naked Oat in China

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Journal of Integrative Agriculture 2014年第8期13卷 1809-1816页

作者： TONG Li-tao LIU Li-ya zhong Kui WANG Yan guo Li-na zhou Su-mei Institute of Agro-Products Processing Science and Technology Chinese Academy of Agricultural Sciences/Key Laboratory of Agro-Products ProcessingMinistry of Agriculture

To evaluate the effects of naked oat cultivars on their phenolic contents and antioxidant activities, the oat seeds from 21 different cultivars in China were collected, and their major nutritional components, compositions of polyphenols, and antioxidant activities were measured. As the results, oat cultivars affected its phenolic composition and antioxidant activity significantly. Vanillin, chlorogenic acid, ferulic acid, avenanthramide C（Bc）, avenanthramide A（Bp）, and avenanthramide B（Bf） in oat polyphenols extracts were detected in all cultivars of oat, while caffeic acid, p-coumaric acid and rutin were partly detected. All oat cultivars showed significant free radical scavenging activity, although their activities were lower than that of vitamin C（VC）. Different oat varieties showed different antioxidant activities, among which Yanke 1 had the best ability to scavenge ·OH（（58.78±1.99） μg mL-1）, Baiyan 10 showed the strongest DPPH·（（22.00±0.43） μg mL-1） and ABTS·＋（（6.92±0.44） μg mL-1） scavenging activity, and Dingyou 1 showed good scavenging ability of DPPH·（（22.71±0.42） μg mL-1） and ·OH（（81.50±1.73） μg mL-1）. In addition, the correlation coefficients of contents between the major nutritional components in different cultivars of oat and phenolic compounds indicated that determination of main nutrients could be used as an easy technique to evaluate approximately the contents and compositions of oat polyphenols, which simplifies the selection of good oat cultivar.

关键词： oat phenolics cultivar antioxidant

Relationship between copulation and cold hardiness in Ophraella communa(Coleoptera: Chrysomelidae)

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Journal of Integrative Agriculture 2019年第4期18卷 900-906页

作者： ZHAO Chen-chen YUE Lei WANG Yao guo Jian-ying zhou zhong-shi WAN Fang-hao State Key Laboratory for Biology of Plant Diseases and Insect Pests Institute of Plant Protection Chinese Academy of Agricultural Sciences

Ophraella communa(Coleoptera: Chrysomelidae), the ragweed leaf beetle, is a biological control agent of the invasive common ragweed, Ambrosia artemisiifolia(Asterales: Asteraceae). Adults can survive cold conditions that occur during winter. The adults mate before entering overwintering. Understanding the connection between copulation and overwintering will be useful for determining O. communa seasonality. Determining the relationship between overwintering and copulation required comparison of mated and unmated beetles at mean lethal temperature(LTemp_(50)) exposures for 2 h. Cold-related physiological indices, including the water ratio, super cooling point(SCP), cryoprotectant levels, and energy reserve levels, were also measured. Mating treatment decreased the LTemp_(50) of both sexes by reducing their mean SCP and water ratios. Although the changes of cryoprotectant levels in mated adults were not precisely consistent in between the genders, they increased greatly in both males and females. Body sugar may play a role in copulation and may also elevate cold hardiness in O. communa.

关键词： Ophraella communa mating status cold tolerance hibernation super cooling point energy reserves

Spatiotemporal changeof vegetationcoverage recovery and its driving factors in the Wenchuan earthquake-hit areas

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Journal of Mountain Science 2021年第11期18卷 2854-2869页

作者： SUN Xiao-fei YUAN Lin-guo zhou Ying-zhi SHAO Huai-yong LI Xian-feng zhong Ping Faculty of Geosciences and Environmental Engineering Southwest Jiaotong UniversityChengdu 611756China College of Earth Science Chengdu University of TechnologyChengdu 610059China Natural Resources and Planning Bureau of Nanchong Nanchong 637000China Department of Geography National University of SingaporeKent Ridge 117570Singapore

Vegetation coverage recovery after the Wenchuan earthquake has important implications for preventing post-seismic geohazards and soil ***,spatiotemporal changes in vegetation coverage recovery and its driving factors have not been sufficiently studied in the quake-hit *** paper aims to analyze vegetation coverage recovery and its driving factors in the quake-hit areas using monadic linear regression,coefficient of variation,and geographical ***,we used Moderate-resolution Imaging Spectroradiometer(MODIS)data to calculate the vegetation coverage from 2008 to 2018 in the quake-hit ***,we assessed the trend and stability of vegetation recovery in the quake-hit areas based on vegetation ***,combined with topography,climate,soil type,vegetation type,and human activities in the quake-hit areas,the driving factors affecting vegetation coverage recovery were *** results showed that the vegetation coverage level in the quake-hit areas recovered about 90%of that before the *** coverage recovery was mainly improved in a stepwise manner:increasing and then stabilizing,then increasing and stabilizing ***,soil type,and road density were the main factors affecting vegetation coverage recovery,and the interaction among all factors positively strengthened their impacts on vegetation coverage *** addition,the results also revealed the categories that were conducive to vegetation coverage recovery among the same environmental factors and can provide a scientific reference for vegetation coverage recovery in the quake-hit areas.

关键词： Wenchuan earthquake Vegetation coverage recovery Geographical detector Driving factors

Moxibustion inhibits the macrophage M1 polarization toll-like receptor 4/myeloid differentiation factor 88/nuclear factor kappa B signaling pathway by regulating T-cell immunoglobulin and mucin-containing protein-3 in rheumatoid arthritis

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Journal of Traditional Chinese Medicine 2024年第6期44卷 1227-1235页

作者： LUO Kun zhong Yumei guo Yanding ZHANG Linlin HU Danhui MA Wenbin YANG Xin zhou Haiyan Acupuncture and Tuina School Chengdu University of Traditional Chinese MedicineChengdu 610075China Department of Painology Chengdu Integrated TCM&Western Medicine Hospital/Chengdu First People's HospitalChengdu 610095China Health Rehabilitation School Chengdu University of Traditional Chinese MedicineChengdu 610075China

OBJECTIVE: To explore whether moxibustion exerts therapeutic effects on rheumatoid arthritis(RA) by regulating the expression of T-cell immunoglobulin and mucin-containing protein-3(TIM-3) and subsequently modulating the macrophage M1 polarization toll-like receptor 4(TLR4)-myeloid differentiation factor 88(My D88)-nuclear factor kappa B(NF-κB) signaling pathway. METHODS: We utilized moxibustion treatment in RA rat models using the Zusanli(ST36) and Shenshu(BL23) acupoints. Hematoxylin and eosin(HE) staining was used to observe the pathological changes of the synovial tissue under a section light microscope, and pathological scoring was performed according to the grading standard of the degree of synovial tissue disease. Enzyme-linked immunosorbent assay(ELISA) was applied to verify the efficacy of moxibustion in reducing inflammation. Quantitative real-time polymerase chain reaction(q RTPCR) was used to detect the expression of the TIM-3/TLR4-My D88-NF-κB signaling pathway-related molecules, and Western blot was used to detect the contents of synovial NF-κB. RESULTS: We established the Freund's complete adjuvant(FCA)-induced RA model in rats. The expression level of M1 polarization signaling pathway TLR4-My D88-NF-κB and the inflammatory factors interleukin-12(IL-12), tumor necrosis factor alpha(TNF-α), and tumor necrosis factor beta(TNF-β) were significantly increased in the RA model. After moxibustion treatment, the expression level of TLR4-My D88-NF-κB was significantly decreased, and the inflammatory factors IL-12, TNF-α, and TNF-β were decreased, but the expression level was significantly increased in the RA model. When TIM-3 expression was inhibited, the expression level of TLR4-My D88-NF-κB, and the inflammatory factors IL-12, TNF-α, and TNF-β were not suppressed, even after moxibustion treatment. CONCLUSIONS: Moxibustion regulates the key target TIM-3 by acting on the Zusanli(ST36) and Shenshu(BL23) points, thereby inhibiting the M1 polarization of macropha

关键词： moxibustion arthritis rheumatoid TIM-3 macrophage polarization toll-like receptor 4 myeloid differentiation factor 88 nuclear factor kappa B signal transduction

Evaluation of the WRF Model with Different Land Surface Schemes: A Drought Event Simulation in Southwest China during 2009–10

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Atmospheric and Oceanic Science Letters 2014年第2期7卷 168-173页

作者： HU Zu-Heng XU zhong-Feng zhou Ning-Fang MA Zhu-guo LI guo-Ping Key Laboratory of Regional Climate-Environment Research for East Asia Institute of Atmospheric Physics Chinese Academy of Sciences College of Atmospheric Sciences Chengdu University of Information Technology Young Scientists Laboratory Institute of Atmospheric Physics Chinese Academy of Sciences National Meteorological Center China Meteorological Administration

The authors examined the performance of version 3.4.1 of the Weather Research and Forecasting Model(WRF) with various land surface schemes in simulating a severe drought event in Southwest China. Five numerical experiments were completed using the Noah land surface scheme, the Pleim-Xiu land surface scheme, the Noah-MP land surface schemes, the Noah- MP scheme with dynamic vegetation, and the Noah-MP scheme with dynamic vegetation and groundwater processes. In general, all the simulations reasonably reproduced the spatial and temporal variations in precipitation, but significant bias was also found, especially for the spatial pattern of simulated precipitation. The WRF simulations with the Noah-MP series land surface schemes performed slightly better than the WRF simulation with the Noah and Pleim-Xiu land surface schemes in reproducing the severe drought events in Southwest China. The leaf area index(LAI) simulated by the different land surface schemes showed significant deviations in Southwest China. The Pleim-Xiu scheme overestimated the value of LAI by a factor of two. The Noah-MP scheme with dynamical vegetation overestimated the magnitude of the annual cycle of the LAI, although the annual mean LAI was close to observations. The simulated LAI showed a long-term lower value from autumn 2009 to spring 2010 relative to normal years. This indicates that the LAI is a potential indictor to monitor drought events.

关键词： land surface model drought Southwest China Noah-MP precipitation leaf area index

Thermal Decomposition of Ammonium 3-Nitro-1,2,4-triazol-5-onate Monohydrate

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Chemical Research in Chinese Universities 2008年第6期24卷 786-789页

作者： LI Ji-zhen FAN Xue-zhong ZHANG Jiao-qiang ZHANG guo-fang WANG Bo-zhou Xi＇an Modern Chemistry Research Institute Xi＇an 710065 P R. China School of Science Northwestern Polytechnical University Xi＇an 710072 P R. China School of Chemistry and Materials Science Shaanxi Normal University Xi＇an 710062 P. R. China

The thermal decomposition of ammonium 3-nitro-1,2,4-triazol-5-onate monohydrate[NH4（NTO）·H2O] was studied by means of thermal analysis-MS coupling and the combination technique of in situ thermolysis cell with rapid-scan Fourier transform infrared spectroscopy. The results show that there are two endothermic steps and one exothermic step in the decomposition process of NH4（NTO）·H2O. The detected gas products consist of NH3, H2O, N2, CO2, CO, and NO2.

关键词： Ammonium 3-nitro-1,2,4-triazol-5-onate monohydrate Thermal decomposition DSC TG MS IR

Phosphorus migration mechanism between iron and high phosphorus gangue phase at high temperatures

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Journal of Iron and Steel Research International 2019年第2期26卷 113-122页

作者： Lei guo Jin-tao Gao Sheng-ping zhong Zhan-cheng guo State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China

The phosphorus migration mechanism during melting separation of non-carbon-reduced high phosphorus iron ore was ***,the equilibrium compositions of hydrogen-reduced high phosphorus iron ore at different temperatures were simulated by the use of equilibrium composition module of HSC Chemistry ***,thermodynamic calculation was verified by the real heat treatment of simulated hydrogen-reduced high phosphorus iron ore with several pure reagents including self-made pure *** iron particles in the simulated samples gathered and grew up during heat ***,the hypoeutectic structure of Fe-P with grid shape of high phosphorus phase and circular shape of low phosphorus phase emerged within those iron *** the penetration of phosphorus from the periphery into the iron particles,the grid structure became denser and *** proves that the elemenlal phosphorus can be reduced from the gangue phase by metallic iron without solid carbon at high temperatures.

关键词： Melting separation Fluorapatite Thermodynamics Phosphorus migration High phosphorus iron ore